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Reusable nitrogen-doped mesoporous carbon adsorbent for carbon dioxide adsorption in fixed-bed

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  • Yaumi, A.L.
  • Bakar, M.Z. Abu
  • Hameed, B.H.

Abstract

Reusable nitrogen-doped carbon derived from coconut shell was prepared as a sustainable alternative for carbon dioxide (CO2) adsorption from gas streams. The procedure is based on carbonization and chemical activation with coconut shell, glucosamine, and KOH as the activating agent. The textural properties, as well as the fixed-bed adsorption and regeneration performance of the adsorbent were investigated using the fixed-bed adsorption column. The surface nature and properties of the adsorbent changed remarkably due to the surface modification that enhanced the adsorption process. The adsorbent showed a maximum CO2 uptake of 4.23 mmol/g at 30 °C and 1 bar. CO2 adsorption capacity increased with initial concentration and decreased with increases in temperature and flowrate. The adsorption capacity and physiochemical properties of the adsorbent were preserved after 20 adsorption–desorption cycles without significant loss in capacity. This finding suggests that the synthesized adsorbent is a good candidate for CO2 capture from post-fossil fuel combustion processes.

Suggested Citation

  • Yaumi, A.L. & Bakar, M.Z. Abu & Hameed, B.H., 2017. "Reusable nitrogen-doped mesoporous carbon adsorbent for carbon dioxide adsorption in fixed-bed," Energy, Elsevier, vol. 138(C), pages 776-784.
    • Handle: RePEc:eee:energy:v:138:y:2017:i:c:p:776-784
    DOI: 10.1016/j.energy.2017.07.130
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    Cited by:

    1. Park, Jaewoo & Attia, Nour F. & Jung, Minji & Lee, Myoung Eun & Lee, Kiyoung & Chung, Jaewoo & Oh, Hyunchul, 2018. "Sustainable nanoporous carbon for CO2, CH4, N2, H2 adsorption and CO2/CH4 and CO2/N2 separation," Energy, Elsevier, vol. 158(C), pages 9-16.
    2. Alves, Luís & Pereira, Vítor & Lagarteira, Tiago & Mendes, Adélio, 2021. "Catalytic methane decomposition to boost the energy transition: Scientific and technological advancements," Renewable and Sustainable Energy Reviews, Elsevier, vol. 137(C).
    3. Mirzaeian, Mojtaba & Abbas, Qaisar & Gibson, Des & Mazur, Michal, 2019. "Effect of nitrogen doping on the electrochemical performance of resorcinol-formaldehyde based carbon aerogels as electrode material for supercapacitor applications," Energy, Elsevier, vol. 173(C), pages 809-819.
    4. Yaumi, A.L. & Bakar, M.Z. Abu & Hameed, B.H., 2018. "Melamine-nitrogenated mesoporous activated carbon derived from rice husk for carbon dioxide adsorption in fixed-bed," Energy, Elsevier, vol. 155(C), pages 46-55.
    5. He Gao & Shaohua Wang & Miaomiao Hao & Wei Shao & Shuhui Zhang & Lei Zhang & Xiaohan Ren, 2023. "CO 2 Adsorption Performance of Activated Coke Prepared from Biomass and Coal," Energies, MDPI, vol. 16(9), pages 1-21, May.
    6. Jian Yu & Lirong Zhang & Bin Liu, 2019. "Adsorption of Malachite Green with Sodium Dodecylbenzene Sulfonate Modified Sepiolite: Characterization, Adsorption Performance and Regeneration," IJERPH, MDPI, vol. 16(18), pages 1-14, September.

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