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CFD simulation of CO2 sorption on K2CO3 solid sorbent in novel high flux circulating-turbulent fluidized bed riser: Parametric statistical experimental design study

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  • Thummakul, Theeranan
  • Gidaspow, Dimitri
  • Piumsomboon, Pornpote
  • Chalermsinsuwan, Benjapon

Abstract

In this study a high flux circulating-turbulent fluidized bed (CTFB) riser was confirmed to be advantageous for carbon dioxide (CO2) sorption on a potassium carbonate solid sorbent. The effect of various parameters on the CO2 removal level was evaluated using a statistical experimental design. The most appropriate fluidization regime was found to occur between the turbulent and fast fluidization regimes, which was shown to capture CO2 more efficiently than conventional fluidization regimes. The highest CO2 sorption level was 93.4% under optimized CTFB operating conditions. The important parameters for CO2 capture were the inlet gas velocity and the interactions between the CO2 concentration and the inlet gas velocity and water vapor concentration. The CTFB regime had a high and uniform solid particle distribution in both the axial and radial system directions and could transport the solid sorbent to the regeneration reactor. In addition, the process system continuity had a stronger effect on the CO2 removal level in the system than the process system mixing.

Suggested Citation

  • Thummakul, Theeranan & Gidaspow, Dimitri & Piumsomboon, Pornpote & Chalermsinsuwan, Benjapon, 2017. "CFD simulation of CO2 sorption on K2CO3 solid sorbent in novel high flux circulating-turbulent fluidized bed riser: Parametric statistical experimental design study," Applied Energy, Elsevier, vol. 190(C), pages 122-134.
    • Handle: RePEc:eee:appene:v:190:y:2017:i:c:p:122-134
    DOI: 10.1016/j.apenergy.2016.12.110
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    1. Qin, Changlei & Yin, Junjun & Ran, Jingyu & Zhang, Li & Feng, Bo, 2014. "Effect of support material on the performance of K2CO3-based pellets for cyclic CO2 capture," Applied Energy, Elsevier, vol. 136(C), pages 280-288.
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    6. Guo, Yafei & Zhao, Chuanwen & Li, Changhai & Lu, Shouxiang, 2014. "Application of PEI–K2CO3/AC for capturing CO2 from flue gas after combustion," Applied Energy, Elsevier, vol. 129(C), pages 17-24.
    7. Zhao, Wenying & Sprachmann, Gerald & Li, Zhenshan & Cai, Ningsheng & Zhang, Xiaohui, 2013. "Effect of K2CO3·1.5H2O on the regeneration energy consumption of potassium-based sorbents for CO2 capture," Applied Energy, Elsevier, vol. 112(C), pages 381-387.
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    Cited by:

    1. Choi, Seungyeong & Yun, Maroosol & Kim, Kiwoong & Park, Yong-Ki & Cho, Hyung Hee, 2022. "Energy-efficient design of dual circulating fluidized bed system for CCUS by multi-tube configuration with junctions," Energy, Elsevier, vol. 245(C).
    2. Park, Junhyung & Won, Wangyun & Jung, Wonho & Lee, Kwang Soon, 2019. "One-dimensional modeling of a turbulent fluidized bed for a sorbent-based CO2 capture process with solid–solid sensible heat exchange," Energy, Elsevier, vol. 168(C), pages 1168-1180.
    3. Tritippayanon, Rattapong & Piemjaiswang, Ratchanon & Piumsomboon, Pornpote & Chalermsinsuwan, Benjapon, 2019. "Computational fluid dynamics of sulfur dioxide and carbon dioxide capture using mixed feeding of calcium carbonate/calcium oxide in an industrial scale circulating fluidized bed boiler," Applied Energy, Elsevier, vol. 250(C), pages 493-502.
    4. Zhang, Xiaowen & Zhang, Xin & Liu, Helei & Li, Wensheng & Xiao, Min & Gao, Hongxia & Liang, Zhiwu, 2017. "Reduction of energy requirement of CO2 desorption from a rich CO2-loaded MEA solution by using solid acid catalysts," Applied Energy, Elsevier, vol. 202(C), pages 673-684.
    5. Ju, Youngsan & Lee, Chang-Ha, 2019. "Dynamic modeling of a dual fluidized-bed system with the circulation of dry sorbent for CO2 capture," Applied Energy, Elsevier, vol. 241(C), pages 640-651.

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