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Application of PEI–K2CO3/AC for capturing CO2 from flue gas after combustion

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  • Guo, Yafei
  • Zhao, Chuanwen
  • Li, Changhai
  • Lu, Shouxiang

Abstract

The capture of CO2 from flue gas after combustion using solid sorbents is one of the efficient options for reducing CO2 emissions from fossil fuel-fired power plants. To satisfy the requirement of large quantities flue gas treatment, the CO2 capture capacities of the solid sorbents must be focused on. In order to obtain a sorbent with high CO2 capture capacity, a novel PEI–K2CO3/AC sorbent was prepared by impregnating potassium carbonate (K2CO3) and polyethylenimine (PEI) on activated carbon (AC) in this work. The CO2 capture performance of this sorbent was investigated using a fixed bed reactor system. The CO2 capture capacity of PEI–K2CO3/AC with the total K2CO3 and PEI loadings of 50wt% was measured as 3.60mmol CO2/g under the condition of 60°C, 8% CO2+10% H2O. In addition, this sorbent is proved to be regenerable and stable during 5 cycle CO2 sorption–desorption tests. Compared with K2CO3/AC (loading of 58wt%) and PEI/AC (loading of 43wt%), PEI–K2CO3/AC presents higher CO2 capture capacity and long-term stability. Therefore, PEI–K2CO3/AC should be considered as a new option for capturing CO2 from flue gas after combustion.

Suggested Citation

  • Guo, Yafei & Zhao, Chuanwen & Li, Changhai & Lu, Shouxiang, 2014. "Application of PEI–K2CO3/AC for capturing CO2 from flue gas after combustion," Applied Energy, Elsevier, vol. 129(C), pages 17-24.
    • Handle: RePEc:eee:appene:v:129:y:2014:i:c:p:17-24
    DOI: 10.1016/j.apenergy.2014.05.003
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    2. Qin, Changlei & Yin, Junjun & Ran, Jingyu & Zhang, Li & Feng, Bo, 2014. "Effect of support material on the performance of K2CO3-based pellets for cyclic CO2 capture," Applied Energy, Elsevier, vol. 136(C), pages 280-288.
    3. Qin, Qiaoyun & Liu, Hongyan & Zhang, Riguang & Ling, Lixia & Fan, Maohong & Wang, Baojun, 2018. "Application of density functional theory in studying CO2 capture with TiO2-supported K2CO3 being an example," Applied Energy, Elsevier, vol. 231(C), pages 167-178.
    4. Fan Yu & Ye Wu & Wenjing Zhang & Tianyi Cai & Yuhao Xu & Xiaoping Chen, 2016. "A novel aerogel sodium‐based sorbent for low temperature CO 2 capture," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 6(4), pages 561-573, August.
    5. Thummakul, Theeranan & Gidaspow, Dimitri & Piumsomboon, Pornpote & Chalermsinsuwan, Benjapon, 2017. "CFD simulation of CO2 sorption on K2CO3 solid sorbent in novel high flux circulating-turbulent fluidized bed riser: Parametric statistical experimental design study," Applied Energy, Elsevier, vol. 190(C), pages 122-134.
    6. Junya Wang & Qiuyun Pu & Ping Ning & Shijian Lu, 2021. "Activated carbon‐based composites for capturing CO2: a review," Greenhouse Gases: Science and Technology, Blackwell Publishing, vol. 11(2), pages 377-393, April.
    7. Kong, Yong & Shen, Xiaodong & Cui, Sheng & Fan, Maohong, 2015. "Development of monolithic adsorbent via polymeric sol–gel process for low-concentration CO2 capture," Applied Energy, Elsevier, vol. 147(C), pages 308-317.
    8. Chen, S.J. & Zhu, M. & Fu, Y. & Huang, Y.X. & Tao, Z.C. & Li, W.L., 2017. "Using 13X, LiX, and LiPdAgX zeolites for CO2 capture from post-combustion flue gas," Applied Energy, Elsevier, vol. 191(C), pages 87-98.
    9. Ren, Yanping & Ding, Ruiyu & Yue, Hairong & Tang, Siyang & Liu, Changjun & Zhao, Jinbo & Lin, Wen & Liang, Bin, 2017. "Amine-grafted mesoporous copper silicates as recyclable solid amine sorbents for post-combustion CO2 capture," Applied Energy, Elsevier, vol. 198(C), pages 250-260.

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