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Lithium-ion storage capacitors achieved by CVD graphene/TaC/Ta-wires and carbon hollow spheres

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  • Zhao, Liwei
  • Li, Hongji
  • Li, Mingji
  • Xu, Sheng
  • Li, Cuiping
  • Qu, Changqing
  • Zhang, Lijun
  • Yang, Baohe

Abstract

Lithium-ion storage capacitors were assembled using graphene/tantalum carbide/tantalum wire electrodes and carbon hollow spheres as electrolyte. The graphene/tantalum carbide layers were prepared by electron-assisted hot filament chemical vapor deposition; the carbon hollow spheres were synthesized by hydrothermal reaction and pyrolysis treatment. The specific capacitance of the capacitor was 593Fg−1 at a current density of 10Ag−1. The capacitor showed excellent cycling stability, retaining 91.2% of its initial capacitance after 8000 cycles. Moreover, the capacitor provided a high specific energy density of 132Whkg−1 at a high power density of 3.17kWkg−1. The high energy density is attributed to the widened operation window ranging from 0 to 3.0V. The graphene layer of the electrode and carbon hollow spheres in electrolyte synergistic affect influence on the electrochemical performance of the capacitor are discussed. In addition, the use of a low-cost lithium salt, lithium chloride, is also featured in this paper.

Suggested Citation

  • Zhao, Liwei & Li, Hongji & Li, Mingji & Xu, Sheng & Li, Cuiping & Qu, Changqing & Zhang, Lijun & Yang, Baohe, 2016. "Lithium-ion storage capacitors achieved by CVD graphene/TaC/Ta-wires and carbon hollow spheres," Applied Energy, Elsevier, vol. 162(C), pages 197-206.
  • Handle: RePEc:eee:appene:v:162:y:2016:i:c:p:197-206
    DOI: 10.1016/j.apenergy.2015.10.093
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    References listed on IDEAS

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    Cited by:

    1. Zhu, Wenhua H. & Tatarchuk, Bruce J., 2016. "Characterization of asymmetric ultracapacitors as hybrid pulse power devices for efficient energy storage and power delivery applications," Applied Energy, Elsevier, vol. 169(C), pages 460-468.
    2. Hemmati, Reza & Azizi, Neda, 2017. "Advanced control strategy on battery storage system for energy management and bidirectional power control in electrical networks," Energy, Elsevier, vol. 138(C), pages 520-528.
    3. Xu, Jun & Tang, Hao & Su, Sheng & Liu, Jiawei & Xu, Kai & Qian, Kun & Wang, Yi & Zhou, Yingbiao & Hu, Song & Zhang, Anchao & Xiang, Jun, 2018. "A study of the relationships between coal structures and combustion characteristics: The insights from micro-Raman spectroscopy based on 32 kinds of Chinese coals," Applied Energy, Elsevier, vol. 212(C), pages 46-56.

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