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Effect of operating parameters on the transient performance of a polymer electrolyte membrane fuel cell stack with a dead-end anode

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  • Gomez, Alberto
  • Raj, Abhishek
  • Sasmito, Agus P.
  • Shamim, Tariq

Abstract

The operation of polymer electrolyte membrane fuel cell (PEMFC) stack with a dead-end anode requires careful consideration on the gas and water management. Water accumulation at the anode and the nitrogen crossover from cathode to anode lead to performance deterioration over time. The accumulated water and nitrogen need to be removed properly by purging method to ensure good and stable stack performance. Thus, the careful selection of the operating parameters – inlet humidification, stoichiometry, and operating current – is the key factor for ensuring efficient water and gas management. This study aims at the experimental and numerical evaluation of the effect of the key operating parameters on the transient performance of a dead-end anode fuel cell stack. The experiments were carried out on a stack with 24 cells and a catalyst active area of 300cm2. By employing a validated transient two-phase mathematical model of a PEMFC with a dead-end anode, numerical simulations were performed which yield a better and deeper understanding of local distribution of water and species, i.e., hydrogen, oxygen, water vapor and nitrogen.

Suggested Citation

  • Gomez, Alberto & Raj, Abhishek & Sasmito, Agus P. & Shamim, Tariq, 2014. "Effect of operating parameters on the transient performance of a polymer electrolyte membrane fuel cell stack with a dead-end anode," Applied Energy, Elsevier, vol. 130(C), pages 692-701.
    • Handle: RePEc:eee:appene:v:130:y:2014:i:c:p:692-701
    DOI: 10.1016/j.apenergy.2013.12.030
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    1. Wan, Zhongmin & Liu, Jing & Luo, Zhiping & Tu, Zhengkai & Liu, Zhichun & Liu, Wei, 2013. "Evaluation of self-water-removal in a dead-ended proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 104(C), pages 751-757.
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    1. De las Heras, A. & Vivas, F.J. & Segura, F. & Redondo, M.J. & Andújar, J.M., 2018. "Air-cooled fuel cells: Keys to design and build the oxidant/cooling system," Renewable Energy, Elsevier, vol. 125(C), pages 1-20.
    2. Ettihir, K. & Boulon, L. & Agbossou, K., 2016. "Optimization-based energy management strategy for a fuel cell/battery hybrid power system," Applied Energy, Elsevier, vol. 163(C), pages 142-153.
    3. Wang, Bowen & Deng, Hao & Jiao, Kui, 2018. "Purge strategy optimization of proton exchange membrane fuel cell with anode recirculation," Applied Energy, Elsevier, vol. 225(C), pages 1-13.
    4. Jang, Jer-Huan & Yan, Wei-Mon & Chiu, Han-Chieh & Lui, Jun-Yi, 2015. "Dynamic cell performance of kW-grade proton exchange membrane fuel cell stack with dead-ended anode," Applied Energy, Elsevier, vol. 142(C), pages 108-114.
    5. Liu, Guicheng & Li, Xinyang & Wang, Hui & Liu, Xiuying & Chen, Ming & Woo, Jae Young & Kim, Ji Young & Wang, Xindong & Lee, Joong Kee, 2017. "Design of 3-electrode system for in situ monitoring direct methanol fuel cells during long-time running test at high temperature," Applied Energy, Elsevier, vol. 197(C), pages 163-168.
    6. Kim, Bosung & Cha, Dowon & Kim, Yongchan, 2015. "The effects of air stoichiometry and air excess ratio on the transient response of a PEMFC under load change conditions," Applied Energy, Elsevier, vol. 138(C), pages 143-149.
    7. Soopee, Asif & Sasmito, Agus P. & Shamim, Tariq, 2019. "Water droplet dynamics in a dead-end anode proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 233, pages 300-311.
    8. Chen, Huicui & Zhao, Xin & Qu, Bingwang & Zhang, Tong & Pei, Pucheng & Li, Congxin, 2018. "An evaluation method of gas distribution quality in dynamic process of proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 232(C), pages 26-35.
    9. Wu, Horng-Wen, 2016. "A review of recent development: Transport and performance modeling of PEM fuel cells," Applied Energy, Elsevier, vol. 165(C), pages 81-106.
    10. Kang, Sanggyu & Zhao, Li & Brouwer, Jacob, 2019. "Dynamic modeling and verification of a proton exchange membrane fuel cell-battery hybrid system to power servers in data centers," Renewable Energy, Elsevier, vol. 143(C), pages 313-327.
    11. Kurnia, Jundika C. & Sasmito, Agus P. & Shamim, Tariq, 2019. "Advances in proton exchange membrane fuel cell with dead-end anode operation: A review," Applied Energy, Elsevier, vol. 252(C), pages 1-1.
    12. Zhang, Qian & Lin, Rui & Técher, Ludovic & Cui, Xin, 2016. "Experimental study of variable operating parameters effects on overall PEMFC performance and spatial performance distribution," Energy, Elsevier, vol. 115(P1), pages 550-560.
    13. Chen, Ben & Ke, Wandi & Luo, Maji & Wang, Jun & Tu, Zhengkai & Pan, Mu & Zhang, Haining & Liu, Xiaowei & Liu, Wei, 2015. "Operation characteristics and carbon corrosion of PEMFC (Proton exchange membrane fuel cell) with dead-ended anode for high hydrogen utilization," Energy, Elsevier, vol. 91(C), pages 799-806.
    14. Chen, Ben & Wang, Jun & Yang, Tianqi & Cai, Yonghua & Zhang, Caizhi & Chan, Siew Hwa & Yu, Yi & Tu, Zhengkai, 2016. "Carbon corrosion and performance degradation mechanism in a proton exchange membrane fuel cell with dead-ended anode and cathode," Energy, Elsevier, vol. 106(C), pages 54-62.
    15. Wu, Ziyao & Pei, Pucheng & Xu, Huachi & Jia, Xiaoning & Ren, Peng & Wang, Bozheng, 2019. "Study on the effect of membrane electrode assembly parameters on polymer electrolyte membrane fuel cell performance by galvanostatic charging method," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    16. Myo-Eun Kim & Young-Jun Sohn, 2020. "Study on Polymer Electrolyte Fuel Cells with Nonhumidification Using Metal Foam in Dead-Ended Operation," Energies, MDPI, vol. 13(5), pages 1-12, March.

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