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Development of amino acid and amino acid-complex based solid sorbents for CO2 capture

Author

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  • Jiang, Bingbing
  • Wang, Xianfeng
  • Gray, McMahan L.
  • Duan, Yuhua
  • Luebke, David
  • Li, Bingyun

Abstract

For the first time, amino acid (AA) and AA-complex based solid sorbents for CO2 removal were investigated by immobilizing AAs and AA-complexes into porous polymethylmethacrylate (PMMA) microspheres. Deposition of pure AAs into porous PMMA supports led to limited CO2 adsorption in sorbents, because large AA particles or crystals were formed during deposition of pure AAs into PMMA microspheres and some pores of the PMMA microspheres were clogged. Among the AA sorbents studied, Arginine (Arg) solid sorbents had the highest CO2 adsorption capacity. Interestingly, by forming AA-complexes with other polymers, we substantially improved AA water solubility, achieved uniform immobilization of AAs inside PMMA microspheres, and obtained high CO2 adsorption capacity. We found that the types of AA-complexes, complex loading capacity, and ratio of AAs in the complexes could have significant effects on CO2 adsorption properties. Especially, complexing Arg with a strong polyelectrolyte (i.e. polystyrene sulfonate) resulted in substantially improved AA water solubility and high CO2 adsorption capacity. Our developed AA-complex based solid sorbents could be innovative since they could eliminate concerns related to potential equipment corrosion as well as high heat duty associated with aqueous solvent regeneration all the while retaining the advantageous properties (high thermal stability, excellent biocompatibility, and negligible volatility) of AAs.

Suggested Citation

  • Jiang, Bingbing & Wang, Xianfeng & Gray, McMahan L. & Duan, Yuhua & Luebke, David & Li, Bingyun, 2013. "Development of amino acid and amino acid-complex based solid sorbents for CO2 capture," Applied Energy, Elsevier, vol. 109(C), pages 112-118.
    • Handle: RePEc:eee:appene:v:109:y:2013:i:c:p:112-118
    DOI: 10.1016/j.apenergy.2013.03.070
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    References listed on IDEAS

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    2. Luis Míguez, José & Porteiro, Jacobo & Pérez-Orozco, Raquel & Patiño, David & Rodríguez, Sandra, 2018. "Evolution of CO2 capture technology between 2007 and 2017 through the study of patent activity," Applied Energy, Elsevier, vol. 211(C), pages 1282-1296.
    3. Grace, Andrews Nirmala & Choi, Song Yi & Vinoba, Mari & Bhagiyalakshmi, Margandan & Chu, Dae Hyun & Yoon, Yeoil & Nam, Sung Chan & Jeong, Soon Kwan, 2014. "Electrochemical reduction of carbon dioxide at low overpotential on a polyaniline/Cu2O nanocomposite based electrode," Applied Energy, Elsevier, vol. 120(C), pages 85-94.
    4. Guo, Yafei & Zhao, Chuanwen & Chen, Xiaoping & Li, Changhai, 2015. "CO2 capture and sorbent regeneration performances of some wood ash materials," Applied Energy, Elsevier, vol. 137(C), pages 26-36.
    5. Ganapathy, Harish & Steinmayer, Sascha & Shooshtari, Amir & Dessiatoun, Serguei & Ohadi, Michael M. & Alshehhi, Mohamed, 2016. "Process intensification characteristics of a microreactor absorber for enhanced CO2 capture," Applied Energy, Elsevier, vol. 162(C), pages 416-427.
    6. Wang, Xianfeng & Akhmedov, Novruz G. & Hopkinson, David & Hoffman, James & Duan, Yuhua & Egbebi, Adefemi & Resnik, Kevin & Li, Bingyun, 2016. "Phase change amino acid salt separates into CO2-rich and CO2-lean phases upon interacting with CO2," Applied Energy, Elsevier, vol. 161(C), pages 41-47.
    7. Ganapathy, H. & Shooshtari, A. & Dessiatoun, S. & Alshehhi, M. & Ohadi, M., 2014. "Fluid flow and mass transfer characteristics of enhanced CO2 capture in a minichannel reactor," Applied Energy, Elsevier, vol. 119(C), pages 43-56.
    8. Guo, Yafei & Zhao, Chuanwen & Li, Changhai & Lu, Shouxiang, 2014. "Application of PEI–K2CO3/AC for capturing CO2 from flue gas after combustion," Applied Energy, Elsevier, vol. 129(C), pages 17-24.
    9. José Luis Míguez & Jacobo Porteiro & Raquel Pérez-Orozco & Miguel Ángel Gómez, 2018. "Technology Evolution in Membrane-Based CCS," Energies, MDPI, vol. 11(11), pages 1-18, November.
    10. Zhang, Shihan & Shen, Yao & Wang, Lidong & Chen, Jianmeng & Lu, Yongqi, 2019. "Phase change solvents for post-combustion CO2 capture: Principle, advances, and challenges," Applied Energy, Elsevier, vol. 239(C), pages 876-897.
    11. Zhang, Zhonghua & Wang, Baodong & Sun, Qi & Zheng, Lingru, 2014. "A novel method for the preparation of CO2 sorption sorbents with high performance," Applied Energy, Elsevier, vol. 123(C), pages 179-184.
    12. Susmita Datta Peu & Arnob Das & Md. Sanowar Hossain & Md. Abdul Mannan Akanda & Md. Muzaffer Hosen Akanda & Mahbubur Rahman & Md. Naim Miah & Barun K. Das & Abu Reza Md. Towfiqul Islam & Mostafa M. Sa, 2023. "A Comprehensive Review on Recent Advancements in Absorption-Based Post Combustion Carbon Capture Technologies to Obtain a Sustainable Energy Sector with Clean Environment," Sustainability, MDPI, vol. 15(7), pages 1-33, March.

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