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CO2 capture with amine-loaded carbon nanotubes via a dual-column temperature/vacuum swing adsorption

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  • Su, Fengsheng
  • Lu, Chungsying
  • Chung, Ai-Ju
  • Liao, Chien-Hsiang

Abstract

A dual-column temperature/vacuum swing adsorption (TVSA) with 3-aminopropyltriethoxysilane-loaded carbon nanotubes (CNT(APTS)) was built to study cyclic CO2 capture from gas streams. The working CO2 capacities and the characteristics of CNT(APTS) were preserved through 100 TVSA cycles under dry or wet conditions, displaying the multi-cycle stability of CO2 capture with CNT(APTS). The cyclic working CO2 capacity of CNT(APTS) was notably enhanced in the presence of saturated water vapor in the gas stream at 25°C which gives relatively high desorbed CO2 concentrations (∼67%). These results suggest that a dual-column TVSA with solid CNT(APTS) has the possibility to be a promising CO2 capture technology, especially in the post-flue gas desulfurization in which saturated water vapor is present in the flue gas.

Suggested Citation

  • Su, Fengsheng & Lu, Chungsying & Chung, Ai-Ju & Liao, Chien-Hsiang, 2014. "CO2 capture with amine-loaded carbon nanotubes via a dual-column temperature/vacuum swing adsorption," Applied Energy, Elsevier, vol. 113(C), pages 706-712.
    • Handle: RePEc:eee:appene:v:113:y:2014:i:c:p:706-712
    DOI: 10.1016/j.apenergy.2013.08.001
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    1. Ben-Mansour, R. & Habib, M.A. & Bamidele, O.E. & Basha, M. & Qasem, N.A.A. & Peedikakkal, A. & Laoui, T. & Ali, M., 2016. "Carbon capture by physical adsorption: Materials, experimental investigations and numerical modeling and simulations – A review," Applied Energy, Elsevier, vol. 161(C), pages 225-255.
    2. Guo, Yafei & Zhao, Chuanwen & Li, Changhai & Lu, Shouxiang, 2014. "Application of PEI–K2CO3/AC for capturing CO2 from flue gas after combustion," Applied Energy, Elsevier, vol. 129(C), pages 17-24.
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    6. Sreenivasulu, B. & Gayatri, D.V. & Sreedhar, I. & Raghavan, K.V., 2015. "A journey into the process and engineering aspects of carbon capture technologies," Renewable and Sustainable Energy Reviews, Elsevier, vol. 41(C), pages 1324-1350.
    7. Chen, S.J. & Fu, Y. & Huang, Y.X. & Tao, Z.C. & Zhu, M., 2016. "Experimental investigation of CO2 separation by adsorption methods in natural gas purification," Applied Energy, Elsevier, vol. 179(C), pages 329-337.
    8. Pal, Animesh & Uddin, Kutub & Saha, Bidyut Baran & Thu, Kyaw & Kil, Hyun-Sig & Yoon, Seong-Ho & Miyawaki, Jin, 2020. "A benchmark for CO2 uptake onto newly synthesized biomass-derived activated carbons," Applied Energy, Elsevier, vol. 264(C).
    9. Qasem, Naef A.A. & Ben-Mansour, Rached, 2018. "Energy and productivity efficient vacuum pressure swing adsorption process to separate CO2 from CO2/N2 mixture using Mg-MOF-74: A CFD simulation," Applied Energy, Elsevier, vol. 209(C), pages 190-202.
    10. Kong, Yong & Shen, Xiaodong & Cui, Sheng & Fan, Maohong, 2015. "Development of monolithic adsorbent via polymeric sol–gel process for low-concentration CO2 capture," Applied Energy, Elsevier, vol. 147(C), pages 308-317.
    11. Chen, S.J. & Zhu, M. & Fu, Y. & Huang, Y.X. & Tao, Z.C. & Li, W.L., 2017. "Using 13X, LiX, and LiPdAgX zeolites for CO2 capture from post-combustion flue gas," Applied Energy, Elsevier, vol. 191(C), pages 87-98.
    12. Md Sumon Reza & Shammya Afroze & Kairat Kuterbekov & Asset Kabyshev & Kenzhebatyr Zh. Bekmyrza & Md Naimul Haque & Shafi Noor Islam & Md Aslam Hossain & Mahbub Hassan & Hridoy Roy & Md Shahinoor Islam, 2023. "Advanced Applications of Carbonaceous Materials in Sustainable Water Treatment, Energy Storage, and CO 2 Capture: A Comprehensive Review," Sustainability, MDPI, vol. 15(11), pages 1-56, May.
    13. Chen, S.J. & Tao, Z.C. & Fu, Y. & Zhu, M. & Li, W.L. & Li, X.D., 2017. "CO2 separation from offshore natural gas in quiescent and flowing states using 13X zeolite," Applied Energy, Elsevier, vol. 205(C), pages 1435-1446.
    14. Zhao, Ruikai & Liu, Longcheng & Zhao, Li & Deng, Shuai & Li, Shuangjun & Zhang, Yue, 2019. "A comprehensive performance evaluation of temperature swing adsorption for post-combustion carbon dioxide capture," Renewable and Sustainable Energy Reviews, Elsevier, vol. 114(C), pages 1-1.

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