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Effects of SO2 on CO2 capture using a hollow fiber membrane contactor

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  • Yang, Jie
  • Yu, Xinhai
  • Yan, Jinyue
  • Tu, Shan-Tung
  • Dahlquist, Erik

Abstract

Membrane gas absorption technology is a promising alternative to conventional technologies for the mitigation of acid gases. In this study, with a polypropylene (PP) hollow fiber membrane contactor as absorber and a packed column as stripper, the influence of SO2 on the CO2 capture from coal-fired power plant flue gas was investigated in an absorption–desorption experimental set-up using aqueous monoethanolamine (MEA) as the absorbent. The experimental results showed that the MEA loss per ton captured CO2 increased with the addition of SO2, resulting in sharp decreases in CO2 removal efficiency and mass transfer rate of CO2 after initial several days of operation. This tendency is mainly attributed to the promotional effect of SO2 on the degradation of MEA by the formation of sulfate. Thus, it is necessary to regenerate MEA using a reclaimer in this case. The respective SO2 concentrations at the outlets of absorber and stripper remained constant values of 24 and 120ppb throughout the operation although the CO2 removal efficiency decreased dramatically with time. This co-capture of CO2 and SO2 could play an important role in further desulfuration, thus alleviating the burden of desulfuration to some extent and benefiting the subsequent CO2 purification and storage. More progresses are greatly needed in high-efficiency and stable absorbents, high-efficiency reclaimer, and methods to reduce MEA loss by evaporation.

Suggested Citation

  • Yang, Jie & Yu, Xinhai & Yan, Jinyue & Tu, Shan-Tung & Dahlquist, Erik, 2013. "Effects of SO2 on CO2 capture using a hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 112(C), pages 755-764.
    • Handle: RePEc:eee:appene:v:112:y:2013:i:c:p:755-764
    DOI: 10.1016/j.apenergy.2012.11.052
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    References listed on IDEAS

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    1. Hu, Yukun & Yan, Jinyue & Li, Hailong, 2012. "Effects of flue gas recycle on oxy-coal power generation systems," Applied Energy, Elsevier, vol. 97(C), pages 255-263.
    2. Lv, Yuexia & Yu, Xinhai & Jia, Jingjing & Tu, Shan-Tung & Yan, Jinyue & Dahlquist, Erik, 2012. "Fabrication and characterization of superhydrophobic polypropylene hollow fiber membranes for carbon dioxide absorption," Applied Energy, Elsevier, vol. 90(1), pages 167-174.
    3. Lv, Yuexia & Yu, Xinhai & Tu, Shan-Tung & Yan, Jinyue & Dahlquist, Erik, 2012. "Experimental studies on simultaneous removal of CO2 and SO2 in a polypropylene hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 97(C), pages 283-288.
    4. Li, H. & Yan, J. & Yan, J. & Anheden, M., 2009. "Impurity impacts on the purification process in oxy-fuel combustion based CO2 capture and storage system," Applied Energy, Elsevier, vol. 86(2), pages 202-213, February.
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    2. Zhang, Xiaowen & Zhang, Xin & Liu, Helei & Li, Wensheng & Xiao, Min & Gao, Hongxia & Liang, Zhiwu, 2017. "Reduction of energy requirement of CO2 desorption from a rich CO2-loaded MEA solution by using solid acid catalysts," Applied Energy, Elsevier, vol. 202(C), pages 673-684.
    3. Zhang, Xiaowen & Huang, Yufei & Gao, Hongxia & Luo, Xiao & Liang, Zhiwu & Tontiwachwuthikul, Paitoon, 2019. "Zeolite catalyst-aided tri-solvent blend amine regeneration: An alternative pathway to reduce the energy consumption in amine-based CO2 capture process," Applied Energy, Elsevier, vol. 240(C), pages 827-841.
    4. Garlapalli, Ravinder K. & Spencer, Michael W. & Alam, Khairul & Trembly, Jason P., 2018. "Integration of heat recovery unit in coal fired power plants to reduce energy cost of carbon dioxide capture," Applied Energy, Elsevier, vol. 229(C), pages 900-909.
    5. Sreedhar, I. & Vaidhiswaran, R. & Kamani, Bansi. M. & Venugopal, A., 2017. "Process and engineering trends in membrane based carbon capture," Renewable and Sustainable Energy Reviews, Elsevier, vol. 68(P1), pages 659-684.
    6. Yang, Yan & Wen, Chuang & Wang, Shuli & Feng, Yuqing, 2014. "Theoretical and numerical analysis on pressure recovery of supersonic separators for natural gas dehydration," Applied Energy, Elsevier, vol. 132(C), pages 248-253.
    7. Lin, Yi-Feng & Chang, Jun-Min & Ye, Qian & Tung, Kuo-Lun, 2015. "Hydrophobic fluorocarbon-modified silica aerogel tubular membranes with excellent CO2 recovery ability in membrane contactors," Applied Energy, Elsevier, vol. 154(C), pages 21-25.
    8. Yang, Jie & Yu, Xinhai & An, Lin & Tu, Shan-Tung & Yan, Jinyue, 2017. "CO2 capture with the absorbent of a mixed ionic liquid and amine solution considering the effects of SO2 and O2," Applied Energy, Elsevier, vol. 194(C), pages 9-18.
    9. Hyun Sic Park & Dongwoan Kang & Jo Hong Kang & Kwanghwi Kim & Jaehyuk Kim & Hojun Song, 2021. "Selective Sulfur Dioxide Absorption from Simulated Flue Gas Using Various Aqueous Alkali Solutions in a Polypropylene Hollow Fiber Membrane Contactor: Removal Efficiency and Use of Sulfur Dioxide," IJERPH, MDPI, vol. 18(2), pages 1-15, January.
    10. Fang, Zhongqiu & Yu, Xiaochen & Tang, Weiqiang & Yu, Xinhai & Zhao, Shuangliang & Tu, Shan-Tung, 2017. "Denitration by oxidation-absorption with polypropylene hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 206(C), pages 858-868.
    11. Lin, Yi-Feng & Ko, Chia-Chieh & Chen, Chien-Hua & Tung, Kuo-Lun & Chang, Kai-Shiun & Chung, Tsair-Wang, 2014. "Sol–gel preparation of polymethylsilsesquioxane aerogel membranes for CO2 absorption fluxes in membrane contactors," Applied Energy, Elsevier, vol. 129(C), pages 25-31.

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