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Experimental studies on simultaneous removal of CO2 and SO2 in a polypropylene hollow fiber membrane contactor

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  • Lv, Yuexia
  • Yu, Xinhai
  • Tu, Shan-Tung
  • Yan, Jinyue
  • Dahlquist, Erik

Abstract

Membrane gas absorption technology is a promising alternative to conventional technologies for the mitigation of acid gases. In this study, simultaneous removal of SO2 and CO2 from coal-fired flue gas was carried out in a polypropylene hollow fiber membrane contactor using aqueous monoethanolamine as the absorbent. The influences of liquid and gas flow rates on the simultaneous absorption performance of CO2 and SO2 were investigated. The experimental results indicated that the membrane contactor could eliminate these two sour gases simultaneously and effectively. Absorption of SO2 and CO2 was enhanced by the increase in liquid flow rate and decrease in gas flow rate. It was observed that a small amount of SO2 in the flue gas had a slight influence on the absorption of CO2. In addition, the membrane contactor was operated continuously for two weeks to evaluate its duration performance. The results showed that the CO2 mass transfer rate was decreased significantly with the operating time due to partial wetting of membrane pores. After 14days of continuous operation, the CO2 mass transfer rate of the wetted membrane contactor was decreased by 41% but could be retrieved to 86% of the fresh one by increasing the gas phase pressure.

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  • Lv, Yuexia & Yu, Xinhai & Tu, Shan-Tung & Yan, Jinyue & Dahlquist, Erik, 2012. "Experimental studies on simultaneous removal of CO2 and SO2 in a polypropylene hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 97(C), pages 283-288.
    • Handle: RePEc:eee:appene:v:97:y:2012:i:c:p:283-288
    DOI: 10.1016/j.apenergy.2012.01.034
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    1. Lv, Yuexia & Yu, Xinhai & Jia, Jingjing & Tu, Shan-Tung & Yan, Jinyue & Dahlquist, Erik, 2012. "Fabrication and characterization of superhydrophobic polypropylene hollow fiber membranes for carbon dioxide absorption," Applied Energy, Elsevier, vol. 90(1), pages 167-174.
    2. Zhao, Guoying & Aziz, Baroz & Hedin, Niklas, 2010. "Carbon dioxide adsorption on mesoporous silica surfaces containing amine-like motifs," Applied Energy, Elsevier, vol. 87(9), pages 2907-2913, September.
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    2. Hyun Sic Park & Dongwoan Kang & Jo Hong Kang & Kwanghwi Kim & Jaehyuk Kim & Hojun Song, 2021. "Selective Sulfur Dioxide Absorption from Simulated Flue Gas Using Various Aqueous Alkali Solutions in a Polypropylene Hollow Fiber Membrane Contactor: Removal Efficiency and Use of Sulfur Dioxide," IJERPH, MDPI, vol. 18(2), pages 1-15, January.
    3. Qi, Run & Li, Zhaohao & Zhang, Hongyuan & Fu, Hongming & Zhang, Heng & Gao, Dan & Chen, Haiping, 2023. "CO2 capture performance of ceramic membrane with superhydrophobic modification based on deposited SiO2 particles," Energy, Elsevier, vol. 283(C).
    4. Fang, Zhongqiu & Yu, Xiaochen & Tang, Weiqiang & Yu, Xinhai & Zhao, Shuangliang & Tu, Shan-Tung, 2017. "Denitration by oxidation-absorption with polypropylene hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 206(C), pages 858-868.
    5. Ganapathy, Harish & Steinmayer, Sascha & Shooshtari, Amir & Dessiatoun, Serguei & Ohadi, Michael M. & Alshehhi, Mohamed, 2016. "Process intensification characteristics of a microreactor absorber for enhanced CO2 capture," Applied Energy, Elsevier, vol. 162(C), pages 416-427.
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    7. Ganapathy, H. & Shooshtari, A. & Dessiatoun, S. & Alshehhi, M. & Ohadi, M., 2014. "Fluid flow and mass transfer characteristics of enhanced CO2 capture in a minichannel reactor," Applied Energy, Elsevier, vol. 119(C), pages 43-56.
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