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Selective Sulfur Dioxide Absorption from Simulated Flue Gas Using Various Aqueous Alkali Solutions in a Polypropylene Hollow Fiber Membrane Contactor: Removal Efficiency and Use of Sulfur Dioxide

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  • Hyun Sic Park

    (Green Materials & Processes R&D Group, Korea Institute of Industrial Technology, 55 Jongga-ro, Jung-gu, Ulsan 44413, Korea
    These authors contributed equally to this work.)

  • Dongwoan Kang

    (Green Materials & Processes R&D Group, Korea Institute of Industrial Technology, 55 Jongga-ro, Jung-gu, Ulsan 44413, Korea
    Department of Civil and Environmental Engineering, Pusan National University, 2 Busandaehak-ro, 63beon-gil, Geumjeong-gu, Pusan 46241, Korea
    These authors contributed equally to this work.)

  • Jo Hong Kang

    (Green Materials & Processes R&D Group, Korea Institute of Industrial Technology, 55 Jongga-ro, Jung-gu, Ulsan 44413, Korea)

  • Kwanghwi Kim

    (Green Materials & Processes R&D Group, Korea Institute of Industrial Technology, 55 Jongga-ro, Jung-gu, Ulsan 44413, Korea)

  • Jaehyuk Kim

    (Department of Civil and Environmental Engineering, Pusan National University, 2 Busandaehak-ro, 63beon-gil, Geumjeong-gu, Pusan 46241, Korea)

  • Hojun Song

    (Green Materials & Processes R&D Group, Korea Institute of Industrial Technology, 55 Jongga-ro, Jung-gu, Ulsan 44413, Korea)

Abstract

Hollow fiber membrane contactors (HFMCs) provide a large specific surface area. Thus, their significantly reduced volume provides an advantage compared to the conventional gas–liquid contactor. In this study, the selective removal efficiency of flue gas, in which sulfur oxide (SO 2 ) and carbon dioxide (CO 2 ) coexist, was measured using a polypropylene (PP) HFMC with such advantages. To increase the selective removal efficiency of SO 2 , experiments were conducted using various alkaline absorbents. As a result, with 0.05 M ammonia solution, the removal efficiency of 95% or more was exhibited with continuous operation for 100 h or more. We confirmed that the absorbent saturated by the once-through mode was aqueous ammonium sulfate ((NH 4 ) 2 SO 4 ) solution and could be used as a fertilizer without additional processing.

Suggested Citation

  • Hyun Sic Park & Dongwoan Kang & Jo Hong Kang & Kwanghwi Kim & Jaehyuk Kim & Hojun Song, 2021. "Selective Sulfur Dioxide Absorption from Simulated Flue Gas Using Various Aqueous Alkali Solutions in a Polypropylene Hollow Fiber Membrane Contactor: Removal Efficiency and Use of Sulfur Dioxide," IJERPH, MDPI, vol. 18(2), pages 1-15, January.
    • Handle: RePEc:gam:jijerp:v:18:y:2021:i:2:p:597-:d:479016
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    References listed on IDEAS

    as
    1. Lv, Yuexia & Yu, Xinhai & Jia, Jingjing & Tu, Shan-Tung & Yan, Jinyue & Dahlquist, Erik, 2012. "Fabrication and characterization of superhydrophobic polypropylene hollow fiber membranes for carbon dioxide absorption," Applied Energy, Elsevier, vol. 90(1), pages 167-174.
    2. Yang, Jie & Yu, Xinhai & Yan, Jinyue & Tu, Shan-Tung & Dahlquist, Erik, 2013. "Effects of SO2 on CO2 capture using a hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 112(C), pages 755-764.
    3. Lv, Yuexia & Yu, Xinhai & Tu, Shan-Tung & Yan, Jinyue & Dahlquist, Erik, 2012. "Experimental studies on simultaneous removal of CO2 and SO2 in a polypropylene hollow fiber membrane contactor," Applied Energy, Elsevier, vol. 97(C), pages 283-288.
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