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High-efficiency two-dimensional Ruddlesden–Popper perovskite solar cells

Author

Listed:
  • Hsinhan Tsai

    (Los Alamos National Laboratory, Los Alamos
    Rice University)

  • Wanyi Nie

    (Los Alamos National Laboratory, Los Alamos)

  • Jean-Christophe Blancon

    (Los Alamos National Laboratory, Los Alamos)

  • Constantinos C. Stoumpos

    (Northwestern University
    Northwestern University
    Engineering and Argonne-Northwestern Solar Energy Research (ANSER) Center, Northwestern University)

  • Reza Asadpour

    (School of Electrical and Computer Engineering, Purdue University)

  • Boris Harutyunyan

    (Northwestern University
    Engineering and Argonne-Northwestern Solar Energy Research (ANSER) Center, Northwestern University)

  • Amanda J. Neukirch

    (Los Alamos National Laboratory, Los Alamos)

  • Rafael Verduzco

    (Rice University
    Rice University, Houston, Texas 77005, USA)

  • Jared J. Crochet

    (Los Alamos National Laboratory, Los Alamos)

  • Sergei Tretiak

    (Los Alamos National Laboratory, Los Alamos)

  • Laurent Pedesseau

    (Fonctions Optiques pour les Technologies de l’Information, FOTON UMR 6082, CNRS, INSA de Rennes)

  • Jacky Even

    (Fonctions Optiques pour les Technologies de l’Information, FOTON UMR 6082, CNRS, INSA de Rennes)

  • Muhammad A. Alam

    (School of Electrical and Computer Engineering, Purdue University)

  • Gautam Gupta

    (Los Alamos National Laboratory, Los Alamos)

  • Jun Lou

    (Rice University)

  • Pulickel M. Ajayan

    (Rice University)

  • Michael J. Bedzyk

    (Northwestern University
    Engineering and Argonne-Northwestern Solar Energy Research (ANSER) Center, Northwestern University)

  • Mercouri G. Kanatzidis

    (Northwestern University
    Northwestern University
    Engineering and Argonne-Northwestern Solar Energy Research (ANSER) Center, Northwestern University)

  • Aditya D. Mohite

    (Los Alamos National Laboratory, Los Alamos)

Abstract

Thin-film solar cells were fabricated using layered two-dimensional perovskites with near-single-crystalline out-of-plane alignment, which facilitates efficient charge transport leading to greatly improved power conversion efficiency with technologically relevant stability to light exposure, humidity and heat stress.

Suggested Citation

  • Hsinhan Tsai & Wanyi Nie & Jean-Christophe Blancon & Constantinos C. Stoumpos & Reza Asadpour & Boris Harutyunyan & Amanda J. Neukirch & Rafael Verduzco & Jared J. Crochet & Sergei Tretiak & Laurent P, 2016. "High-efficiency two-dimensional Ruddlesden–Popper perovskite solar cells," Nature, Nature, vol. 536(7616), pages 312-316, August.
    • Handle: RePEc:nat:nature:v:536:y:2016:i:7616:d:10.1038_nature18306
    DOI: 10.1038/nature18306
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    3. Dejian Yu & Fei Cao & Jinfeng Liao & Bingzhe Wang & Chenliang Su & Guichuan Xing, 2022. "Direct observation of photoinduced carrier blocking in mixed-dimensional 2D/3D perovskites and the origin," Nature Communications, Nature, vol. 13(1), pages 1-11, December.
    4. Priyadarshini, P. & Senapati, S. & Naik, R., 2023. "Lead-free organic inorganic hybrid halide perovskites: An emerging candidate for bifunctional applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 186(C).
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    6. Nian Li & Shambhavi Pratap & Volker Körstgens & Sundeep Vema & Lin Song & Suzhe Liang & Anton Davydok & Christina Krywka & Peter Müller-Buschbaum, 2022. "Mapping structure heterogeneities and visualizing moisture degradation of perovskite films with nano-focus WAXS," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    7. Xuan-Kun Li & Jian-Xu Ma & Xiang-Yu Li & Jun-Jie Hu & Chuan-Yang Ding & Feng-Kai Han & Xiao-Min Guo & Xi Tan & Xian-Min Jin, 2024. "High-efficiency reinforcement learning with hybrid architecture photonic integrated circuit," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    8. Weichuan Zhang & Ziyuan Liu & Lizhi Zhang & Hui Wang & Chuanxiu Jiang & Xianxin Wu & Chuanyun Li & Shengli Yue & Rongsheng Yang & Hong Zhang & Jianqi Zhang & Xinfeng Liu & Yuan Zhang & Huiqiong Zhou, 2024. "Ultrastable and efficient slight-interlayer-displacement 2D Dion-Jacobson perovskite solar cells," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    9. Yiyang Gong & Shuai Yue & Yin Liang & Wenna Du & Tieyuan Bian & Chuanxiu Jiang & Xiaotian Bao & Shuai Zhang & Mingzhu Long & Guofu Zhou & Jun Yin & Shibin Deng & Qing Zhang & Bo Wu & Xinfeng Liu, 2024. "Boosting exciton mobility approaching Mott-Ioffe-Regel limit in Ruddlesden−Popper perovskites by anchoring the organic cation," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    10. Xixiang Zhu & Liping Peng & Jinpeng Li & Haomiao Yu & Yulin Xie, 2021. "Formation of a Fast Charge Transfer Channel in Quasi-2D Perovskite Solar Cells through External Electric Field Modulation," Energies, MDPI, vol. 14(21), pages 1-10, November.
    11. Shunran Li & Xian Xu & Conrad A. Kocoj & Chenyu Zhou & Yanyan Li & Du Chen & Joseph A. Bennett & Sunhao Liu & Lina Quan & Suchismita Sarker & Mingzhao Liu & Diana Y. Qiu & Peijun Guo, 2024. "Large exchange-driven intrinsic circular dichroism of a chiral 2D hybrid perovskite," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    12. Dhruba B. Khadka & Yasuhiro Shirai & Masatoshi Yanagida & Hitoshi Ota & Andrey Lyalin & Tetsuya Taketsugu & Kenjiro Miyano, 2024. "Defect passivation in methylammonium/bromine free inverted perovskite solar cells using charge-modulated molecular bonding," Nature Communications, Nature, vol. 15(1), pages 1-16, December.
    13. Raman, Rohith Kumar & Gurusamy Thangavelu, Senthil A. & Venkataraj, Selvaraj & Krishnamoorthy, Ananthanarayanan, 2021. "Materials, methods and strategies for encapsulation of perovskite solar cells: From past to present," Renewable and Sustainable Energy Reviews, Elsevier, vol. 151(C).
    14. Liangliang Min & Haoxuan Sun & Linqi Guo & Meng Wang & Fengren Cao & Jun Zhong & Liang Li, 2024. "Frequency-selective perovskite photodetector for anti-interference optical communications," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    15. Xiaoming Zhao & Melissa L. Ball & Arvin Kakekhani & Tianran Liu & Andrew M. Rappe & Yueh-Lin Loo, 2022. "A charge transfer framework that describes supramolecular interactions governing structure and properties of 2D perovskites," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    16. Jongchul Lim & Manuel Kober-Czerny & Yen-Hung Lin & James M. Ball & Nobuya Sakai & Elisabeth A. Duijnstee & Min Ji Hong & John G. Labram & Bernard Wenger & Henry J. Snaith, 2022. "Long-range charge carrier mobility in metal halide perovskite thin-films and single crystals via transient photo-conductivity," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    17. Cheng-Chieh Lin & Shing-Jong Huang & Pei-Hao Wu & Tzu-Pei Chen & Chih-Ying Huang & Ying-Chiao Wang & Po-Tuan Chen & Denitsa Radeva & Ognyan Petrov & Vladimir M. Gelev & Raman Sankar & Chia-Chun Chen &, 2022. "Direct investigation of the reorientational dynamics of A-site cations in 2D organic-inorganic hybrid perovskite by solid-state NMR," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
    18. Chee, A. Kuan-Way, 2023. "On current technology for light absorber materials used in highly efficient industrial solar cells," Renewable and Sustainable Energy Reviews, Elsevier, vol. 173(C).
    19. Zihan Qu & Yang Zhao & Fei Ma & Le Mei & Xian-Kai Chen & Haitao Zhou & Xinbo Chu & Yingguo Yang & Qi Jiang & Xingwang Zhang & Jingbi You, 2024. "Enhanced charge carrier transport and defects mitigation of passivation layer for efficient perovskite solar cells," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    20. Xiang, Huimin & Liu, Pengyun & Ran, Ran & Wang, Wei & Zhou, Wei & Shao, Zongping, 2022. "Two-dimensional Dion-Jacobson halide perovskites as new-generation light absorbers for perovskite solar cells," Renewable and Sustainable Energy Reviews, Elsevier, vol. 166(C).

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