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Ultrastable and efficient slight-interlayer-displacement 2D Dion-Jacobson perovskite solar cells

Author

Listed:
  • Weichuan Zhang

    (National Center for Nanoscience and Technology
    University of South China
    University of Chinese Academy of Sciences)

  • Ziyuan Liu

    (National Center for Nanoscience and Technology, Chinese Academy of Sciences)

  • Lizhi Zhang

    (National Center for Nanoscience and Technology, Chinese Academy of Sciences)

  • Hui Wang

    (National Center for Nanoscience and Technology, Chinese Academy of Sciences)

  • Chuanxiu Jiang

    (University of Chinese Academy of Sciences
    National Center for Nanoscience and Technology)

  • Xianxin Wu

    (University of Chinese Academy of Sciences
    National Center for Nanoscience and Technology)

  • Chuanyun Li

    (National Center for Nanoscience and Technology
    Beijing Technology And Business University)

  • Shengli Yue

    (Beihang University)

  • Rongsheng Yang

    (National Center for Nanoscience and Technology)

  • Hong Zhang

    (National Center for Nanoscience and Technology)

  • Jianqi Zhang

    (National Center for Nanoscience and Technology)

  • Xinfeng Liu

    (University of Chinese Academy of Sciences
    National Center for Nanoscience and Technology)

  • Yuan Zhang

    (Beihang University)

  • Huiqiong Zhou

    (National Center for Nanoscience and Technology
    University of Chinese Academy of Sciences)

Abstract

Stability has been a long-standing concern for solution-processed perovskite photovoltaics and their practical applications. However, stable perovskite materials for photovoltaic remain insufficient to date. Here we demonstrate a series of ultrastable Dion−Jacobson (DJ) perovskites (1,4-cyclohexanedimethanammonium)(methylammonium)n−1PbnI3n+1 (n ≥ 1) for photovoltaic applications. The scalable technology by blade-coated solar cells for the designed DJ perovskites (nominal n = 5) achieves a maximum stabilized power conversion efficiency (PCE) of 19.11% under an environmental atmosphere. Un-encapsulated cells by blade-coated technology retain 92% of their initial efficiencies for over 4000 hours under ~90% relative humidity (RH) aging conditions. More importantly, these cells also exhibit remarkable thermal (85 °C) and operational stability, which shows negligible efficiency loss after exceeding 5000-hour heat treatment or after operation at maximum power point (MPP) exceeding 6000 hours at 45 °C under a 100 mW cm−2 continuous light illumination.

Suggested Citation

  • Weichuan Zhang & Ziyuan Liu & Lizhi Zhang & Hui Wang & Chuanxiu Jiang & Xianxin Wu & Chuanyun Li & Shengli Yue & Rongsheng Yang & Hong Zhang & Jianqi Zhang & Xinfeng Liu & Yuan Zhang & Huiqiong Zhou, 2024. "Ultrastable and efficient slight-interlayer-displacement 2D Dion-Jacobson perovskite solar cells," Nature Communications, Nature, vol. 15(1), pages 1-10, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-50018-4
    DOI: 10.1038/s41467-024-50018-4
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    References listed on IDEAS

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