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Anomalous magnetoresistance by breaking ice rule in Bi2Ir2O7/Dy2Ti2O7 heterostructure

Author

Listed:
  • Han Zhang

    (University of Tennessee)

  • Chengkun Xing

    (University of Tennessee)

  • Kyle Noordhoek

    (University of Tennessee)

  • Zhaoyu Liu

    (University of Washington)

  • Tianhao Zhao

    (Georgia Institute of Technology)

  • Lukas Horák

    (Charles University)

  • Qing Huang

    (University of Tennessee)

  • Lin Hao

    (University of Tennessee)

  • Junyi Yang

    (University of Tennessee)

  • Shashi Pandey

    (University of Tennessee)

  • Elbio Dagotto

    (University of Tennessee
    Oak Ridge National Laboratory)

  • Zhigang Jiang

    (Georgia Institute of Technology)

  • Jiun-Haw Chu

    (University of Washington)

  • Yan Xin

    (Florida State University)

  • Eun Sang Choi

    (Florida State University)

  • Haidong Zhou

    (University of Tennessee)

  • Jian Liu

    (University of Tennessee)

Abstract

While geometrically frustrated quantum magnets host rich exotic spin states with potentials for revolutionary quantum technologies, most of them are necessarily good insulators which are difficult to be integrated with modern electrical circuit. The grand challenge is to electrically detect the emergent fluctuations and excitations by introducing charge carriers that interact with the localized spins without destroying their collective spin states. Here, we show that, by designing a Bi2Ir2O7/Dy2Ti2O7 heterostructure, the breaking of the spin-ice rule in insulating Dy2Ti2O7 leads to a charge response in the conducting Bi2Ir2O7 measured as anomalous magnetoresistance during the field-induced Kagome ice-to-saturated ice transition. The magnetoresistive anomaly also captures the characteristic angular and temperature dependence of this ice-rule-breaking transition, which has been understood as magnetic monopole condensation. These results demonstrate a novel heteroepitaxial approach for electronically probing the transition between exotic insulating spin states, laying out a blueprint for the metallization of frustrated quantum magnets.

Suggested Citation

  • Han Zhang & Chengkun Xing & Kyle Noordhoek & Zhaoyu Liu & Tianhao Zhao & Lukas Horák & Qing Huang & Lin Hao & Junyi Yang & Shashi Pandey & Elbio Dagotto & Zhigang Jiang & Jiun-Haw Chu & Yan Xin & Eun , 2023. "Anomalous magnetoresistance by breaking ice rule in Bi2Ir2O7/Dy2Ti2O7 heterostructure," Nature Communications, Nature, vol. 14(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-36886-2
    DOI: 10.1038/s41467-023-36886-2
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    References listed on IDEAS

    as
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