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Controlling Floquet states on ultrashort time scales

Author

Listed:
  • Matteo Lucchini

    (Politecnico di Milano
    IFN-CNR)

  • Fabio Medeghini

    (Politecnico di Milano)

  • Yingxuan Wu

    (Politecnico di Milano
    IFN-CNR)

  • Federico Vismarra

    (Politecnico di Milano
    IFN-CNR)

  • Rocío Borrego-Varillas

    (IFN-CNR)

  • Aurora Crego

    (IFN-CNR)

  • Fabio Frassetto

    (IFN-CNR)

  • Luca Poletto

    (IFN-CNR)

  • Shunsuke A. Sato

    (University of Tsukuba
    Max Planck Institute for the Structure and Dynamics of Matter)

  • Hannes Hübener

    (Max Planck Institute for the Structure and Dynamics of Matter)

  • Umberto Giovannini

    (Max Planck Institute for the Structure and Dynamics of Matter
    Università degli Studi di Palermo, Dipartimento di Fisica e Chimica-Emilio Segrè)

  • Ángel Rubio

    (Max Planck Institute for the Structure and Dynamics of Matter
    The Flatiron Institute)

  • Mauro Nisoli

    (Politecnico di Milano
    IFN-CNR)

Abstract

The advent of ultrafast laser science offers the unique opportunity to combine Floquet engineering with extreme time resolution, further pushing the optical control of matter into the petahertz domain. However, what is the shortest driving pulse for which Floquet states can be realised remains an unsolved matter, thus limiting the application of Floquet theory to pulses composed by many optical cycles. Here we ionized Ne atoms with few-femtosecond pulses of selected time duration and show that a Floquet state can be observed already with a driving field that lasts for only 10 cycles. For shorter pulses, down to 2 cycles, the finite lifetime of the driven state can still be explained using an analytical model based on Floquet theory. By demonstrating that the amplitude and number of Floquet-like sidebands in the photoelectron spectrum can be controlled not only with the driving laser pulse intensity and frequency, but also by its duration, our results add a new lever to the toolbox of Floquet engineering.

Suggested Citation

  • Matteo Lucchini & Fabio Medeghini & Yingxuan Wu & Federico Vismarra & Rocío Borrego-Varillas & Aurora Crego & Fabio Frassetto & Luca Poletto & Shunsuke A. Sato & Hannes Hübener & Umberto Giovannini & , 2022. "Controlling Floquet states on ultrashort time scales," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-34973-4
    DOI: 10.1038/s41467-022-34973-4
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    References listed on IDEAS

    as
    1. Matteo Lucchini & Shunsuke A. Sato & Giacinto D. Lucarelli & Bruno Moio & Giacomo Inzani & Rocío Borrego-Varillas & Fabio Frassetto & Luca Poletto & Hannes Hübener & Umberto Giovannini & Angel Rubio &, 2021. "Unravelling the intertwined atomic and bulk nature of localised excitons by attosecond spectroscopy," Nature Communications, Nature, vol. 12(1), pages 1-7, December.
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