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Highly nonlinear dipolar exciton-polaritons in bilayer MoS2

Author

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  • Biswajit Datta

    (City College of New York)

  • Mandeep Khatoniar

    (City College of New York
    Graduate Center of the City University of New York (CUNY))

  • Prathmesh Deshmukh

    (City College of New York
    Graduate Center of the City University of New York (CUNY))

  • Félix Thouin

    (École Polytechnique de Montréal)

  • Rezlind Bushati

    (City College of New York
    Graduate Center of the City University of New York (CUNY))

  • Simone Liberato

    (School of Physics and Astronomy, University of Southampton)

  • Stephane Kena Cohen

    (École Polytechnique de Montréal)

  • Vinod M. Menon

    (City College of New York
    Graduate Center of the City University of New York (CUNY))

Abstract

Realizing nonlinear optical response in the low photon density limit in solid-state systems has been a long-standing challenge. Semiconductor microcavities in the strong coupling regime hosting exciton-polaritons have emerged as attractive candidates in this context. However, the weak interaction between these quasiparticles has been a hurdle in this quest. Dipolar excitons provide an attractive strategy to overcome this limitation but are often hindered by their weak oscillator strength. The interlayer dipolar excitons in naturally occurring homobilayer MoS2 alleviates this issue owing to their formation via hybridization of interlayer charge transfer exciton with intralayer B exciton. Here we demonstrate the formation of dipolar exciton polaritons in bilayer MoS2 resulting in unprecedented nonlinear interaction strengths. A ten-fold increase in nonlinearity is observed for the interlayer dipolar excitons compared to the conventional A excitons. These highly nonlinear dipolar polaritons will likely be a frontrunner in the quest for solid-state quantum nonlinear devices.

Suggested Citation

  • Biswajit Datta & Mandeep Khatoniar & Prathmesh Deshmukh & Félix Thouin & Rezlind Bushati & Simone Liberato & Stephane Kena Cohen & Vinod M. Menon, 2022. "Highly nonlinear dipolar exciton-polaritons in bilayer MoS2," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-33940-3
    DOI: 10.1038/s41467-022-33940-3
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    2. Yesenia A. García Jomaso & Brenda Vargas & David Ley Domínguez & Román J. Armenta-Rico & Huziel E. Sauceda & César L. Ordoñez-Romero & Hugo A. Lara-García & Arturo Camacho-Guardian & Giuseppe Pirrucci, 2024. "Intercavity polariton slows down dynamics in strongly coupled cavities," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    3. Ke Wei & Qirui Liu & Yuxiang Tang & Yingqian Ye & Zhongjie Xu & Tian Jiang, 2023. "Charged biexciton polaritons sustaining strong nonlinearity in 2D semiconductor-based nanocavities," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    4. Charalambos Louca & Armando Genco & Salvatore Chiavazzo & Thomas P. Lyons & Sam Randerson & Chiara Trovatello & Peter Claronino & Rahul Jayaprakash & Xuerong Hu & James Howarth & Kenji Watanabe & Taka, 2023. "Interspecies exciton interactions lead to enhanced nonlinearity of dipolar excitons and polaritons in MoS2 homobilayers," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    5. Shun Feng & Aidan J. Campbell & Mauro Brotons-Gisbert & Daniel Andres-Penares & Hyeonjun Baek & Takashi Taniguchi & Kenji Watanabe & Bernhard Urbaszek & Iann C. Gerber & Brian D. Gerardot, 2024. "Highly tunable ground and excited state excitonic dipoles in multilayer 2H-MoSe2," Nature Communications, Nature, vol. 15(1), pages 1-10, December.

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