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Charged biexciton polaritons sustaining strong nonlinearity in 2D semiconductor-based nanocavities

Author

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  • Ke Wei

    (National University of Defense Technology)

  • Qirui Liu

    (National University of Defense Technology)

  • Yuxiang Tang

    (National University of Defense Technology)

  • Yingqian Ye

    (National University of Defense Technology)

  • Zhongjie Xu

    (National University of Defense Technology)

  • Tian Jiang

    (National University of Defense Technology)

Abstract

Controlling the interaction between light and matter at micro- and nano-scale can provide new opportunities for modern optics and optoelectronics. An archetypical example is polariton, a half-light-half-matter quasi particle inheriting simultaneously the robust coherence of light and the strong interaction of matter, which plays an important role in many exotic phenomena. Here, we open up a new kind of cooperative coupling between plasmon and different excitonic complexes in WS2-silver nanocavities, namely plasmon-exciton-trion-charged biexciton four coupling states. Thanks to the large Bohr radius of up to 5 nm, the charged biexciton polariton exhibits strong saturation nonlinearity, ~30 times higher than the neutral exciton polariton. Transient absorption dynamics further reveal the ultrafast many-body interaction nature, with a timescale of

Suggested Citation

  • Ke Wei & Qirui Liu & Yuxiang Tang & Yingqian Ye & Zhongjie Xu & Tian Jiang, 2023. "Charged biexciton polaritons sustaining strong nonlinearity in 2D semiconductor-based nanocavities," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    • Handle: RePEc:nat:natcom:v:14:y:2023:i:1:d:10.1038_s41467-023-41079-y
    DOI: 10.1038/s41467-023-41079-y
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