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Durable radiative cooling against environmental aging

Author

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  • Jianing Song

    (University of Electronic Science and Technology of China)

  • Wenluan Zhang

    (University of Electronic Science and Technology of China
    University of Electronic Science and Technology of China)

  • Zhengnan Sun

    (University of Electronic Science and Technology of China)

  • Mengyao Pan

    (University of Electronic Science and Technology of China)

  • Feng Tian

    (Shanghai Synchrotron Radiation Facility, Zhangjiang Lab, Shanghai Advanced Research Institute, Chinese Academy of Science)

  • Xiuhong Li

    (Shanghai Synchrotron Radiation Facility, Zhangjiang Lab, Shanghai Advanced Research Institute, Chinese Academy of Science)

  • Ming Ye

    (Material Physics and Analytics, BASF Advanced Chemicals Co., Ltd. 333 Jiang Xin Sha Road, Pudong)

  • Xu Deng

    (University of Electronic Science and Technology of China)

Abstract

To fight against global warming, subambient daytime radiative cooling technology provides a promising path to meet sustainable development goals. To achieve subambient daytime radiative cooling, the reflection of most sunlight is the essential prerequisite. However, the desired high solar reflectance is easily dampened by environmental aging, mainly natural soiling and ultraviolet irradiation from sunlight causing yellowish color for most polymers, making the cooling ineffective. We demonstrate a simple strategy to use titanium dioxide nanoparticles, with ultraviolet resistance, forming hierarchical porous morphology via evaporation-driven assembly, which guarantees a balanced anti-soiling and high solar reflectance, rendering anti-aging cooling paint based coatings. We challenge the cooling coatings in an accelerated weathering test against simulated 3 years of natural soiling and simulated 1 year of natural sunshine, and find that the solar reflectance only declined by 0.4% and 0.5% compared with the un-aged ones. We further show over 6 months of aging under real-world conditions with barely no degradation to the cooling performance. Our anti-aging cooling paint is scalable and can be spray coated on desired outdoor architecture and container, presenting durable radiative cooling, promising for real-world applications.

Suggested Citation

  • Jianing Song & Wenluan Zhang & Zhengnan Sun & Mengyao Pan & Feng Tian & Xiuhong Li & Ming Ye & Xu Deng, 2022. "Durable radiative cooling against environmental aging," Nature Communications, Nature, vol. 13(1), pages 1-12, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-32409-7
    DOI: 10.1038/s41467-022-32409-7
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    1. Matteo Alberghini & Seongdon Hong & L. Marcelo Lozano & Volodymyr Korolovych & Yi Huang & Francesco Signorato & S. Hadi Zandavi & Corey Fucetola & Ihsan Uluturk & Michael Y. Tolstorukov & Gang Chen & , 2021. "Sustainable polyethylene fabrics with engineered moisture transport for passive cooling," Nature Sustainability, Nature, vol. 4(8), pages 715-724, August.
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    Cited by:

    1. Sai Liu & Yang Li & Ying Wang & Yuwei Du & Kin Man Yu & Hin-Lap Yip & Alex K. Y. Jen & Baoling Huang & Chi Yan Tso, 2024. "Mask-inspired moisture-transmitting and durable thermochromic perovskite smart windows," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    2. Chen, Xing-ni & Xu, Bin & Fei, Yue & Pei, Gang, 2024. "Combination optimization, importance order of parameters and aging consequence prediction for thermal insulation coating with radiation characteristics," Energy, Elsevier, vol. 290(C).
    3. Dongpyo Hong & Yong Joon Lee & Ok Sung Jeon & In-Sung Lee & Se Hun Lee & Jae Yeon Won & Young Pyo Jeon & Yunju La & Seonmyeong Kim & Gun-Sik Park & Young Joon Yoo & Sang Yoon Park, 2024. "Humidity-tolerant porous polymer coating for passive daytime radiative cooling," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    4. Dong, Yan & Zhang, Xinping & Chen, Lingling & Meng, Weifeng & Wang, Cunhai & Cheng, Ziming & Liang, Huaxu & Wang, Fuqiang, 2023. "Progress in passive daytime radiative cooling: A review from optical mechanism, performance test, and application," Renewable and Sustainable Energy Reviews, Elsevier, vol. 188(C).
    5. Xueke Wu & Jinlei Li & Fei Xie & Xun-En Wu & Siming Zhao & Qinyuan Jiang & Shiliang Zhang & Baoshun Wang & Yunrui Li & Di Gao & Run Li & Fei Wang & Ya Huang & Yanlong Zhao & Yingying Zhang & Wei Li & , 2024. "A dual-selective thermal emitter with enhanced subambient radiative cooling performance," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    6. Lianhu Xiong & Yun Wei & Chuanliang Chen & Xin Chen & Qiang Fu & Hua Deng, 2023. "Thin lamellar films with enhanced mechanical properties for durable radiative cooling," Nature Communications, Nature, vol. 14(1), pages 1-9, December.

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