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Determining the interlayer shearing in twisted bilayer MoS2 by nanoindentation

Author

Listed:
  • Yufei Sun

    (Tsinghua University)

  • Yujia Wang

    (Tsinghua University)

  • Enze Wang

    (Tsinghua University)

  • Bolun Wang

    (Tsinghua University)

  • Hengyi Zhao

    (Tsinghua University)

  • Yongpan Zeng

    (Tsinghua University)

  • Qinghua Zhang

    (Institute of Physics, Chinese Academy of Sciences)

  • Yonghuang Wu

    (Tsinghua University)

  • Lin Gu

    (Institute of Physics, Chinese Academy of Sciences)

  • Xiaoyan Li

    (Tsinghua University)

  • Kai Liu

    (Tsinghua University)

Abstract

The rise of twistronics has increased the attention of the community to the twist-angle-dependent properties of two-dimensional van der Waals integrated architectures. Clarification of the relationship between twist angles and interlayer mechanical interactions is important in benefiting the design of two-dimensional twisted structures. However, current mechanical methods have critical limitations in quantitatively probing the twist-angle dependence of two-dimensional interlayer interactions in monolayer limits. Here we report a nanoindentation-based technique and a shearing-boundary model to determine the interlayer mechanical interactions of twisted bilayer MoS2. Both in-plane elastic moduli and interlayer shear stress are found to be independent of the twist angle, which is attributed to the long-range interaction of intermolecular van der Waals forces that homogenously spread over the interfaces of MoS2. Our work provides a universal approach to determining the interlayer shear stress and deepens the understanding of twist-angle-dependent behaviours of two-dimensional layered materials.

Suggested Citation

  • Yufei Sun & Yujia Wang & Enze Wang & Bolun Wang & Hengyi Zhao & Yongpan Zeng & Qinghua Zhang & Yonghuang Wu & Lin Gu & Xiaoyan Li & Kai Liu, 2022. "Determining the interlayer shearing in twisted bilayer MoS2 by nanoindentation," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
    • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-31685-7
    DOI: 10.1038/s41467-022-31685-7
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