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Magic in twisted transition metal dichalcogenide bilayers

Author

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  • Trithep Devakul

    (Massachusetts Institute of Technology)

  • Valentin Crépel

    (Massachusetts Institute of Technology)

  • Yang Zhang

    (Massachusetts Institute of Technology)

  • Liang Fu

    (Massachusetts Institute of Technology)

Abstract

The long-wavelength moiré superlattices in twisted 2D structures have emerged as a highly tunable platform for strongly correlated electron physics. We study the moiré bands in twisted transition metal dichalcogenide homobilayers, focusing on WSe2, at small twist angles using a combination of first principles density functional theory, continuum modeling, and Hartree-Fock approximation. We reveal the rich physics at small twist angles θ

Suggested Citation

  • Trithep Devakul & Valentin Crépel & Yang Zhang & Liang Fu, 2021. "Magic in twisted transition metal dichalcogenide bilayers," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
  • Handle: RePEc:nat:natcom:v:12:y:2021:i:1:d:10.1038_s41467-021-27042-9
    DOI: 10.1038/s41467-021-27042-9
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    References listed on IDEAS

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    1. Yuan Cao & Valla Fatemi & Shiang Fang & Kenji Watanabe & Takashi Taniguchi & Efthimios Kaxiras & Pablo Jarillo-Herrero, 2018. "Unconventional superconductivity in magic-angle graphene superlattices," Nature, Nature, vol. 556(7699), pages 43-50, April.
    2. Yang Xu & Song Liu & Daniel A. Rhodes & Kenji Watanabe & Takashi Taniguchi & James Hone & Veit Elser & Kin Fai Mak & Jie Shan, 2020. "Correlated insulating states at fractional fillings of moiré superlattices," Nature, Nature, vol. 587(7833), pages 214-218, November.
    3. Zhiren Zheng & Qiong Ma & Zhen Bi & Sergio Barrera & Ming-Hao Liu & Nannan Mao & Yang Zhang & Natasha Kiper & Kenji Watanabe & Takashi Taniguchi & Jing Kong & William A. Tisdale & Ray Ashoori & Nuh Ge, 2020. "Unconventional ferroelectricity in moiré heterostructures," Nature, Nature, vol. 588(7836), pages 71-76, December.
    4. Zhen Bi & Liang Fu, 2021. "Excitonic density wave and spin-valley superfluid in bilayer transition metal dichalcogenide," Nature Communications, Nature, vol. 12(1), pages 1-10, December.
    5. Yuan Cao & Daniel Rodan-Legrain & Oriol Rubies-Bigorda & Jeong Min Park & Kenji Watanabe & Takashi Taniguchi & Pablo Jarillo-Herrero, 2020. "Tunable correlated states and spin-polarized phases in twisted bilayer–bilayer graphene," Nature, Nature, vol. 583(7815), pages 215-220, July.
    6. Emma C. Regan & Danqing Wang & Chenhao Jin & M. Iqbal Bakti Utama & Beini Gao & Xin Wei & Sihan Zhao & Wenyu Zhao & Zuocheng Zhang & Kentaro Yumigeta & Mark Blei & Johan D. Carlström & Kenji Watanabe , 2020. "Mott and generalized Wigner crystal states in WSe2/WS2 moiré superlattices," Nature, Nature, vol. 579(7799), pages 359-363, March.
    7. Xiaobo Lu & Petr Stepanov & Wei Yang & Ming Xie & Mohammed Ali Aamir & Ipsita Das & Carles Urgell & Kenji Watanabe & Takashi Taniguchi & Guangyu Zhang & Adrian Bachtold & Allan H. MacDonald & Dmitri K, 2019. "Superconductors, orbital magnets and correlated states in magic-angle bilayer graphene," Nature, Nature, vol. 574(7780), pages 653-657, October.
    8. Yuan Cao & Daniel Rodan-Legrain & Oriol Rubies-Bigorda & Jeong Min Park & Kenji Watanabe & Takashi Taniguchi & Pablo Jarillo-Herrero, 2020. "Author Correction: Tunable correlated states and spin-polarized phases in twisted bilayer–bilayer graphene," Nature, Nature, vol. 583(7816), pages 27-27, July.
    9. Yanhao Tang & Lizhong Li & Tingxin Li & Yang Xu & Song Liu & Katayun Barmak & Kenji Watanabe & Takashi Taniguchi & Allan H. MacDonald & Jie Shan & Kin Fai Mak, 2020. "Simulation of Hubbard model physics in WSe2/WS2 moiré superlattices," Nature, Nature, vol. 579(7799), pages 353-358, March.
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    1. Manzhang Xu & Hongjia Ji & Lu Zheng & Weiwei Li & Jing Wang & Hanxin Wang & Lei Luo & Qianbo Lu & Xuetao Gan & Zheng Liu & Xuewen Wang & Wei Huang, 2024. "Reconfiguring nucleation for CVD growth of twisted bilayer MoS2 with a wide range of twist angles," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    2. Lei Chen & Fang Xie & Shouvik Sur & Haoyu Hu & Silke Paschen & Jennifer Cano & Qimiao Si, 2024. "Emergent flat band and topological Kondo semimetal driven by orbital-selective correlations," Nature Communications, Nature, vol. 15(1), pages 1-7, December.
    3. Xiao-Wei Zhang & Chong Wang & Xiaoyu Liu & Yueyao Fan & Ting Cao & Di Xiao, 2024. "Polarization-driven band topology evolution in twisted MoTe2 and WSe2," Nature Communications, Nature, vol. 15(1), pages 1-8, December.

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