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Scanning gradiometry with a single spin quantum magnetometer

Author

Listed:
  • W. S. Huxter

    (ETH Zurich)

  • M. L. Palm

    (ETH Zurich)

  • M. L. Davis

    (ETH Zurich)

  • P. Welter

    (ETH Zurich)

  • C.-H. Lambert

    (ETH Zurich)

  • M. Trassin

    (ETH Zurich)

  • C. L. Degen

    (ETH Zurich
    ETH Zurich)

Abstract

Quantum sensors based on spin defects in diamond have recently enabled detailed imaging of nanoscale magnetic patterns, such as chiral spin textures, two-dimensional ferromagnets, or superconducting vortices, based on a measurement of the static magnetic stray field. Here, we demonstrate a gradiometry technique that significantly enhances the measurement sensitivity of such static fields, leading to new opportunities in the imaging of weakly magnetic systems. Our method relies on the mechanical oscillation of a single nitrogen-vacancy center at the tip of a scanning diamond probe, which up-converts the local spatial gradients into ac magnetic fields enabling the use of sensitive ac quantum protocols. We show that gradiometry provides important advantages over static field imaging: (i) an order-of-magnitude better sensitivity, (ii) a more localized and sharper image, and (iii) a strong suppression of field drifts. We demonstrate the capabilities of gradiometry by imaging the nanotesla fields appearing above topographic defects and atomic steps in an antiferromagnet, direct currents in a graphene device, and para- and diamagnetic metals.

Suggested Citation

  • W. S. Huxter & M. L. Palm & M. L. Davis & P. Welter & C.-H. Lambert & M. Trassin & C. L. Degen, 2022. "Scanning gradiometry with a single spin quantum magnetometer," Nature Communications, Nature, vol. 13(1), pages 1-9, December.
  • Handle: RePEc:nat:natcom:v:13:y:2022:i:1:d:10.1038_s41467-022-31454-6
    DOI: 10.1038/s41467-022-31454-6
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    1. I. Gross & W. Akhtar & V. Garcia & L. J. Martínez & S. Chouaieb & K. Garcia & C. Carrétéro & A. Barthélémy & P. Appel & P. Maletinsky & J.-V. Kim & J. Y. Chauleau & N. Jaouen & M. Viret & M. Bibes & S, 2017. "Real-space imaging of non-collinear antiferromagnetic order with a single-spin magnetometer," Nature, Nature, vol. 549(7671), pages 252-256, September.
    2. M. Fiebig & Th. Lottermoser & D. Fröhlich & A. V. Goltsev & R. V. Pisarev, 2002. "Observation of coupled magnetic and electric domains," Nature, Nature, vol. 419(6909), pages 818-820, October.
    3. Ke Bian & Wentian Zheng & Xianzhe Zeng & Xiakun Chen & Rainer Stöhr & Andrej Denisenko & Sen Yang & Jörg Wrachtrup & Ying Jiang, 2021. "Nanoscale electric-field imaging based on a quantum sensor and its charge-state control under ambient condition," Nature Communications, Nature, vol. 12(1), pages 1-9, December.
    4. Y. Dovzhenko & F. Casola & S. Schlotter & T. X. Zhou & F. Büttner & R. L. Walsworth & G. S. D. Beach & A. Yacoby, 2018. "Magnetostatic twists in room-temperature skyrmions explored by nitrogen-vacancy center spin texture reconstruction," Nature Communications, Nature, vol. 9(1), pages 1-7, December.
    5. X. Z. Yu & Y. Onose & N. Kanazawa & J. H. Park & J. H. Han & Y. Matsui & N. Nagaosa & Y. Tokura, 2010. "Real-space observation of a two-dimensional skyrmion crystal," Nature, Nature, vol. 465(7300), pages 901-904, June.
    6. D. Rugar & R. Budakian & H. J. Mamin & B. W. Chui, 2004. "Single spin detection by magnetic resonance force microscopy," Nature, Nature, vol. 430(6997), pages 329-332, July.
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