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Lifetime Prediction of a Polymer Electrolyte Membrane Fuel Cell under Automotive Load Cycling Using a Physically-Based Catalyst Degradation Model

Author

Listed:
  • Manik Mayur

    (Institute of Energy Systems Technology (INES), Offenburg University of Applied Sciences, Badstrasse 24, 77652 Offenburg, Germany)

  • Mathias Gerard

    (CEA LITEN, University of Grenoble Alpes, F-38054 Grenoble, France)

  • Pascal Schott

    (CEA LITEN, University of Grenoble Alpes, F-38054 Grenoble, France)

  • Wolfgang G. Bessler

    (Institute of Energy Systems Technology (INES), Offenburg University of Applied Sciences, Badstrasse 24, 77652 Offenburg, Germany)

Abstract

One of the bottlenecks hindering the usage of polymer electrolyte membrane fuel cell technology in automotive applications is the highly load-sensitive degradation of the cell components. The cell failure cases reported in the literature show localized cell component degradation, mainly caused by flow-field dependent non-uniform distribution of reactants. The existing methodologies for diagnostics of localized cell failure are either invasive or require sophisticated and expensive apparatus. In this study, with the help of a multiscale simulation framework, a single polymer electrolyte membrane fuel cell (PEMFC) model is exposed to a standardized drive cycle provided by a system model of a fuel cell car. A 2D multiphysics model of the PEMFC is used to investigate catalyst degradation due to spatio-temporal variations in the fuel cell state variables under the highly transient load cycles. A three-step (extraction, oxidation, and dissolution) model of platinum loss in the cathode catalyst layer is used to investigate the cell performance degradation due to the consequent reduction in the electro-chemical active surface area (ECSA). By using a time-upscaling methodology, we present a comparative prediction of cell end-of-life (EOL) under different driving behavior of New European Driving Cycle (NEDC) and Worldwide Harmonized Light Vehicles Test Cycle (WLTC).

Suggested Citation

  • Manik Mayur & Mathias Gerard & Pascal Schott & Wolfgang G. Bessler, 2018. "Lifetime Prediction of a Polymer Electrolyte Membrane Fuel Cell under Automotive Load Cycling Using a Physically-Based Catalyst Degradation Model," Energies, MDPI, vol. 11(8), pages 1-21, August.
    • Handle: RePEc:gam:jeners:v:11:y:2018:i:8:p:2054-:d:162528
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    References listed on IDEAS

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    1. Pérez, Luis C. & Brandão, Lúcia & Sousa, José M. & Mendes, Adélio, 2011. "Segmented polymer electrolyte membrane fuel cells--A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(1), pages 169-185, January.
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    1. Culubret, S. & Rubio, M.A. & Sanchez, D.G. & Urquia, A., 2024. "Performance uniformity analysis in polymer electrolyte fuel cell using long-term dynamic simulation," Applied Energy, Elsevier, vol. 365(C).
    2. Chiara Dall’Armi & Davide Pivetta & Rodolfo Taccani, 2023. "Hybrid PEM Fuel Cell Power Plants Fuelled by Hydrogen for Improving Sustainability in Shipping: State of the Art and Review on Active Projects," Energies, MDPI, vol. 16(4), pages 1-34, February.
    3. Xuan Meng & Jian Mei & Xingwang Tang & Jinhai Jiang & Chuanyu Sun & Kai Song, 2024. "The Degradation Prediction of Proton Exchange Membrane Fuel Cell Performance Based on a Transformer Model," Energies, MDPI, vol. 17(12), pages 1-13, June.
    4. Shantanu Pardhi & Sajib Chakraborty & Dai-Duong Tran & Mohamed El Baghdadi & Steven Wilkins & Omar Hegazy, 2022. "A Review of Fuel Cell Powertrains for Long-Haul Heavy-Duty Vehicles: Technology, Hydrogen, Energy and Thermal Management Solutions," Energies, MDPI, vol. 15(24), pages 1-55, December.
    5. Olivier Bethoux, 2020. "Hydrogen Fuel Cell Road Vehicles: State of the Art and Perspectives," Energies, MDPI, vol. 13(21), pages 1-28, November.
    6. Huu-Linh Nguyen & Sang-Min Lee & Sangseok Yu, 2023. "A Comprehensive Review of Degradation Prediction Methods for an Automotive Proton Exchange Membrane Fuel Cell," Energies, MDPI, vol. 16(12), pages 1-32, June.
    7. Lorenzo, Charles & Bouquain, David & Hibon, Samuel & Hissel, Daniel, 2021. "Synthesis of degradation mechanisms and of their impacts on degradation rates on proton-exchange membrane fuel cells and lithium-ion nickel–manganese–cobalt batteries in hybrid transport applicati," Reliability Engineering and System Safety, Elsevier, vol. 212(C).
    8. Johannes Klütsch & Stefan Pischinger, 2024. "Systematic Design of Cathode Air Supply Systems for PEM Fuel Cells," Energies, MDPI, vol. 17(14), pages 1-30, July.
    9. Zuo, Jian & Steiner, Nadia Yousfi & Li, Zhongliang & Hissel, Daniel, 2024. "Health management review for fuel cells: Focus on action phase," Renewable and Sustainable Energy Reviews, Elsevier, vol. 201(C).
    10. Liu, Hao & Chen, Jian & Hissel, Daniel & Lu, Jianguo & Hou, Ming & Shao, Zhigang, 2020. "Prognostics methods and degradation indexes of proton exchange membrane fuel cells: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 123(C).
    11. Aihua Tang & Yuanhang Yang & Quanqing Yu & Zhigang Zhang & Lin Yang, 2022. "A Review of Life Prediction Methods for PEMFCs in Electric Vehicles," Sustainability, MDPI, vol. 14(16), pages 1-18, August.
    12. Tom Fletcher & Kambiz Ebrahimi, 2020. "The Effect of Fuel Cell and Battery Size on Efficiency and Cell Lifetime for an L7e Fuel Cell Hybrid Vehicle," Energies, MDPI, vol. 13(22), pages 1-18, November.

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