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Biomass to hydrogen-rich syngas via catalytic steam reforming of bio-oil

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  • Chen, Guanyi
  • Yao, Jingang
  • Liu, Jing
  • Yan, Beibei
  • Shan, Rui

Abstract

Hydrogen-rich syngas production from the catalytic steam reforming of bio-oil from fast pyrolysis of pinewood sawdust was investigated by using La1−xKxMnO3 perovskite-type catalysts. The effects of the K substitution, temperature, water to carbon molar ratio (WCMR) and bio-oil weight hourly space velocity (WbHSV) on H2 yield, carbon conversion and the product distribution were studied in a fixed-bed reactor. The results showed that La1−xKxMnO3 perovskite-type catalysts with a K substitution of 0.2 gave the best performance and had a higher catalytic activity than the commercial Ni/ZrO2. Both high temperature and low WbHSV led to higher H2 yield. However, excessive steam reduced hydrogen yield. For the La0.8K0.2MnO3 catalyst, a hydrogen yield of 72.5% was obtained under the optimum operating condition (T = 800 °C, WCMR = 3 and WbHSV = 12 h−1). The deactivation of the catalysts mainly was caused by coke deposition.

Suggested Citation

  • Chen, Guanyi & Yao, Jingang & Liu, Jing & Yan, Beibei & Shan, Rui, 2016. "Biomass to hydrogen-rich syngas via catalytic steam reforming of bio-oil," Renewable Energy, Elsevier, vol. 91(C), pages 315-322.
    • Handle: RePEc:eee:renene:v:91:y:2016:i:c:p:315-322
    DOI: 10.1016/j.renene.2016.01.073
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    6. Xie, Huaqing & Li, Rongquan & Yu, Zhenyu & Wang, Zhengyu & Yu, Qingbo & Qin, Qin, 2020. "Combined steam/dry reforming of bio-oil for H2/CO syngas production with blast furnace slag as heat carrier," Energy, Elsevier, vol. 200(C).
    7. Huang, Yongcheng & Li, Yaoting & Han, Xudong & Zhang, Jiating & Luo, Kun & Yang, Shangsheng & Wang, Jiyuan, 2020. "Investigation on fuel properties and engine performance of the extraction phase liquid of bio-oil/biodiesel blends," Renewable Energy, Elsevier, vol. 147(P1), pages 1990-2002.
    8. Singh, Piyush Pratap & Jaswal, Anurag & Nirmalkar, Neelkanth & Mondal, Tarak, 2023. "Synergistic effect of transition metals substitution on the catalytic activity of LaNi0.5M0.5O3 (M = Co, Cu, and Fe) perovskite catalyst for steam reforming of simulated bio-oil for green hydrogen pro," Renewable Energy, Elsevier, vol. 207(C), pages 575-587.

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