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Biomass to hydrogen-rich syngas via catalytic steam reforming of bio-oil

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  • Chen, Guanyi
  • Yao, Jingang
  • Liu, Jing
  • Yan, Beibei
  • Shan, Rui

Abstract

Hydrogen-rich syngas production from the catalytic steam reforming of bio-oil from fast pyrolysis of pinewood sawdust was investigated by using La1−xKxMnO3 perovskite-type catalysts. The effects of the K substitution, temperature, water to carbon molar ratio (WCMR) and bio-oil weight hourly space velocity (WbHSV) on H2 yield, carbon conversion and the product distribution were studied in a fixed-bed reactor. The results showed that La1−xKxMnO3 perovskite-type catalysts with a K substitution of 0.2 gave the best performance and had a higher catalytic activity than the commercial Ni/ZrO2. Both high temperature and low WbHSV led to higher H2 yield. However, excessive steam reduced hydrogen yield. For the La0.8K0.2MnO3 catalyst, a hydrogen yield of 72.5% was obtained under the optimum operating condition (T = 800 °C, WCMR = 3 and WbHSV = 12 h−1). The deactivation of the catalysts mainly was caused by coke deposition.

Suggested Citation

  • Chen, Guanyi & Yao, Jingang & Liu, Jing & Yan, Beibei & Shan, Rui, 2016. "Biomass to hydrogen-rich syngas via catalytic steam reforming of bio-oil," Renewable Energy, Elsevier, vol. 91(C), pages 315-322.
    • Handle: RePEc:eee:renene:v:91:y:2016:i:c:p:315-322
    DOI: 10.1016/j.renene.2016.01.073
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    3. José Juan Alvarado-Flores & Jorge Víctor Alcaraz-Vera & María Liliana Ávalos-Rodríguez & Erandini Guzmán-Mejía & José Guadalupe Rutiaga-Quiñones & Luís Fernando Pintor-Ibarra & Santiago José Guevara-M, 2024. "Thermochemical Production of Hydrogen from Biomass: Pyrolysis and Gasification," Energies, MDPI, vol. 17(2), pages 1-21, January.
    4. Chen, Wei-Hsin & Farooq, Wasif & Shahbaz, Muhammad & Naqvi, Salman Raza & Ali, Imtiaz & Al-Ansari, Tareq & Saidina Amin, Nor Aishah, 2021. "Current status of biohydrogen production from lignocellulosic biomass, technical challenges and commercial potential through pyrolysis process," Energy, Elsevier, vol. 226(C).
    5. Elena David, 2020. "Evaluation of Hydrogen Yield Evolution in Gaseous Fraction and Biochar Structure Resulting from Walnut Shells Pyrolysis," Energies, MDPI, vol. 13(23), pages 1-17, December.
    6. Huang, Yongcheng & Li, Yaoting & Han, Xudong & Zhang, Jiating & Luo, Kun & Yang, Shangsheng & Wang, Jiyuan, 2020. "Investigation on fuel properties and engine performance of the extraction phase liquid of bio-oil/biodiesel blends," Renewable Energy, Elsevier, vol. 147(P1), pages 1990-2002.
    7. Wang, Yishuang & Liang, Defang & Wang, Chunsheng & Chen, Mingqiang & Tang, Zhiyuan & Hu, Jiaxin & Yang, Zhonglian & Zhang, Han & Wang, Jun & Liu, Shaomin, 2020. "Influence of calcination temperature of Ni/Attapulgite on hydrogen production by steam reforming ethanol," Renewable Energy, Elsevier, vol. 160(C), pages 597-611.
    8. Singh, Piyush Pratap & Jaswal, Anurag & Nirmalkar, Neelkanth & Mondal, Tarak, 2023. "Synergistic effect of transition metals substitution on the catalytic activity of LaNi0.5M0.5O3 (M = Co, Cu, and Fe) perovskite catalyst for steam reforming of simulated bio-oil for green hydrogen pro," Renewable Energy, Elsevier, vol. 207(C), pages 575-587.

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