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Aqueous phase reforming (APR) of glycerol over platinum supported on Al2O3 catalyst

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  • Seretis, A.
  • Tsiakaras, P.

Abstract

The glycerol's APR reaction over 5% Pt/Al2O3 catalyst for H2 production in a batch reactor is investigated in the present work. The effect of the operating parameters, such as the: i) reaction time, ii) operating temperature, iii) glycerol concentration and iv) catalyst concentration on: a) the gaseous and liquid products selectivity, b) the glycerol's conversion and c) the H2 yield is investigated. Initially, the glycerol's APR is studied at various temperature (200, 220, 240 °C) and reaction time (30, 60, 120, 240 min), using 1 wt.% or 10 wt.% glycerol solution and 0.5, 1, 2.5 g of 5% Pt/Al2O3 catalyst weight.

Suggested Citation

  • Seretis, A. & Tsiakaras, P., 2016. "Aqueous phase reforming (APR) of glycerol over platinum supported on Al2O3 catalyst," Renewable Energy, Elsevier, vol. 85(C), pages 1116-1126.
    • Handle: RePEc:eee:renene:v:85:y:2016:i:c:p:1116-1126
    DOI: 10.1016/j.renene.2015.07.068
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    References listed on IDEAS

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    1. Guo, Yong & Azmat, Muhammad Usman & Liu, Xiaohui & Wang, Yanqin & Lu, Guanzhong, 2012. "Effect of support’s basic properties on hydrogen production in aqueous-phase reforming of glycerol and correlation between WGS and APR," Applied Energy, Elsevier, vol. 92(C), pages 218-223.
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    4. Lucia, Umberto, 2014. "Overview on fuel cells," Renewable and Sustainable Energy Reviews, Elsevier, vol. 30(C), pages 164-169.
    5. Tuza, Pablo V. & Manfro, Robinson L. & Ribeiro, Nielson F.P. & Souza, Mariana M.V.M., 2013. "Production of renewable hydrogen by aqueous-phase reforming of glycerol over Ni–Cu catalysts derived from hydrotalcite precursors," Renewable Energy, Elsevier, vol. 50(C), pages 408-414.
    6. Menezes, André O. & Rodrigues, Michelly T. & Zimmaro, Adriana & Borges, Luiz E.P. & Fraga, Marco A., 2011. "Production of renewable hydrogen from aqueous-phase reforming of glycerol over Pt catalysts supported on different oxides," Renewable Energy, Elsevier, vol. 36(2), pages 595-599.
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    2. Kim, Min-Cheol & Kim, Tae-Wan & Kim, Hyung Ju & Kim, Chul-Ung & Bae, Jong Wook, 2016. "Aqueous phase reforming of polyols for hydrogen production using supported PtFe bimetallic catalysts," Renewable Energy, Elsevier, vol. 95(C), pages 396-403.
    3. Liu, Dashuai & Dou, Binlin & Zhang, Hua & Zhao, Longfei & Wu, Kai & Zeng, Pingchao & Chen, Haisheng & Xu, Yujie, 2022. "Comparison of gelatinous and calcined magnesia supported Ni or/and Co-based catalysts for aqueous phase reforming of glycerol," Renewable Energy, Elsevier, vol. 186(C), pages 656-666.
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    5. Justicia, Jéssica & Alberto Baeza, José & de Oliveira, Adriana S. & Calvo, Luisa & Heras, Francisco & Gilarranz, Miguel A., 2022. "Aqueous-phase reforming of water-soluble compounds from pyrolysis bio-oils," Renewable Energy, Elsevier, vol. 199(C), pages 895-907.

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