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Crude bio-glycerol aqueous phase reforming and hydrogenolysis over commercial SiO2Al2O3 nickel catalyst

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  • Seretis, Antonios
  • Tsiakaras, Panagiotis

Abstract

In the present work, an one-pot Aqueous Phase Reforming (APR) and Aqueous Phase Hydrogenolysis (APH) of crude glycerol in a batch reactor containing commercial SiO2Al2O3 supported 65%Ni catalyst is performed. The effect of: i) the glycerol’s impurities, ii) the operating temperature (200–240 °C) and iii) the crude glycerol concentration (10–40 wt%) is investigated.

Suggested Citation

  • Seretis, Antonios & Tsiakaras, Panagiotis, 2016. "Crude bio-glycerol aqueous phase reforming and hydrogenolysis over commercial SiO2Al2O3 nickel catalyst," Renewable Energy, Elsevier, vol. 97(C), pages 373-379.
    • Handle: RePEc:eee:renene:v:97:y:2016:i:c:p:373-379
    DOI: 10.1016/j.renene.2016.05.085
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    1. R. D. Cortright & R. R. Davda & J. A. Dumesic, 2002. "Hydrogen from catalytic reforming of biomass-derived hydrocarbons in liquid water," Nature, Nature, vol. 418(6901), pages 964-967, August.
    2. Tuza, Pablo V. & Manfro, Robinson L. & Ribeiro, Nielson F.P. & Souza, Mariana M.V.M., 2013. "Production of renewable hydrogen by aqueous-phase reforming of glycerol over Ni–Cu catalysts derived from hydrotalcite precursors," Renewable Energy, Elsevier, vol. 50(C), pages 408-414.
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    5. Quispe, César A.G. & Coronado, Christian J.R. & Carvalho Jr., João A., 2013. "Glycerol: Production, consumption, prices, characterization and new trends in combustion," Renewable and Sustainable Energy Reviews, Elsevier, vol. 27(C), pages 475-493.
    6. Menezes, André O. & Rodrigues, Michelly T. & Zimmaro, Adriana & Borges, Luiz E.P. & Fraga, Marco A., 2011. "Production of renewable hydrogen from aqueous-phase reforming of glycerol over Pt catalysts supported on different oxides," Renewable Energy, Elsevier, vol. 36(2), pages 595-599.
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