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Production of renewable hydrogen from aqueous-phase reforming of glycerol over Pt catalysts supported on different oxides

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  • Menezes, André O.
  • Rodrigues, Michelly T.
  • Zimmaro, Adriana
  • Borges, Luiz E.P.
  • Fraga, Marco A.

Abstract

Aqueous-phase reforming of oxygenated hydrocarbons for hydrogen production presents several advantages as feed molecules can be easily found in a wide range of biomass, there is no need for its vaporization and the process allows thorough exploitation of the environmental benefits of using hydrogen as an energy carrier. The use of glycerol in particular is motivated due to its availability as a consequence of increasing biodiesel production worldwide. In this contribution, the performance of Pt-based catalysts supported on different oxides (Al2O3, ZrO2, MgO and CeO2) is studied on glycerol reforming. All catalysts led to a hydrogen-rich gas phase. However, a good potential activity with high production of hydrogen and low concentration of undesired hydrocarbons was accomplished over the catalysts supported on MgO and ZrO2. The high electron donating character of such oxides indicates the influence of the nature of the support in catalytic performance for glycerol reforming.

Suggested Citation

  • Menezes, André O. & Rodrigues, Michelly T. & Zimmaro, Adriana & Borges, Luiz E.P. & Fraga, Marco A., 2011. "Production of renewable hydrogen from aqueous-phase reforming of glycerol over Pt catalysts supported on different oxides," Renewable Energy, Elsevier, vol. 36(2), pages 595-599.
    • Handle: RePEc:eee:renene:v:36:y:2011:i:2:p:595-599
    DOI: 10.1016/j.renene.2010.08.004
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    References listed on IDEAS

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    1. Adhikari, Sushil & Fernando, Sandun D. & Haryanto, Agus, 2008. "Hydrogen production from glycerin by steam reforming over nickel catalysts," Renewable Energy, Elsevier, vol. 33(5), pages 1097-1100.
    2. R. D. Cortright & R. R. Davda & J. A. Dumesic, 2002. "Hydrogen from catalytic reforming of biomass-derived hydrocarbons in liquid water," Nature, Nature, vol. 418(6901), pages 964-967, August.
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    1. Bruno, Arthur M. & Chagas, Carlos Alberto & Souza, Mariana M.V.M. & Manfro, Robinson L., 2018. "Lactic acid production from glycerol in alkaline medium using Pt-based catalysts in continuous flow reaction system," Renewable Energy, Elsevier, vol. 118(C), pages 160-171.
    2. Jiménez, Roberto X. & Young, André F. & Fernandes, Heloisa L.S., 2020. "Propylene glycol from glycerol: Process evaluation and break-even price determination," Renewable Energy, Elsevier, vol. 158(C), pages 181-191.
    3. Quispe, César A.G. & Coronado, Christian J.R. & Carvalho Jr., João A., 2013. "Glycerol: Production, consumption, prices, characterization and new trends in combustion," Renewable and Sustainable Energy Reviews, Elsevier, vol. 27(C), pages 475-493.
    4. Seretis, Antonios & Tsiakaras, Panagiotis, 2016. "Crude bio-glycerol aqueous phase reforming and hydrogenolysis over commercial SiO2Al2O3 nickel catalyst," Renewable Energy, Elsevier, vol. 97(C), pages 373-379.
    5. Gupta, Mayank & Kumar, Naveen, 2012. "Scope and opportunities of using glycerol as an energy source," Renewable and Sustainable Energy Reviews, Elsevier, vol. 16(7), pages 4551-4556.
    6. Seretis, A. & Tsiakaras, P., 2016. "Aqueous phase reforming (APR) of glycerol over platinum supported on Al2O3 catalyst," Renewable Energy, Elsevier, vol. 85(C), pages 1116-1126.
    7. Guo, Yong & Azmat, Muhammad Usman & Liu, Xiaohui & Wang, Yanqin & Lu, Guanzhong, 2012. "Effect of support’s basic properties on hydrogen production in aqueous-phase reforming of glycerol and correlation between WGS and APR," Applied Energy, Elsevier, vol. 92(C), pages 218-223.

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