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The process optimization and exergy efficiency analysis for biogas to renewable hydrogen by chemical looping technology

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  • Wang, Zhentong
  • Li, Huan
  • Liu, Jianguo

Abstract

The study on biogas-Chemical Looping Hydrogen Production (biogas-CLHP) highlights its potential to produce high-purity hydrogen with recycling waste bioenergy. It delves into the gas-solid reaction characteristics and optimizes crucial process parameters for the fixed-bed CLHP system. Movement rate equations for the reaction fronts of Fe2O3-Fe3O4 (Rf1), Fe3O4-FeO (Rf2), and FeO-Fe (Rf3) are formulated, aiding in clarifying CO breakthrough curves. The identified convergence temperatures (Tm) under CO and H2 atmospheres are 916 °C and 907 °C, respectively. Rf1 and Rf2 converged above Tm, which leads to the disappearance of the Fe3O4 region in oxygen carrier (OC) beds. A theoretical model for calculating the reduction solid conversion (Xaver) is established, accurately characterizing Xaver under varying reaction times, H2/CO ratios, and temperatures. By using the Particle Swarm Optimization (PSO) algorithm and thermodynamic analysis, the study determines the optimal length-radius ratio (L/r), reduction temperature (T), and H2/CO ratio (α) for the OC bed as 12.5, 916 °C, and 0.72, respectively, at which a maximum conversion ratio of 43.55 % is achieved. Based on optimal parameters, the results of Aspen simulation reveal energy and exergy efficiencies of 74.9 % and 70.8 %. Generally, this research comprehensively outlines the process dynamics, optimizes key parameters, and evaluates exergy efficiency of the biogas-CLHP system.

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  • Wang, Zhentong & Li, Huan & Liu, Jianguo, 2024. "The process optimization and exergy efficiency analysis for biogas to renewable hydrogen by chemical looping technology," Renewable Energy, Elsevier, vol. 235(C).
    • Handle: RePEc:eee:renene:v:235:y:2024:i:c:s0960148124013934
    DOI: 10.1016/j.renene.2024.121325
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    References listed on IDEAS

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