IDEAS home Printed from https://ideas.repec.org/a/eee/energy/v57y2013icp574-580.html
   My bibliography  Save this article

Optimization of parameters for hot-pressing manufacture of membrane electrode assembly for PEM (polymer electrolyte membrane fuel cells) fuel cell

Author

Listed:
  • Okur, Osman
  • İyigün Karadağ, Çiğdem
  • Boyacı San, Fatma Gül
  • Okumuş, Emin
  • Behmenyar, Gamze

Abstract

In this study, optimization of the hot-pressing parameters in manufacturing of the MEA (membrane electrode assembly) is carried out using RSM (response surface method). The important parameters to be optimized in the MEA production are temperature, pressure and the processing (pressing) time. Therefore, the studied temperature, pressure and pressing time intervals are 80–130 °C, 10–100 kg cm−2, and 1–5 min, respectively. In the RSM, the objective function to be maximized is power density, whereas temperature, pressure and pressing time are all independent variables. This method generates a non-linear quadratic equation in terms of independent parameters. Based on contour plots and variance analysis, two optimum operation conditions are determined with respect to maximum power densities. In the first case; where the manufacturing cost and difficulties in operating conditions are taken into account, maximum power density is 862 mW cm−2 at the manufacture parameters of 97 °C, 66 kg cm−2 and 3.6 min. In the second case; where temperature, pressure and hot-pressing time are set to minimum values in order to save energy and manufacturing time, maximum power density of 768 mW cm−2 is achieved at 87 °C, 48 kg cm−2 and 1.15 min.

Suggested Citation

  • Okur, Osman & İyigün Karadağ, Çiğdem & Boyacı San, Fatma Gül & Okumuş, Emin & Behmenyar, Gamze, 2013. "Optimization of parameters for hot-pressing manufacture of membrane electrode assembly for PEM (polymer electrolyte membrane fuel cells) fuel cell," Energy, Elsevier, vol. 57(C), pages 574-580.
    • Handle: RePEc:eee:energy:v:57:y:2013:i:c:p:574-580
    DOI: 10.1016/j.energy.2013.05.001
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S036054421300385X
    Download Restriction: Full text for ScienceDirect subscribers only
    File URL: https://libkey.io/10.1016/j.energy.2013.05.001?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. Carton, J.G. & Olabi, A.G., 2010. "Design of experiment study of the parameters that affect performance of three flow plate configurations of a proton exchange membrane fuel cell," Energy, Elsevier, vol. 35(7), pages 2796-2806.
    2. Carton, J.G. & Lawlor, V. & Olabi, A.G. & Hochenauer, C. & Zauner, G., 2012. "Water droplet accumulation and motion in PEM (Proton Exchange Membrane) fuel cell mini-channels," Energy, Elsevier, vol. 39(1), pages 63-73.
    3. Therdthianwong, Apichai & Manomayidthikarn, Phochan & Therdthianwong, Supaporn, 2007. "Investigation of membrane electrode assembly (MEA) hot-pressing parameters for proton exchange membrane fuel cell," Energy, Elsevier, vol. 32(12), pages 2401-2411.
    4. Zhang, Xiuqin & Guo, Juncheng & Chen, Jincan, 2010. "The parametric optimum analysis of a proton exchange membrane (PEM) fuel cell and its load matching," Energy, Elsevier, vol. 35(12), pages 5294-5299.
    5. Calise, Francesco & Ferruzzi, Gabriele & Vanoli, Laura, 2012. "Transient simulation of polygeneration systems based on PEM fuel cells and solar heating and cooling technologies," Energy, Elsevier, vol. 41(1), pages 18-30.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Parnian, Mohammad Javad & Rowshanzamir, Soosan & Gashoul, Fatemeh, 2017. "Comprehensive investigation of physicochemical and electrochemical properties of sulfonated poly (ether ether ketone) membranes with different degrees of sulfonation for proton exchange membrane fuel ," Energy, Elsevier, vol. 125(C), pages 614-628.
    2. Sayadi, Parvin & Rowshanzamir, Soosan & Parnian, Mohammad Javad, 2016. "Study of hydrogen crossover and proton conductivity of self-humidifying nanocomposite proton exchange membrane based on sulfonated poly (ether ether ketone)," Energy, Elsevier, vol. 94(C), pages 292-303.
    3. Jung, Chi-Young & Yi, Jae-You & Yi, Sung-Chul, 2014. "On the role of the silica-containing catalyst layer for proton exchange membrane fuel cells," Energy, Elsevier, vol. 68(C), pages 794-800.
    4. Najafi Roudbari, Mohsen & Ojani, Reza & Raoof, Jahan Bakhsh, 2017. "Investigation of hot pressing parameters for manufacture of catalyst-coated membrane electrode (CCME) for polymer electrolyte membrane fuel cells by response surface method," Energy, Elsevier, vol. 140(P1), pages 794-803.
    5. Rahnavard, Aylin & Rowshanzamir, Soosan & Parnian, Mohammad Javad & Amirkhanlou, Gholam Reza, 2015. "The effect of sulfonated poly (ether ether ketone) as the electrode ionomer for self-humidifying nanocomposite proton exchange membrane fuel cells," Energy, Elsevier, vol. 82(C), pages 746-757.
    6. Chen, Chaogang & Gao, Yuan, 2024. "Using multi-threshold non-local means joint distribution method to analysis the spatial distribution patterns of binder and fibers in gas diffusion layers of fuel cells," Applied Energy, Elsevier, vol. 358(C).
    7. Roudbari, Mohsen Najafi & Ojani, Reza & Raoof, Jahan Bakhsh, 2019. "Performance improvement of polymer fuel cell by simultaneously inspection of catalyst loading, catalyst content and ionomer using home-made cathodic half-cell and response surface method," Energy, Elsevier, vol. 173(C), pages 151-161.
    8. Liu, Jiaran & Tan, Jinzhu & Yang, Weizhan & Li, Yang & Wang, Chao, 2021. "Better electrochemical performance of PEMFC under a novel pneumatic clamping mechanism," Energy, Elsevier, vol. 229(C).
    9. Bhosale, Amit C. & Ghosh, Prakash C. & Assaud, Loïc, 2020. "Preparation methods of membrane electrode assemblies for proton exchange membrane fuel cells and unitized regenerative fuel cells: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 133(C).

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Rahnavard, Aylin & Rowshanzamir, Soosan & Parnian, Mohammad Javad & Amirkhanlou, Gholam Reza, 2015. "The effect of sulfonated poly (ether ether ketone) as the electrode ionomer for self-humidifying nanocomposite proton exchange membrane fuel cells," Energy, Elsevier, vol. 82(C), pages 746-757.
    2. Parnian, Mohammad Javad & Rowshanzamir, Soosan & Gashoul, Fatemeh, 2017. "Comprehensive investigation of physicochemical and electrochemical properties of sulfonated poly (ether ether ketone) membranes with different degrees of sulfonation for proton exchange membrane fuel ," Energy, Elsevier, vol. 125(C), pages 614-628.
    3. Lee, Chi-Hung & Chen, Szu-Hsien & Wang, Yen-Zen & Lin, Chao-Chien & Huang, Chih-Kai & Chuang, Ching-Nan & Wang, Chih-Kuang & Hsieh, Kuo-Huang, 2013. "Preparation and characterization of proton exchange membranes based on semi-interpenetrating sulfonated poly(imide-siloxane)/epoxy polymer networks," Energy, Elsevier, vol. 55(C), pages 905-915.
    4. Yang, Meijun & Zhang, Dongming, 2014. "Effect of surface treatment on the interfacial contact resistance and corrosion resistance of Fe–Ni–Cr alloy as a bipolar plate for polymer electrolyte membrane fuel cells," Energy, Elsevier, vol. 64(C), pages 242-247.
    5. Rakhshanpouri, S. & Rowshanzamir, S., 2013. "Water transport through a PEM (proton exchange membrane) fuel cell in a seven-layer model," Energy, Elsevier, vol. 50(C), pages 220-231.
    6. Abdollahzadeh, M. & Ribeirinha, P. & Boaventura, M. & Mendes, A., 2018. "Three-dimensional modeling of PEMFC with contaminated anode fuel," Energy, Elsevier, vol. 152(C), pages 939-959.
    7. Yuan, Zhenyu & Yang, Jie & Li, Xiaoyang & Wang, Shikai, 2016. "The micro-scale analysis of the micro direct methanol fuel cell," Energy, Elsevier, vol. 100(C), pages 10-17.
    8. Wang, Junye, 2015. "Theory and practice of flow field designs for fuel cell scaling-up: A critical review," Applied Energy, Elsevier, vol. 157(C), pages 640-663.
    9. Perng, Shiang-Wuu & Wu, Horng-Wen & Shih, Gin-Jang, 2015. "Effect of prominent gas diffusion layer (GDL) on non-isothermal transport characteristics and cell performance of a proton exchange membrane fuel cell (PEMFC)," Energy, Elsevier, vol. 88(C), pages 126-138.
    10. Mirzaei, Farokh & Parnian, Mohammad Javad & Rowshanzamir, Soosan, 2017. "Durability investigation and performance study of hydrothermal synthesized platinum-multi walled carbon nanotube nanocomposite catalyst for proton exchange membrane fuel cell," Energy, Elsevier, vol. 138(C), pages 696-705.
    11. Alipour Najmi, Ali & Rowshanzamir, Soosan & Parnian, Mohammad Javad, 2016. "Investigation of NaOH concentration effect in injected fuel on the performance of passive direct methanol alkaline fuel cell with modified cation exchange membrane," Energy, Elsevier, vol. 94(C), pages 589-599.
    12. Yuan, Zhenyu & Yang, Jie & Zhang, Yufeng & Wang, Shikai & Xu, Tingnian, 2015. "Mass transport optimization in the anode diffusion layer of a micro direct methanol fuel cell," Energy, Elsevier, vol. 93(P1), pages 599-605.
    13. Díaz, Manuel Antonio & Iranzo, Alfredo & Rosa, Felipe & Isorna, Fernando & López, Eduardo & Bolivar, Juan Pedro, 2015. "Effect of carbon dioxide on the contamination of low temperature and high temperature PEM (polymer electrolyte membrane) fuel cells. Influence of temperature, relative humidity and analysis of regener," Energy, Elsevier, vol. 90(P1), pages 299-309.
    14. An, Myung-Gi & Mehmood, Asad & Hwang, Jinyeon & Ha, Heung Yong, 2016. "A novel method of methanol concentration control through feedback of the amplitudes of output voltage fluctuations for direct methanol fuel cells," Energy, Elsevier, vol. 100(C), pages 217-226.
    15. Alipour Najmi, Ali & Rowshanzamir, Soosan & Parnian, Mohammad Javad, 2016. "Study of physicochemical characterization of potassium-doped Nafion117 membrane and performance evaluation of air-breathing fuel cell in different alkali-methanol solutions," Energy, Elsevier, vol. 113(C), pages 1090-1098.
    16. Wang, Luwen & He, Mingyan & Hu, Yue & Zhang, Yufeng & Liu, Xiaowei & Wang, Gaofeng, 2015. "A “4-cell” modular passive DMFC (direct methanol fuel cell) stack for portable applications," Energy, Elsevier, vol. 82(C), pages 229-235.
    17. Oh, Taek Hyun & Jang, Bosun & Kwon, Sejin, 2015. "Estimating the energy density of direct borohydride–hydrogen peroxide fuel cell systems for air-independent propulsion applications," Energy, Elsevier, vol. 90(P1), pages 980-986.
    18. Chou, Chang-Chen & Liu, Cheng-Hong & Chen, Bing-Hung, 2014. "Effects of reduction temperature and pH value of polyol process on reduced graphene oxide supported Pt electrocatalysts for oxygen reduction reaction," Energy, Elsevier, vol. 70(C), pages 231-238.
    19. Afshari, E. & Mosharaf-Dehkordi, M. & Rajabian, H., 2017. "An investigation of the PEM fuel cells performance with partially restricted cathode flow channels and metal foam as a flow distributor," Energy, Elsevier, vol. 118(C), pages 705-715.
    20. Ding, Xiangqian & Zhu, Yunfeng & Wei, Lingjun & Li, Ying & Li, Liquan, 2013. "Synergistic hydrogen desorption of HCS MgH2 + LiAlH4 composite," Energy, Elsevier, vol. 55(C), pages 933-938.

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:energy:v:57:y:2013:i:c:p:574-580. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.journals.elsevier.com/energy .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.