IDEAS home Printed from https://ideas.repec.org/a/eee/appene/v358y2024ics0306261923018779.html
   My bibliography  Save this article

Using multi-threshold non-local means joint distribution method to analysis the spatial distribution patterns of binder and fibers in gas diffusion layers of fuel cells

Author

Listed:
  • Chen, Chaogang
  • Gao, Yuan

Abstract

The gas diffusion layer (GDL) in fuel cell plays a crucial role in mass transfer, electron conduction and structural support. The distribution of binder and hydrophobic agent directly affects the mass transfer and conductivity of the fuel cell. In this study, a multi-threshold segmentation-based image processing method was used to distinguish between pores, fibers, and binder in the GDL. The relationship between binder distribution and fiber density as well as the thickness of the binder layer was investigated. Specifically, the study first utilized a joint distribution map based on grayscale values and non-local means values, with global Rényi entropy as the optimization objective. A bee algorithm was employed to search for the global optimal point, achieving threshold segmentation of micro-scale images. Subsequently, by comparing the results of element segmentation using one-dimensional and multi-dimensional segmentation methods, a three-dimensional convolutional kernel of different sizes was used to obtain the distance from each point in the structure to the edge, effectively separating adherent fibers. Finally, convolutional methods were used to analyze the relationship between the thickness of the binder layer and fiber density. It was found that there is a positive correlation between thickness and spatial density of fibers when the fiber layer is thin. These research findings provide theoretical basis for the content and distribution of binder in the basal layer process of GDL fabrication, and contribute to a more accurate description of the microstructure and properties of actual materials, enhancing the understanding of the preparation process and microstructure properties of GDL in fuel cells. The image processing method utilized in this study enables the computation of crucial parameters within the GDLs' multi-component segmentation algorithm, utilizing a limited sample size. Additionally, it offers valuable insights into the spatial distribution characteristics of fibers and the presence of thin matrix layers. These findings highlight the potential of this method for future applications in the realm of realistic three-dimensional structural reconstructions, thus holding promising prospects for further advancements in this field.

Suggested Citation

  • Chen, Chaogang & Gao, Yuan, 2024. "Using multi-threshold non-local means joint distribution method to analysis the spatial distribution patterns of binder and fibers in gas diffusion layers of fuel cells," Applied Energy, Elsevier, vol. 358(C).
  • Handle: RePEc:eee:appene:v:358:y:2024:i:c:s0306261923018779
    DOI: 10.1016/j.apenergy.2023.122513
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S0306261923018779
    Download Restriction: Full text for ScienceDirect subscribers only

    File URL: https://libkey.io/10.1016/j.apenergy.2023.122513?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. Okur, Osman & İyigün Karadağ, Çiğdem & Boyacı San, Fatma Gül & Okumuş, Emin & Behmenyar, Gamze, 2013. "Optimization of parameters for hot-pressing manufacture of membrane electrode assembly for PEM (polymer electrolyte membrane fuel cells) fuel cell," Energy, Elsevier, vol. 57(C), pages 574-580.
    2. Lai, Tao & Qu, Zhiguo, 2023. "Two polytetrafluoroethylene distribution effects on liquid water dynamic behavior in gas diffusion layer of polymer electrolyte membrane fuel cell with a pore-scale method," Energy, Elsevier, vol. 271(C).
    3. Lee, Yongtaek & Kim, Bosung & Kim, Yongchan & Li, Xianguo, 2011. "Degradation of gas diffusion layers through repetitive freezing," Applied Energy, Elsevier, vol. 88(12), pages 5111-5119.
    4. Guo, Lingyi & Chen, Li & Zhang, Ruiyuan & Peng, Ming & Tao, Wen-Quan, 2022. "Pore-scale simulation of two-phase flow and oxygen reactive transport in gas diffusion layer of proton exchange membrane fuel cells: Effects of nonuniform wettability and porosity," Energy, Elsevier, vol. 253(C).
    5. Yang, Bo & Li, Danyang & Zeng, Chunyuan & Chen, Yijun & Guo, Zhengxun & Wang, Jingbo & Shu, Hongchun & Yu, Tao & Zhu, Jiawei, 2021. "Parameter extraction of PEMFC via Bayesian regularization neural network based meta-heuristic algorithms," Energy, Elsevier, vol. 228(C).
    6. Ye, Lingfeng & Qiu, Diankai & Peng, Linfa & Lai, Xinmin, 2022. "Microstructures and electrical conductivity properties of compressed gas diffusion layers using X-ray tomography," Applied Energy, Elsevier, vol. 326(C).
    7. Wang, Yulin & Xu, Haokai & Zhang, Zhe & Li, Hua & Wang, Xiaodong, 2022. "Lattice Boltzmann simulation of a gas diffusion layer with a gradient polytetrafluoroethylene distribution for a proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 320(C).
    8. Chen, Huicui & Song, Zhen & Zhao, Xin & Zhang, Tong & Pei, Pucheng & Liang, Chen, 2018. "A review of durability test protocols of the proton exchange membrane fuel cells for vehicle," Applied Energy, Elsevier, vol. 224(C), pages 289-299.
    9. Oh, Hwanyeong & Park, Jaeman & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2015. "Effects of pore size gradient in the substrate of a gas diffusion layer on the performance of a proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 149(C), pages 186-193.
    10. Xia, Lingchao & Ni, Meng & He, Qijiao & Xu, Qidong & Cheng, Chun, 2021. "Optimization of gas diffusion layer in high temperature PEMFC with the focuses on thickness and porosity," Applied Energy, Elsevier, vol. 300(C).
    11. Kui Jiao & Jin Xuan & Qing Du & Zhiming Bao & Biao Xie & Bowen Wang & Yan Zhao & Linhao Fan & Huizhi Wang & Zhongjun Hou & Sen Huo & Nigel P. Brandon & Yan Yin & Michael D. Guiver, 2021. "Designing the next generation of proton-exchange membrane fuel cells," Nature, Nature, vol. 595(7867), pages 361-369, July.
    12. Yang, Yange & Li, Xiang & Chu, Tiankuo & Li, Bing & Zhang, Cunman, 2022. "Property evolution of gas diffusion layer and performance shrink of fuel cell during operation," Renewable Energy, Elsevier, vol. 194(C), pages 596-603.
    13. Bouziane, Khadidja & Khetabi, El Mahdi & Lachat, Rémy & Zamel, Nada & Meyer, Yann & Candusso, Denis, 2020. "Impact of cyclic mechanical compression on the electrical contact resistance between the gas diffusion layer and the bipolar plate of a polymer electrolyte membrane fuel cell," Renewable Energy, Elsevier, vol. 153(C), pages 349-361.
    14. Zhang, Zhonghao & Guo, Mengdi & Yu, Zhonghao & Yao, Siyue & Wang, Jin & Qiu, Diankai & Peng, Linfa, 2022. "A novel cooperative design with optimized flow field on bipolar plates and hybrid wettability gas diffusion layer for proton exchange membrane unitized regenerative fuel cell," Energy, Elsevier, vol. 239(PD).
    15. Chu, Tiankuo & Tang, Qianwen & Wang, Qinpu & Wang, Yanbo & Du, Hong & Guo, YuQing & Li, Bing & Yang, Daijun & Ming, Pingwen & Zhang, Cunman, 2023. "Experimental study on the effect of flow channel parameters on the durability of PEMFC stack and analysis of hydrogen crossover mechanism," Energy, Elsevier, vol. 264(C).
    Full references (including those not matched with items on IDEAS)

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Song Yan & Mingyang Yang & Chuanyu Sun & Sichuan Xu, 2023. "Liquid Water Characteristics in the Compressed Gradient Porosity Gas Diffusion Layer of Proton Exchange Membrane Fuel Cells Using the Lattice Boltzmann Method," Energies, MDPI, vol. 16(16), pages 1-18, August.
    2. Zhang, Xiaoqing & Yang, Jiapei & Ma, Xiao & Zhuge, Weilin & Shuai, Shijin, 2022. "Modelling and analysis on effects of penetration of microporous layer into gas diffusion layer in PEM fuel cells: Focusing on mass transport," Energy, Elsevier, vol. 254(PA).
    3. Ye, Lingfeng & Qiu, Diankai & Peng, Linfa & Lai, Xinmin, 2024. "Conduction mechanism analysis and modeling of different gas diffusion layers for PEMFC to improve their bulk conductivities via microstructure design," Applied Energy, Elsevier, vol. 362(C).
    4. Ren, Peng & Pei, Pucheng & Chen, Dongfang & Zhang, Lu & Li, Yuehua & Song, Xin & Wang, Mingkai & Wang, He, 2022. "Corrosion of metallic bipolar plates accelerated by operating conditions in a simulated PEM fuel cell cathode environment," Renewable Energy, Elsevier, vol. 194(C), pages 1277-1287.
    5. Yu, Xianxian & Cai, Shanshan & Luo, Xiaobing & Tu, Zhengkai, 2024. "Barrel effect in an air-cooled proton exchange membrane fuel cell stack," Energy, Elsevier, vol. 286(C).
    6. Abdul Ghani Olabi & Tabbi Wilberforce & Abdulrahman Alanazi & Parag Vichare & Enas Taha Sayed & Hussein M. Maghrabie & Khaled Elsaid & Mohammad Ali Abdelkareem, 2022. "Novel Trends in Proton Exchange Membrane Fuel Cells," Energies, MDPI, vol. 15(14), pages 1-35, July.
    7. Xiangyang Chen & Xianglong Luo & Chao Wang & Yingzong Liang & Jianyong Chen & Zhi Yang & Jiacheng He & Ying Chen, 2024. "Channel-to-Rib Width Ratio Optimization for the Electrical Performance Enhancement in PEMFC Based on Accurate Strain-Stress Simulation," Energies, MDPI, vol. 17(3), pages 1-28, February.
    8. Wu, Ziyao & Pei, Pucheng & Xu, Huachi & Jia, Xiaoning & Ren, Peng & Wang, Bozheng, 2019. "Study on the effect of membrane electrode assembly parameters on polymer electrolyte membrane fuel cell performance by galvanostatic charging method," Applied Energy, Elsevier, vol. 251(C), pages 1-1.
    9. Chen, Dongfang & Pei, Pucheng & Ren, Peng & Song, Xin & Wang, He & Zhang, Lu & Wang, Mingkai, 2022. "Analytical methods for the effect of anode nitrogen concentration on performance and voltage consistency of proton exchange membrane fuel cell stack," Energy, Elsevier, vol. 258(C).
    10. Zhang, Yong & He, Shirong & Jiang, Xiaohui & Yang, Xi & Wang, Zhuo & Zhang, Shuanyang & Cao, Jing & Fang, Haoyan & Li, Qiming, 2024. "Full-scale three-dimensional simulation of air cooling metal bipolar plate proton exchange membrane fuel cell stack considering a non-isothermal multiphase model," Applied Energy, Elsevier, vol. 357(C).
    11. Zhou, Yu & Chen, Ben, 2023. "Investigation of optimization and evaluation criteria for flow field in proton exchange membrane fuel cell: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 185(C).
    12. Yang, Fan & Li, Yuehua & Chen, Dongfang & Hu, Song & Xu, Xiaoming, 2024. "Parameter identification of PEMFC steady-state model based on p-dimensional extremum seeking via simplex tuning optimization method," Energy, Elsevier, vol. 292(C).
    13. Zhiming Zhang & Zhihao Chen & Kunpeng Li & Xinfeng Zhang & Caizhi Zhang & Tong Zhang, 2023. "A Multi-Field Coupled PEMFC Model with Force-Temperature-Humidity and Experimental Validation for High Electrochemical Performance Design," Sustainability, MDPI, vol. 15(16), pages 1-17, August.
    14. Zhang, Yong & He, Shirong & Jiang, Xiaohui & Xiong, Mu & Ye, Yuntao & Yang, Xi, 2023. "Three-dimensional multi-phase simulation of proton exchange membrane fuel cell performance considering constriction straight channel," Energy, Elsevier, vol. 267(C).
    15. Parnian, Mohammad Javad & Rowshanzamir, Soosan & Gashoul, Fatemeh, 2017. "Comprehensive investigation of physicochemical and electrochemical properties of sulfonated poly (ether ether ketone) membranes with different degrees of sulfonation for proton exchange membrane fuel ," Energy, Elsevier, vol. 125(C), pages 614-628.
    16. Li, Yuehua & Pei, Pucheng & Ma, Ze & Ren, Peng & Wu, Ziyao & Chen, Dongfang & Huang, Hao, 2019. "Characteristic analysis in lowering current density based on pressure drop for avoiding flooding in proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 248(C), pages 321-329.
    17. Ren, Peng & Pei, Pucheng & Li, Yuehua & Wu, Ziyao & Chen, Dongfang & Huang, Shangwei & Jia, Xiaoning, 2019. "Diagnosis of water failures in proton exchange membrane fuel cell with zero-phase ohmic resistance and fixed-low-frequency impedance," Applied Energy, Elsevier, vol. 239(C), pages 785-792.
    18. Lu, Guolong & Fan, Wenxuan & Lu, Dafeng & Zhao, Taotao & Wu, Qianqian & Liu, Mingxin & Liu, Zhenning, 2024. "Lung-inspired hybrid flow field to enhance PEMFC performance: A case of dual optimization by response surface and artificial intelligence," Applied Energy, Elsevier, vol. 355(C).
    19. Yunjie Yang & Minli Bai & Laisuo Su & Jizu Lv & Chengzhi Hu & Linsong Gao & Yang Li & Yubai Li & Yongchen Song, 2022. "One-Dimensional Numerical Simulation of Pt-Co Alloy Catalyst Aging for Proton Exchange Membrane Fuel Cells," Sustainability, MDPI, vol. 14(18), pages 1-23, September.
    20. Ahmed Mohmed Dafalla & Lin Wei & Bereket Tsegai Habte & Jian Guo & Fangming Jiang, 2022. "Membrane Electrode Assembly Degradation Modeling of Proton Exchange Membrane Fuel Cells: A Review," Energies, MDPI, vol. 15(23), pages 1-26, December.

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:appene:v:358:y:2024:i:c:s0306261923018779. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.elsevier.com/wps/find/journaldescription.cws_home/405891/description#description .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.