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CO2 capture using monoethanolamine (MEA) aqueous solution: Modeling and optimization of the solvent regeneration and CO2 desorption process

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  • Mores, Patricia
  • Scenna, Nicolás
  • Mussati, Sergio

Abstract

This paper deals with the simultaneously optimization of operating conditions (pressures, temperatures and flow-rates) and dimensions (diameter and height) of the amine regeneration unit in the post-combustion CO2 capture process. The proposed model takes into account the effect of kinetic reactions on the mass transfer, the hydraulics of the random packing and the pressure drop along the column. In addition, profiles of temperature, composition and flow-rate along the height of the regenerator are also predicted.

Suggested Citation

  • Mores, Patricia & Scenna, Nicolás & Mussati, Sergio, 2012. "CO2 capture using monoethanolamine (MEA) aqueous solution: Modeling and optimization of the solvent regeneration and CO2 desorption process," Energy, Elsevier, vol. 45(1), pages 1042-1058.
    • Handle: RePEc:eee:energy:v:45:y:2012:i:1:p:1042-1058
    DOI: 10.1016/j.energy.2012.06.038
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    References listed on IDEAS

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    2. Li, Xiaoqiang & Ding, Yudong & Guo, Liheng & Liao, Qiang & Zhu, Xun & Wang, Hong, 2019. "Non-aqueous energy-efficient absorbents for CO2 capture based on porous silica nanospheres impregnated with amine," Energy, Elsevier, vol. 171(C), pages 109-119.
    3. Dutta, Rohan & Nord, Lars O. & Bolland, Olav, 2017. "Selection and design of post-combustion CO2 capture process for 600 MW natural gas fueled thermal power plant based on operability," Energy, Elsevier, vol. 121(C), pages 643-656.
    4. Mohamadi-Baghmolaei, Mohamad & Hajizadeh, Abdollah & Zahedizadeh, Parviz & Azin, Reza & Zendehboudi, Sohrab, 2021. "Evaluation of hybridized performance of amine scrubbing plant based on exergy, energy, environmental, and economic prospects: A gas sweetening plant case study," Energy, Elsevier, vol. 214(C).
    5. Li, Bao-Hong & Zhang, Nan & Smith, Robin, 2016. "Simulation and analysis of CO2 capture process with aqueous monoethanolamine solution," Applied Energy, Elsevier, vol. 161(C), pages 707-717.
    6. N.Borhani, Tohid & Wang, Meihong, 2019. "Role of solvents in CO2 capture processes: The review of selection and design methods," Renewable and Sustainable Energy Reviews, Elsevier, vol. 114(C), pages 1-1.
    7. Wu, Xiao & Wang, Meihong & Liao, Peizhi & Shen, Jiong & Li, Yiguo, 2020. "Solvent-based post-combustion CO2 capture for power plants: A critical review and perspective on dynamic modelling, system identification, process control and flexible operation," Applied Energy, Elsevier, vol. 257(C).
    8. Kazemi, Abolghasem & Mehrabani-Zeinabad, Arjomand, 2016. "Post combustion carbon capture: Does optimization of the processing system based on energy and utility requirements warrant the lowest possible costs?," Energy, Elsevier, vol. 112(C), pages 353-363.
    9. Wilkes, Mathew Dennis & Mukherjee, Sanjay & Brown, Solomon, 2021. "Transient CO2 capture for open-cycle gas turbines in future energy systems," Energy, Elsevier, vol. 216(C).
    10. Gómez-Díaz, D. & Grueiro, J. & Navaza, J.M. & Noval, C., 2018. "CO2 absorption with tri-n-butylamine in GL and GLL systems," Energy, Elsevier, vol. 153(C), pages 568-574.
    11. Zhang, Minkai & Guo, Yincheng, 2013. "Rate based modeling of absorption and regeneration for CO2 capture by aqueous ammonia solution," Applied Energy, Elsevier, vol. 111(C), pages 142-152.
    12. Han, Siyu & Meng, Yuan & Aihemaiti, Aikelaimu & Gao, Yuchen & Ju, Tongyao & Xiang, Honglin & Jiang, Jianguo, 2022. "Biogas upgrading with various single and blended amines solutions: Capacities and kinetics," Energy, Elsevier, vol. 253(C).
    13. Jung, Wonho & Lee, Jinwon, 2022. "Thermodynamic and kinetic modeling of a novel polyamine-based solvent for energy-efficient CO2 capture with energy analysis," Energy, Elsevier, vol. 239(PE).

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