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Large-scale oxygen-enriched air (OEA) production from polymeric membranes for partial oxycombustion processes

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  • García-Luna, S.
  • Ortiz, C.
  • Chacartegui, R.
  • Pérez-Maqueda, L.A.

Abstract

Partial oxycombustion using Oxygen-Enriched Air (OEA), produced by air-gas separation with polymeric membranes, combined synergistically with CO2 capture technologies, can reduce the overall energy cost of CO2 capture, and it is a potential alternative to conventional CO2 capture technologies. An exhaustive review of polymeric membranes for this application is presented. The best membranes showed permeability values in the 450–25,100 barrer and selectivities higher than 3.6 for large-scale operations. These membranes can produce OEA with oxygen molar concentrations of up to 40% for retrofitting large-scale power plants (∼ 500 MWe) with partial oxycombustion. For OEA production, the polymeric membrane system is more efficient than cryogenic distillation since the specific power consumption of the former is 35.17 kWh/ton OEA. In comparison, that of the latter is 49.57 kWh/ton OEA. This work proposes that the OEA produced by the membranes feed a partial oxycombustion process integrated with calcium looping within a hybrid CO2 capture system. The power consumption of the hybrid CO2 capture system proposed here is 29.05% lower than in the case OEA is produced from cryogenic distillation, which justifies the potential interest in using polymeric membranes for OEA production.

Suggested Citation

  • García-Luna, S. & Ortiz, C. & Chacartegui, R. & Pérez-Maqueda, L.A., 2023. "Large-scale oxygen-enriched air (OEA) production from polymeric membranes for partial oxycombustion processes," Energy, Elsevier, vol. 268(C).
    • Handle: RePEc:eee:energy:v:268:y:2023:i:c:s0360544223000919
    DOI: 10.1016/j.energy.2023.126697
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    References listed on IDEAS

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    1. Ortiz, C. & Valverde, J.M. & Chacartegui, R. & Benítez-Guerrero, M. & Perejón, A. & Romeo, L.M., 2017. "The Oxy-CaL process: A novel CO2 capture system by integrating partial oxy-combustion with the Calcium-Looping process," Applied Energy, Elsevier, vol. 196(C), pages 1-17.
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    5. García-Luna, S. & Ortiz, C. & Carro, A. & Chacartegui, R. & Pérez-Maqueda, L.A., 2022. "Oxygen production routes assessment for oxy-fuel combustion," Energy, Elsevier, vol. 254(PB).
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    1. Ortiz, C. & García-Luna, S. & Carro, A. & Chacartegui, R. & Pérez-Maqueda, L., 2023. "Negative emissions power plant based on flexible calcium-looping process integrated with renewables and methane production," Renewable and Sustainable Energy Reviews, Elsevier, vol. 185(C).

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