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Utilization of illumination and thermal field in the preparation of jet–fuel components: The photothermic catalysis of Jatropha oil over the M/TiO2–HZSM–5

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  • Hu, Liangdong
  • Ma, Longlong
  • Hu, Guangzhi
  • Zhang, Wenjie
  • Liu, Ying
  • Xu, Rui
  • Ge, Wen
  • Chen, Yubao

Abstract

Under simultaneous illumination and heating, Jatropha oil was converted into jet–fuel components over modified catalysts. XRD, HRTEM, N2 adsorption–desorption, XRF, NH3/CO–NH3–TPD/CO–TPD, UV–Vis and TG–DTG–MS were employed to determine the surface morphology and acidic site content of the modified catalysts. Through the characterizations and experimental results, the band gap of the catalysts modified with titanium dioxide was found to be significantly reduced, which enhanced the visible light adsorption of the catalysts. Moreover, the catalyst loaded with Pt contained the highest amount of weakly acidic sites, which led to the highest conversion and selectivity for the Pt/TiO2–HZSM–5 catalyst at 100 °C and 0.4 MPa H2 pressure. In addition, the pathway of photocatalytic decarboxylation and catalytic cracking of Jatropha oil was found to involve a cascade reaction from fatty acid to Cn–1 alkane and eventually to cracking products.

Suggested Citation

  • Hu, Liangdong & Ma, Longlong & Hu, Guangzhi & Zhang, Wenjie & Liu, Ying & Xu, Rui & Ge, Wen & Chen, Yubao, 2022. "Utilization of illumination and thermal field in the preparation of jet–fuel components: The photothermic catalysis of Jatropha oil over the M/TiO2–HZSM–5," Energy, Elsevier, vol. 239(PC).
    • Handle: RePEc:eee:energy:v:239:y:2022:i:pc:s0360544221024579
    DOI: 10.1016/j.energy.2021.122209
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    1. Cui, Da & Yin, Helin & Liu, Yupeng & Li, Ji & Pan, Shuo & Wang, Qing, 2022. "Effect of final pyrolysis temperature on the composition and structure of shale oil: Synergistic use of multiple analysis and testing methods," Energy, Elsevier, vol. 252(C).
    2. Tang, Hongbiao & Lin, Jiayu & Cao, Yang & Jibran, Khalil & Li, Jin, 2022. "Influence of NiMoP phase on hydrodeoxygenation pathways of jatropha oil," Energy, Elsevier, vol. 243(C).
    3. Xing, Shiyou & Fu, Junying & Li, Ming & Yang, Gaixiu & Lv, Pengmei, 2024. "Emerging catalysis in solvent-free hydrodeoxygenation of waste lipids under mild conditions: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 200(C).

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