IDEAS home Printed from https://ideas.repec.org/a/eee/energy/v144y2018icp607-618.html
   My bibliography  Save this article

Ternary Bi2Te3In2Te3Ga2Te3 (n-type) thermoelectric film on a flexible PET substrate for use in wearables

Author

Listed:
  • Kim, Sang Hoon
  • Min, Taesik
  • Choi, Jae Won
  • Baek, Seon Hwa
  • Choi, Joon-Phil
  • Aranas, Clodualdo

Abstract

An amorphous structure of BiInGaTe powders with a small size of 10–45 μm and a low melting point of 93.2 °C is fabricated using a gas atomization technique. It is patterned using a roll-to-plate printer and then reflowed at 110 °C to become thin Bi2Te3In2Te3Ga2Te3 thermoelectric film on a flexible polyethylene terephthalate (PET) substrate. Subsequently, the electrical conductivity of the Bi2Te3In2Te3Ga2Te3 thermoelectric film increased from 6.7 × 104 S m−1 to 9.6 × 104 S m−1 and its thermal conductivity even more significantly increased from 0.9 W m−1 K−1 to 1.8 W m−1 K−1 compared to the Bi2Te3 thermoelectric film. As a result, we obtained a relatively low figure of merit (ZT) value (0.3 at 298.15 K) for the novel thermoelectric film. However, all of these results were irrelevant to the intensive phonon scattering at the hierarchical interfacial boundaries, which included the macro-scale phase boundaries of Bi2Te3/In2Te3Ga2Te3 and the nano-scale grain boundaries of each Bi2Te3, In2Te3, and Ga2Te3. As a consequence, the reduction of the ZT value of the proposed novel thermoelectric film can be attributed to the addition of In and Ga with high electrical and thermal conductivity.

Suggested Citation

  • Kim, Sang Hoon & Min, Taesik & Choi, Jae Won & Baek, Seon Hwa & Choi, Joon-Phil & Aranas, Clodualdo, 2018. "Ternary Bi2Te3In2Te3Ga2Te3 (n-type) thermoelectric film on a flexible PET substrate for use in wearables," Energy, Elsevier, vol. 144(C), pages 607-618.
    • Handle: RePEc:eee:energy:v:144:y:2018:i:c:p:607-618
    DOI: 10.1016/j.energy.2017.12.063
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S0360544217321011
    Download Restriction: Full text for ScienceDirect subscribers only
    File URL: https://libkey.io/10.1016/j.energy.2017.12.063?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. Li, Siyang & Pei, Jun & Liu, Dawei & Bao, Liangliang & Li, Jing-Feng & Wu, Huaqiang & Li, Liangliang, 2016. "Fabrication and characterization of thermoelectric power generators with segmented legs synthesized by one-step spark plasma sintering," Energy, Elsevier, vol. 113(C), pages 35-43.
    2. Tan, Ming & Deng, Yuan & Hao, Yanming, 2014. "Improved thermoelectric performance of a film device induced by densely columnar Cu electrode," Energy, Elsevier, vol. 70(C), pages 143-148.
    3. Suarez, Francisco & Parekh, Dishit P. & Ladd, Collin & Vashaee, Daryoosh & Dickey, Michael D. & Öztürk, Mehmet C., 2017. "Flexible thermoelectric generator using bulk legs and liquid metal interconnects for wearable electronics," Applied Energy, Elsevier, vol. 202(C), pages 736-745.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Sarkar, Kamanashis & Debnath, Ajit & Deb, Krishna & Bera, Arun & Saha, Biswajit, 2019. "Effect of NiO incorporation in charge transport of polyaniline: Improved polymer based thermoelectric generator," Energy, Elsevier, vol. 177(C), pages 203-210.
    2. Kong, Deyue & Zhu, Wei & Guo, Zhanpeng & Deng, Yuan, 2019. "High-performance flexible Bi2Te3 films based wearable thermoelectric generator for energy harvesting," Energy, Elsevier, vol. 175(C), pages 292-299.
    3. Fan, Zeng & Zhang, Yaoyun & Pan, Lujun & Ouyang, Jianyong & Zhang, Qian, 2021. "Recent developments in flexible thermoelectrics: From materials to devices," Renewable and Sustainable Energy Reviews, Elsevier, vol. 137(C).

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Liu, Shuang & Hu, Bingkun & Liu, Dawei & Li, Fu & Li, Jing-Feng & Li, Bo & Li, Liangliang & Lin, Yuan-Hua & Nan, Ce-Wen, 2018. "Micro-thermoelectric generators based on through glass pillars with high output voltage enabled by large temperature difference," Applied Energy, Elsevier, vol. 225(C), pages 600-610.
    2. Yu, Yuedong & Zhu, Wei & Wang, Yaling & Zhu, Pengcheng & Peng, Kang & Deng, Yuan, 2020. "Towards high integration and power density: Zigzag-type thin-film thermoelectric generator assisted by rapid pulse laser patterning technique," Applied Energy, Elsevier, vol. 275(C).
    3. Wang, Yancheng & Shi, Yaoguang & Mei, Deqing & Chen, Zichen, 2018. "Wearable thermoelectric generator to harvest body heat for powering a miniaturized accelerometer," Applied Energy, Elsevier, vol. 215(C), pages 690-698.
    4. Alluri, Nagamalleswara Rao & Selvarajan, Sophia & Chandrasekhar, Arunkumar & Saravanakumar, Balasubramaniam & Lee, Gae Myoung & Jeong, Ji Hyun & Kim, Sang-Jae, 2017. "Worm structure piezoelectric energy harvester using ionotropic gelation of barium titanate-calcium alginate composite," Energy, Elsevier, vol. 118(C), pages 1146-1155.
    5. Nour Eddine, A. & Chalet, D. & Faure, X. & Aixala, L. & Chessé, P., 2018. "Effect of engine exhaust gas pulsations on the performance of a thermoelectric generator for wasted heat recovery: An experimental and analytical investigation," Energy, Elsevier, vol. 162(C), pages 715-727.
    6. Tan, Ming & Deng, Yuan & Hao, Yanming, 2014. "Synergistic effect between ordered Bi2Te2.7Se0.3 pillar array and layered Ag electrode for remarkably enhancing thermoelectric device performance," Energy, Elsevier, vol. 77(C), pages 591-596.
    7. Kim, Choong Sun & Lee, Gyu Soup & Choi, Hyeongdo & Kim, Yong Jun & Yang, Hyeong Man & Lim, Se Hwan & Lee, Sang-Gug & Cho, Byung Jin, 2018. "Structural design of a flexible thermoelectric power generator for wearable applications," Applied Energy, Elsevier, vol. 214(C), pages 131-138.
    8. Yuan, Jinfeng & Zhu, Rong, 2020. "A fully self-powered wearable monitoring system with systematically optimized flexible thermoelectric generator," Applied Energy, Elsevier, vol. 271(C).
    9. Yijie Liu & Xiaodong Wang & Shuaihang Hou & Zuoxu Wu & Jian Wang & Jun Mao & Qian Zhang & Zhiguo Liu & Feng Cao, 2023. "Scalable-produced 3D elastic thermoelectric network for body heat harvesting," Nature Communications, Nature, vol. 14(1), pages 1-8, December.
    10. Xu, Zhiheng & Li, Junqin & Tang, Xiaobin & Liu, Yunpeng & Jiang, Tongxin & Yuan, Zicheng & Liu, Kai, 2020. "Electrodeposition preparation and optimization of fan-shaped miniaturized radioisotope thermoelectric generator," Energy, Elsevier, vol. 194(C).
    11. Karana, Dhruv Raj & Sahoo, Rashmi Rekha, 2019. "Influence of geometric parameter on the performance of a new asymmetrical and segmented thermoelectric generator," Energy, Elsevier, vol. 179(C), pages 90-99.
    12. Sargolzaeiaval, Yasaman & Ramesh, Viswanath Padmanabhan & Ozturk, Mehmet C., 2022. "A comprehensive analytical model for thermoelectric body heat harvesting incorporating the impact of human metabolism and physical activity," Applied Energy, Elsevier, vol. 324(C).
    13. Hooshmand Zaferani, Sadeq & Ghomashchi, Reza & Vashaee, Daryoosh, 2019. "Strategies for engineering phonon transport in Heusler thermoelectric compounds," Renewable and Sustainable Energy Reviews, Elsevier, vol. 112(C), pages 158-169.
    14. Lee, Dongkeon & Park, Hwanjoo & Park, Gimin & Kim, Jiyong & Kim, Hoon & Cho, Hanki & Han, Seungwoo & Kim, Woochul, 2019. "Liquid-metal-electrode-based compact, flexible, and high-power thermoelectric device," Energy, Elsevier, vol. 188(C).
    15. Soufiane El Oualid & Francis Kosior & Gerhard Span & Ervin Mehmedovic & Janina Paris & Christophe Candolfi & Bertrand Lenoir, 2022. "Influence of Thermoelectric Properties and Parasitic Effects on the Electrical Power of Thermoelectric Micro-Generators," Energies, MDPI, vol. 15(10), pages 1-13, May.
    16. Abdul Mageeth, Aqeel Mohammed & Park, SungJin & Jeong, Myunghwan & Kim, Woochul & Yu, Choongho, 2020. "Planar-type thermally chargeable supercapacitor without an effective heat sink and performance variations with layer thickness and operation conditions," Applied Energy, Elsevier, vol. 268(C).
    17. Harb, Abd El-Moneim A. & Elsayed, Khairy & Sedrak, Momtaz & Ahmed, Mahmoud & Abdo, Ahmed, 2024. "Enhancing the performance of thermoelectric generators using novel segmental arrangement of multi-functional gradient materials," Renewable Energy, Elsevier, vol. 225(C).
    18. Ni, Dan & Song, Haijun & Chen, Yuanxun & Cai, Kefeng, 2019. "Free-standing highly conducting PEDOT films for flexible thermoelectric generator," Energy, Elsevier, vol. 170(C), pages 53-61.
    19. Lee, Gyusoup & Kim, Choong Sun & Kim, Seongho & Kim, Yong Jun & Choi, Hyeongdo & Cho, Byung Jin, 2019. "Flexible heatsink based on a phase-change material for a wearable thermoelectric generator," Energy, Elsevier, vol. 179(C), pages 12-18.
    20. Sargolzaeiaval, Yasaman & Padmanabhan Ramesh, Viswanath & Neumann, Taylor V. & Misra, Veena & Vashaee, Daryoosh & Dickey, Michael D. & Öztürk, Mehmet C., 2020. "Flexible thermoelectric generators for body heat harvesting – Enhanced device performance using high thermal conductivity elastomer encapsulation on liquid metal interconnects," Applied Energy, Elsevier, vol. 262(C).

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:energy:v:144:y:2018:i:c:p:607-618. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.journals.elsevier.com/energy .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.