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Improved thermoelectric performance of a film device induced by densely columnar Cu electrode

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  • Tan, Ming
  • Deng, Yuan
  • Hao, Yanming

Abstract

In this study, it was found that the columnar Cu film is similar as a parallel microchannel which can create some sort of channels for the easy transport of electrons and phonons in the device. The p-Bi0.5Sb1.5Te3, n-Bi2Se0.3Te2.7 and Cu films were fabricated by a magnetron sputtering method. These films have been integrated into low-dimension cross-plane devices using mask-assisted deposition technology. The performance of the micro-device with densely columnar Cu film electrode has been tested, which was very superior to that of the device with ordinary structure electrode. For the typical device with 98 pairs of p/n couples, the output voltage and maximum power were up to 120.5 mV and 145.2 μW, respectively, for a temperature difference of 4 K. The device could produce a 14.6 K maximum temperature difference at current of 160 mA. The response time to reach the steady condition was less than 2 S. The results prove that excellent performance of micro-device can be realized by integrating the densely columnar Cu electrode.

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  • Tan, Ming & Deng, Yuan & Hao, Yanming, 2014. "Improved thermoelectric performance of a film device induced by densely columnar Cu electrode," Energy, Elsevier, vol. 70(C), pages 143-148.
  • Handle: RePEc:eee:energy:v:70:y:2014:i:c:p:143-148
    DOI: 10.1016/j.energy.2014.03.099
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    Cited by:

    1. Tan, Ming & Deng, Yuan & Hao, Yanming, 2014. "Synergistic effect between ordered Bi2Te2.7Se0.3 pillar array and layered Ag electrode for remarkably enhancing thermoelectric device performance," Energy, Elsevier, vol. 77(C), pages 591-596.
    2. Li, Siyang & Pei, Jun & Liu, Dawei & Bao, Liangliang & Li, Jing-Feng & Wu, Huaqiang & Li, Liangliang, 2016. "Fabrication and characterization of thermoelectric power generators with segmented legs synthesized by one-step spark plasma sintering," Energy, Elsevier, vol. 113(C), pages 35-43.
    3. Twaha, Ssennoga & Zhu, Jie & Yan, Yuying & Li, Bo, 2016. "A comprehensive review of thermoelectric technology: Materials, applications, modelling and performance improvement," Renewable and Sustainable Energy Reviews, Elsevier, vol. 65(C), pages 698-726.
    4. Liu, Shuang & Hu, Bingkun & Liu, Dawei & Li, Fu & Li, Jing-Feng & Li, Bo & Li, Liangliang & Lin, Yuan-Hua & Nan, Ce-Wen, 2018. "Micro-thermoelectric generators based on through glass pillars with high output voltage enabled by large temperature difference," Applied Energy, Elsevier, vol. 225(C), pages 600-610.
    5. Tian, Yu & Ren, Guang-Kun & Wei, Zhijie & Zheng, Zhe & Deng, Shunjie & Ma, Li & Li, Yuansen & Zhou, Zhifang & Chen, Xiaohong & Shi, Yan & Lin, Yuan-Hua, 2024. "Advances of thermoelectric power generation for room temperature: Applications, devices, materials and beyond," Renewable Energy, Elsevier, vol. 226(C).
    6. Kim, Sang Hoon & Min, Taesik & Choi, Jae Won & Baek, Seon Hwa & Choi, Joon-Phil & Aranas, Clodualdo, 2018. "Ternary Bi2Te3In2Te3Ga2Te3 (n-type) thermoelectric film on a flexible PET substrate for use in wearables," Energy, Elsevier, vol. 144(C), pages 607-618.
    7. Yu, Yuedong & Zhu, Wei & Wang, Yaling & Zhu, Pengcheng & Peng, Kang & Deng, Yuan, 2020. "Towards high integration and power density: Zigzag-type thin-film thermoelectric generator assisted by rapid pulse laser patterning technique," Applied Energy, Elsevier, vol. 275(C).

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