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High power generation and COD removal in a microbial fuel cell operated by a novel sulfonated PES/PES blend proton exchange membrane

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  • Zinadini, S.
  • Zinatizadeh, A.A.
  • Rahimi, M.
  • Vatanpour, V.
  • Rahimi, Z.

Abstract

In this paper, firstly sulfonated polyethersulfone (SPES) was synthesized from polyethersulfone (PES) with sulfonation by chlorosulfonic acid as a sulfonating agent dissolved in concentrated sulfuric acid. PES/SPES blend proton exchange membranes (PEMs) were prepared at four different compositions with the non-solvent induced phase separation technique as alternative materials to Nafion membrane for application in a microbial fuel cell (MFC). The prepared PEMs were characterized by FTIR spectroscopy, AFM, SEM, contact angle, water uptake and oxygen permeability. Performances of the fabricated PEMs and commercial Nafion 117 were evaluated in a dual chamber MFC for treating of wastewater and electricity generation. Maximum generated power and current of the fabricated membranes were 58.726 mWm−2 at current density of 317.111 mAm−2, while it was 45.512 mWm−2 at 228.673 mAm−2 for Nafion 117 at the similar experimental condition. The observed properties of low biofouling, low oxygen permeability, high power generation, high COD removal and coulombic efficiency (CE) indicated that the SPES membrane has potential to improve significantly the productivity of MFCs.

Suggested Citation

  • Zinadini, S. & Zinatizadeh, A.A. & Rahimi, M. & Vatanpour, V. & Rahimi, Z., 2017. "High power generation and COD removal in a microbial fuel cell operated by a novel sulfonated PES/PES blend proton exchange membrane," Energy, Elsevier, vol. 125(C), pages 427-438.
    • Handle: RePEc:eee:energy:v:125:y:2017:i:c:p:427-438
    DOI: 10.1016/j.energy.2017.02.146
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    2. Gao, Ningshengjie & Qu, Botong & Xing, Zhenyu & Ji, Xiulei & Zhang, Eugene & Liu, Hong, 2018. "Development of novel polyethylene air-cathode material for microbial fuel cells," Energy, Elsevier, vol. 155(C), pages 763-771.
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    4. Xin, Shuaishuai & Shen, Jianguo & Liu, Guocheng & Chen, Qinghua & Xiao, Zhou & Zhang, Guodong & Xin, Yanjun, 2020. "High electricity generation and COD removal from cattle wastewater in microbial fuel cells with 3D air cathode employed non-precious Cu2O/reduced graphene oxide as cathode catalyst," Energy, Elsevier, vol. 196(C).
    5. Shabani, Mehri & Younesi, Habibollah & Pontié, Maxime & Rahimpour, Ahmad & Rahimnejad, Mostafa & Guo, Hanxiao & Szymczyk, Anthony, 2021. "Enhancement of microbial fuel cell efficiency by incorporation of graphene oxide and functionalized graphene oxide in sulfonated polyethersulfone membrane," Renewable Energy, Elsevier, vol. 179(C), pages 788-801.
    6. Chen, Bor-Yann & Liao, Jia-Hui & Hsueh, Chung-Chuan & Qu, Ziwei & Hsu, An-Wei & Chang, Chang-Tang & Zhang, Shuping, 2018. "Deciphering biostimulation strategy of using medicinal herbs and tea extracts for bioelectricity generation in microbial fuel cells," Energy, Elsevier, vol. 161(C), pages 1042-1054.
    7. Mohamed, Hend Omar & Talas, Sawsan Abo & Sayed, Enas T. & Park, Sung-Gwan & Eisa, Tasnim & Abdelkareem, Mohammad Ali & Fadali, Olfat A. & Chae, Kyu-Jung & Castaño, Pedro, 2021. "Enhancing power generation in microbial fuel cell using tungsten carbide on reduced graphene oxide as an efficient anode catalyst material," Energy, Elsevier, vol. 229(C).
    8. Wang, Yuyang & Zhu, Lin & An, Lijuan, 2020. "Electricity generation and storage in microbial fuel cells with porous polypyrrole-base composite modified carbon brush anodes," Renewable Energy, Elsevier, vol. 162(C), pages 2220-2226.
    9. Zinadini, S. & Zinatizadeh, A.A. & Rahimi, M. & Vatanpour, V. & Bahrami, K., 2017. "Energy recovery and hygienic water production from wastewater using an innovative integrated microbial fuel cell–membrane separation process," Energy, Elsevier, vol. 141(C), pages 1350-1362.
    10. Eisa, Tasnim & Park, Sung-Gwan & Mohamed, Hend Omar & Abdelkareem, Mohammad Ali & Lee, Jieun & Yang, Euntae & Castaño, Pedro & Chae, Kyu-Jung, 2021. "Outstanding performance of direct urea/hydrogen peroxide fuel cell based on precious metal-free catalyst electrodes," Energy, Elsevier, vol. 228(C).

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