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A One-compartment direct glucose alkaline fuel cell with methyl viologen as electron mediator

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  • Liu, Xianhua
  • Hao, Miaoqing
  • Feng, Mengnan
  • Zhang, Lin
  • Zhao, Yong
  • Du, Xiwen
  • Wang, Guangyi

Abstract

Glucose is abundant, renewable, non-toxic and convenient as a fuel for fuel cells, but current technologies are unavailable for us to directly oxidize it to obtain energy. Fuel cells using enzymes and micro-organisms as catalysts are limited by their extremely low power output and rather short durability. Fuel cells using precious metal catalyst are expensive for large-scale use. In this work, a one-compartment direct glucose alkaline fuel cell has been developed that use methyl viologen (MV) as electron mediator and nickel foam as the anode. The rudimentary fuel cell generates a maximum power density of 0.62mWcm−2, while the maximum current density is 5.03mAcm−2. Electro-catalytic activities of MV and the nickel foam in alkaline conditions were studied by cyclic voltammetry. It is indicated that the high performance of the fuel cell is attributed to the combined use of MV and nickel foam. 13C-NMR and HPLC were used to analyze oxidation products of glucose. The result shows that the principal oxidation products are short-chain organic acids indicating deep oxidation of glucose is achieved.

Suggested Citation

  • Liu, Xianhua & Hao, Miaoqing & Feng, Mengnan & Zhang, Lin & Zhao, Yong & Du, Xiwen & Wang, Guangyi, 2013. "A One-compartment direct glucose alkaline fuel cell with methyl viologen as electron mediator," Applied Energy, Elsevier, vol. 106(C), pages 176-183.
    • Handle: RePEc:eee:appene:v:106:y:2013:i:c:p:176-183
    DOI: 10.1016/j.apenergy.2013.01.073
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    Cited by:

    1. Santiago, Óscar & Navarro, Emilio & Raso, Miguel A. & Leo, Teresa J., 2016. "Review of implantable and external abiotically catalysed glucose fuel cells and the differences between their membranes and catalysts," Applied Energy, Elsevier, vol. 179(C), pages 497-522.
    2. Tong Liu, 2022. "Glucose Fuel Cells and Membranes: A Brief Overview and Literature Analysis," Sustainability, MDPI, vol. 14(14), pages 1-17, July.
    3. Bahari, Meisam & Malmberg, Michael A. & Brown, Daniel M. & Hadi Nazari, S. & Lewis, Randy S. & Watt, Gerald D. & Harb, John N., 2020. "Oxidation efficiency of glucose using viologen mediators for glucose fuel cell applications with non-precious anodes," Applied Energy, Elsevier, vol. 261(C).
    4. Irfan, Muhammad & Liu, Xianhua & Li, Shengling & Khan, Izhar Ullah & Li, Yang & Wang, Jiao & Wang, Xin & Du, Xiwen & Wang, Guangyi & Zhang, Pingping, 2020. "High-performance glucose fuel cell with bimetallic Ni–Co composite anchored on reduced graphene oxide as anode catalyst," Renewable Energy, Elsevier, vol. 155(C), pages 1118-1126.

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