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Experimental study on hydrate-based CO2 removal from CH4/CO2 mixture

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  • Wang, Fei
  • Fu, Shanfei
  • Guo, Gang
  • Jia, Zhen-Zhen
  • Luo, Sheng-Jun
  • Guo, Rong-Bo

Abstract

In this work, hydrate-based CO2 removal from a CH4/CO2 mixture was studied. CH4/CO2 led to faster hydrate formation than pure CH4, because the existence of CO2 resulted in easier hydrate nucleation. Kinetic separation of CO2 was observed in the CH4/CO2 hydrate formation with different initial CO2 proportions (1.83–27.76%) due to the higher CO2 affinity of formation of hydrates. However, the initial CO2 proportion of CH4/CO2 showed no obvious effects on the hydration ratio of CH4 and CO2 and the separation efficiency when the gas was superfluous in hydrate formation. In addition, hydrate-based multistage separation of CH4/CO2 was established and conducted at different initial pressures (4, 5 and 6 MPa). The CH4 proportions were increased from 72.24% to 97.30%, 97.22% and 97.14% after separation by four, five and seven stages at initial pressures of 4, 5, and 6 MPa, respectively.

Suggested Citation

  • Wang, Fei & Fu, Shanfei & Guo, Gang & Jia, Zhen-Zhen & Luo, Sheng-Jun & Guo, Rong-Bo, 2016. "Experimental study on hydrate-based CO2 removal from CH4/CO2 mixture," Energy, Elsevier, vol. 104(C), pages 76-84.
    • Handle: RePEc:eee:energy:v:104:y:2016:i:c:p:76-84
    DOI: 10.1016/j.energy.2016.03.107
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