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Effects of operating mode and pressure on hydrate-based desalination and CO2 capture in porous media

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  • Yang, Mingjun
  • Song, Yongchen
  • Jiang, Lanlan
  • Liu, Weiguo
  • Dou, Binlin
  • Jing, Wen

Abstract

The purpose of this study was to obtain the characteristics of CO2 hydrate formation and dissociation by using different experimental modes and pressures with glass beads. From the experiments, it was found that hydrate forms rapidly in each cycle, especially at high pressure. Hydrate blockage rarely appeared during hydrate formation and dissociation when applying gas flow (Case 2); this approach was significantly better than the other two experimental modes. The maximum hydrate saturations for the three experimental modes were 28%, 24% and 67.5%. The overall hydrate saturation of Case 3 was significantly better than those of the other two cases. When a heating process was applied to induce hydrate dissociation, the rapid backpressure decrease led to migration of the pore solution during depressurization. The minimal residual water after hydrate formation resulted in consistent residual water saturation after hydrate dissociation for Case 2. Considering hydrate saturation and operating pressure, 5.00MPa is a better choice for hydrate-based desalination and CO2 capture. If the initial residual solution can be completely converted to hydrate, this technology has potential for industrial applications.

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  • Yang, Mingjun & Song, Yongchen & Jiang, Lanlan & Liu, Weiguo & Dou, Binlin & Jing, Wen, 2014. "Effects of operating mode and pressure on hydrate-based desalination and CO2 capture in porous media," Applied Energy, Elsevier, vol. 135(C), pages 504-511.
    • Handle: RePEc:eee:appene:v:135:y:2014:i:c:p:504-511
    DOI: 10.1016/j.apenergy.2014.08.095
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    Cited by:

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    6. Xia, Zhi-ming & Li, Xiao-sen & Chen, Zhao-yang & Li, Gang & Cai, Jing & Wang, Yi & Yan, Ke-feng & Xu, Chun-gang, 2017. "Hydrate-based acidic gases capture for clean methane with new synergic additives," Applied Energy, Elsevier, vol. 207(C), pages 584-593.
    7. Han, Jinju & Lee, Minkyu & Lee, Wonsuk & Lee, Youngsoo & Sung, Wonmo, 2016. "Effect of gravity segregation on CO2 sequestration and oil production during CO2 flooding," Applied Energy, Elsevier, vol. 161(C), pages 85-91.
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    9. Yi, Jie & Zhong, Dong-Liang & Yan, Jin & Lu, Yi-Yu, 2019. "Impacts of the surfactant sulfonated lignin on hydrate based CO2 capture from a CO2/CH4 gas mixture," Energy, Elsevier, vol. 171(C), pages 61-68.
    10. Sergey Misyura & Pavel Strizhak & Anton Meleshkin & Vladimir Morozov & Olga Gaidukova & Nikita Shlegel & Maria Shkola, 2023. "A Review of Gas Capture and Liquid Separation Technologies by CO 2 Gas Hydrate," Energies, MDPI, vol. 16(8), pages 1-20, April.
    11. Kim, Soyoung & Seo, Yongwon, 2015. "Semiclathrate-based CO2 capture from flue gas mixtures: An experimental approach with thermodynamic and Raman spectroscopic analyses," Applied Energy, Elsevier, vol. 154(C), pages 987-994.
    12. He, Tianbiao & Nair, Sajitha K. & Babu, Ponnivalavan & Linga, Praveen & Karimi, Iftekhar A., 2018. "A novel conceptual design of hydrate based desalination (HyDesal) process by utilizing LNG cold energy," Applied Energy, Elsevier, vol. 222(C), pages 13-24.
    13. Lv, Qiu-Nan & Li, Xiao-Sen & Chen, Zhao-Yang, 2016. "Formation of cyclopentane - methane hydrates in brine systems and characteristics of dissolved ions," Applied Energy, Elsevier, vol. 184(C), pages 482-490.
    14. Zheng, Junjie & Zhang, Peng & Linga, Praveen, 2017. "Semiclathrate hydrate process for pre-combustion capture of CO2 at near ambient temperatures," Applied Energy, Elsevier, vol. 194(C), pages 267-278.
    15. Thakre, Niraj & Jana, Amiya K., 2017. "Modeling phase equilibrium with a modified Wong-Sandler mixing rule for natural gas hydrates: Experimental validation," Applied Energy, Elsevier, vol. 205(C), pages 749-760.

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    Keywords

    Gas hydrate; CO2 capture; Desalination; Porous media;
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