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A Multi-Field Coupled PEMFC Model with Force-Temperature-Humidity and Experimental Validation for High Electrochemical Performance Design

Author

Listed:
  • Zhiming Zhang

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

  • Zhihao Chen

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

  • Kunpeng Li

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

  • Xinfeng Zhang

    (School of Information and Electrical Engineering, Zhejiang University City College, Hangzhou 310015, China)

  • Caizhi Zhang

    (College of Mechanical and Vehicle Engineering, Chongqing University, Chongqing 400044, China)

  • Tong Zhang

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

Abstract

PEMFCs (Proton Exchange Membrane Fuel Cells) are commonly used in fuel cell vehicles, which facilitates energy conversation and environmental protection. The fuel cell electrochemical performance is significantly affected by the contact resistance and the GDL (Gas Diffusion Layer) porosity due to ohmic and concentration losses. However, it is difficult to obtain the exact performance prediction of the electrochemical reaction for a fuel cell design, resulting from the complex operating conditions of fuel cells coupled with the assembly force, operating temperature, relative humidity, etc. Considering the compression behavior of porosity and the contact pressure in GDLs, a force-temperature-humidity multi-field coupled model is established based on FEA (Finite Element Analysis) and CFD (Computational Fluid Dynamics) for the fuel cell electrochemical performance. Aside from that, the characteristics between the contact resistance and the contact pressure are measured and fitted through the experiments in this study. Finally, the numerical model is validated by the experiment of the fuel cell stack, and the error rate between the presented model and the experimentation of the full-dimensional stack being a maximum of 3.37%. This work provides important insight into the force-temperature-humidity coupled action as less empirical testing is required to identify the high fuel cell performance and optimize the fuel cell parameters in a full-dimensional fuel cell stack.

Suggested Citation

  • Zhiming Zhang & Zhihao Chen & Kunpeng Li & Xinfeng Zhang & Caizhi Zhang & Tong Zhang, 2023. "A Multi-Field Coupled PEMFC Model with Force-Temperature-Humidity and Experimental Validation for High Electrochemical Performance Design," Sustainability, MDPI, vol. 15(16), pages 1-17, August.
    • Handle: RePEc:gam:jsusta:v:15:y:2023:i:16:p:12436-:d:1218240
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    References listed on IDEAS

    as
    1. Zhiming Zhang & Jun Zhang & Liang Shi & Tong Zhang, 2022. "A Study of Contact Pressure with Thermo-Mechanical Coupled Action for a Full-Dimensional PEMFC Stack," Sustainability, MDPI, vol. 14(14), pages 1-16, July.
    2. Barzegari, M.M. & Ghadimi, M. & Momenifar, M., 2020. "Investigation of contact pressure distribution on gas diffusion layer of fuel cell with pneumatic endplate," Applied Energy, Elsevier, vol. 263(C).
    3. Atyabi, Seyed Ali & Afshari, Ebrahim & Wongwises, Somchai & Yan, Wen-Mon & Hadjadj, Abdellah & Shadloo, Mostafa Safdari, 2019. "Effects of assembly pressure on PEM fuel cell performance by taking into accounts electrical and thermal contact resistances," Energy, Elsevier, vol. 179(C), pages 490-501.
    4. Bhosale, Amit C. & Rengaswamy, Raghunathan, 2019. "Interfacial contact resistance in polymer electrolyte membrane fuel cells: Recent developments and challenges," Renewable and Sustainable Energy Reviews, Elsevier, vol. 115(C).
    5. Shusheng Xiong & Zhankuan Wu & Wei Li & Daize Li & Teng Zhang & Yu Lan & Xiaoxuan Zhang & Shuyan Ye & Shuhao Peng & Zeyu Han & Jiarui Zhu & Qiujie Song & Zhixiao Jiao & Xiaofeng Wu & Heqing Huang, 2021. "Improvement of Temperature and Humidity Control of Proton Exchange Membrane Fuel Cells," Sustainability, MDPI, vol. 13(19), pages 1-14, September.
    6. Xia, Lingchao & Ni, Meng & He, Qijiao & Xu, Qidong & Cheng, Chun, 2021. "Optimization of gas diffusion layer in high temperature PEMFC with the focuses on thickness and porosity," Applied Energy, Elsevier, vol. 300(C).
    7. Bouziane, Khadidja & Khetabi, El Mahdi & Lachat, Rémy & Zamel, Nada & Meyer, Yann & Candusso, Denis, 2020. "Impact of cyclic mechanical compression on the electrical contact resistance between the gas diffusion layer and the bipolar plate of a polymer electrolyte membrane fuel cell," Renewable Energy, Elsevier, vol. 153(C), pages 349-361.
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