IDEAS home Printed from https://ideas.repec.org/a/gam/jeners/v16y2023i16p6010-d1218709.html
   My bibliography  Save this article

Liquid Water Characteristics in the Compressed Gradient Porosity Gas Diffusion Layer of Proton Exchange Membrane Fuel Cells Using the Lattice Boltzmann Method

Author

Listed:
  • Song Yan

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

  • Mingyang Yang

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

  • Chuanyu Sun

    (School of Electrical Engineering & Automation, Harbin Institute of Technology, Harbin 150001, China)

  • Sichuan Xu

    (School of Automotive Studies, Tongji University, Shanghai 201804, China)

Abstract

The mitigation of water flooding in the gas diffusion layer (GDL) at relatively high current densities is indispensable for enhancing the performance of proton exchange membrane fuel cells (PEMFCs). In this paper, a 2D multicomponent LBM model is developed to investigate the effects of porosity distribution and compression on the liquid water dynamic behaviors and distribution. The results suggest that adopting the gradient GDL structure with increasing porosity along the thickness direction significantly reduces the breakthrough time and steady–state total water saturation inside the GDL. Moreover, the positive gradient structure reaches the highest breakthrough time and water saturation at 10% compression ratio (CR) when the GDL is compressed, and the corresponding values decrease with further increase of the CR. Considering the breakthrough time, total water saturation and water distribution at the entrance of the GDL at the same time, the gradient structure with continuously increasing porosity can perform better water management capacity at 30% CR. This paper is useful for understanding the two–phase process in a gradient GDL structure and provides guidance for future design and manufacturing.

Suggested Citation

  • Song Yan & Mingyang Yang & Chuanyu Sun & Sichuan Xu, 2023. "Liquid Water Characteristics in the Compressed Gradient Porosity Gas Diffusion Layer of Proton Exchange Membrane Fuel Cells Using the Lattice Boltzmann Method," Energies, MDPI, vol. 16(16), pages 1-18, August.
  • Handle: RePEc:gam:jeners:v:16:y:2023:i:16:p:6010-:d:1218709
    as

    Download full text from publisher

    File URL: https://www.mdpi.com/1996-1073/16/16/6010/pdf
    Download Restriction: no

    File URL: https://www.mdpi.com/1996-1073/16/16/6010/
    Download Restriction: no
    ---><---

    References listed on IDEAS

    as
    1. Kui Jiao & Jin Xuan & Qing Du & Zhiming Bao & Biao Xie & Bowen Wang & Yan Zhao & Linhao Fan & Huizhi Wang & Zhongjun Hou & Sen Huo & Nigel P. Brandon & Yan Yin & Michael D. Guiver, 2021. "Designing the next generation of proton-exchange membrane fuel cells," Nature, Nature, vol. 595(7867), pages 361-369, July.
    2. Pourrahmani, Hossein & Van herle, Jan, 2022. "Water management of the proton exchange membrane fuel cells: Optimizing the effect of microstructural properties on the gas diffusion layer liquid removal," Energy, Elsevier, vol. 256(C).
    3. Abdul Ghani Olabi & Tabbi Wilberforce & Abdulrahman Alanazi & Parag Vichare & Enas Taha Sayed & Hussein M. Maghrabie & Khaled Elsaid & Mohammad Ali Abdelkareem, 2022. "Novel Trends in Proton Exchange Membrane Fuel Cells," Energies, MDPI, vol. 15(14), pages 1-35, July.
    4. Annunziata D’Orazio & Arash Karimipour & Ramin Ranjbarzadeh, 2023. "Lattice Boltzmann Modelling of Fluid Flow through Porous Media: A Comparison between Pore-Structure and Representative Elementary Volume Methods," Energies, MDPI, vol. 16(14), pages 1-20, July.
    5. Ijaodola, O.S. & El- Hassan, Zaki & Ogungbemi, E. & Khatib, F.N. & Wilberforce, Tabbi & Thompson, James & Olabi, A.G., 2019. "Energy efficiency improvements by investigating the water flooding management on proton exchange membrane fuel cell (PEMFC)," Energy, Elsevier, vol. 179(C), pages 246-267.
    6. Guo, Lingyi & Chen, Li & Zhang, Ruiyuan & Peng, Ming & Tao, Wen-Quan, 2022. "Pore-scale simulation of two-phase flow and oxygen reactive transport in gas diffusion layer of proton exchange membrane fuel cells: Effects of nonuniform wettability and porosity," Energy, Elsevier, vol. 253(C).
    7. Park, Jaeman & Oh, Hwanyeong & Lee, Yoo Il & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2016. "Effect of the pore size variation in the substrate of the gas diffusion layer on water management and fuel cell performance," Applied Energy, Elsevier, vol. 171(C), pages 200-212.
    8. Oh, Hwanyeong & Park, Jaeman & Min, Kyoungdoug & Lee, Eunsook & Jyoung, Jy-Young, 2015. "Effects of pore size gradient in the substrate of a gas diffusion layer on the performance of a proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 149(C), pages 186-193.
    9. Kong, Im Mo & Jung, Aeri & Kim, Young Sang & Kim, Min Soo, 2017. "Numerical investigation on double gas diffusion backing layer functionalized on water removal in a proton exchange membrane fuel cell," Energy, Elsevier, vol. 120(C), pages 478-487.
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Zhanhui Yao & Wei Qi & Jia Wang & Zhensen Ding & Xiaolong Jiang & Yingchen Hong & Yuejuan Li, 2023. "Safety Risk and Strategy Analysis of On-Board Hydrogen System of Hydrogen Fuel Cell Vehicles in China," Energies, MDPI, vol. 16(23), pages 1-11, November.
    2. Lyubov Slotyuk & Florian Part & Moritz-Caspar Schlegel & Floris Akkerman, 2024. "Life Cycle Assessment of the Domestic Micro Heat and Power Generation Proton Exchange Membrane Fuel Cell in Comparison with the Gas Condensing Boiler Plus Electricity from the Grid," Sustainability, MDPI, vol. 16(6), pages 1-16, March.
    3. Gozde Ustuner & Yue Hung & Devinder Mahajan, 2024. "Investigation of Proton Exchange Membrane Fuel Cell Performance by Exploring the Synergistic Effects of Reaction Parameters via Power Curve and Impedance Spectroscopy Analysis," Energies, MDPI, vol. 17(11), pages 1-14, May.
    4. Anand Sagar & Sachin Chugh & Erik Kjeang, 2023. "Model-Driven Membrane Electrode Assembly Design for High-Performing Open-Cathode Polymer Electrolyte Membrane Fuel Cells," Energies, MDPI, vol. 16(22), pages 1-23, November.
    5. Maximilian Schmitz & Fynn Matthiesen & Steffen Dirkes & Stefan Pischinger, 2024. "Predicting Liquid Water Condensation in PEM Fuel Cells by Coupling CFD with 1D Models," Energies, MDPI, vol. 17(5), pages 1-18, March.
    6. Pedro Andrade & Khaled Laadjal & Adérito Neto Alcaso & Antonio J. Marques Cardoso, 2024. "A Comprehensive Review on Condition Monitoring and Fault Diagnosis in Fuel Cell Systems: Challenges and Issues," Energies, MDPI, vol. 17(3), pages 1-45, January.
    7. Pandu Ranga Tirumalasetti & Fang-Bor Weng & Mangaliso Menzi Dlamini & Chia-Hung Chen, 2024. "Numerical Simulation of Double Layered Wire Mesh Integration on the Cathode for a Proton Exchange Membrane Fuel Cell (PEMFC)," Energies, MDPI, vol. 17(2), pages 1-15, January.
    8. Xuan Meng & Jian Mei & Xingwang Tang & Jinhai Jiang & Chuanyu Sun & Kai Song, 2024. "The Degradation Prediction of Proton Exchange Membrane Fuel Cell Performance Based on a Transformer Model," Energies, MDPI, vol. 17(12), pages 1-13, June.
    9. Nicolas Muck & Christoph David, 2023. "Integrating Fiber Sensing for Spatially Resolved Temperature Measurement in Fuel Cells," Energies, MDPI, vol. 17(1), pages 1-17, December.
    10. Gojmir Radica & Ivan Tolj & Mykhaylo V. Lototskyy & Sivakumar Pasupathi, 2023. "Air Mass Flow and Pressure Optimization of a PEM Fuel Cell Hybrid System for a Forklift Application," Energies, MDPI, vol. 17(1), pages 1-18, December.
    11. Dan Wang & Haitao Min & Honghui Zhao & Weiyi Sun & Bin Zeng & Qun Ma, 2024. "A Data-Driven Prediction Method for Proton Exchange Membrane Fuel Cell Degradation," Energies, MDPI, vol. 17(4), pages 1-17, February.
    12. Xiangyang Chen & Xianglong Luo & Chao Wang & Yingzong Liang & Jianyong Chen & Zhi Yang & Jiacheng He & Ying Chen, 2024. "Channel-to-Rib Width Ratio Optimization for the Electrical Performance Enhancement in PEMFC Based on Accurate Strain-Stress Simulation," Energies, MDPI, vol. 17(3), pages 1-28, February.
    13. Tingke Fang & Coleman Vairin & Annette von Jouanne & Emmanuel Agamloh & Alex Yokochi, 2024. "Review of Fuel-Cell Electric Vehicles," Energies, MDPI, vol. 17(9), pages 1-25, April.
    14. Nestor F. Guerrero-Rodríguez & Daniel A. De La Rosa-Leonardo & Ricardo Tapia-Marte & Francisco A. Ramírez-Rivera & Juan Faxas-Guzmán & Alexis B. Rey-Boué & Enrique Reyes-Archundia, 2024. "An Overview of the Efficiency and Long-Term Viability of Powered Hydrogen Production," Sustainability, MDPI, vol. 16(13), pages 1-29, June.
    15. Teng Teng & Xin Zhang & Qicheng Xue & Baodi Zhang, 2024. "Research of Proton Exchange Membrane Fuel Cell Modeling on Concentration Polarization under Variable-Temperature Operating Conditions," Energies, MDPI, vol. 17(3), pages 1-17, February.
    16. Ireneusz Pielecha & Filip Szwajca & Kinga Skobiej, 2023. "Load Capacity of Nickel–Metal Hydride Battery and Proton-Exchange-Membrane Fuel Cells in the Fuel-Cell-Hybrid-Electric-Vehicle Powertrain," Energies, MDPI, vol. 16(22), pages 1-14, November.

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Zhang, Xiaoqing & Yang, Jiapei & Ma, Xiao & Zhuge, Weilin & Shuai, Shijin, 2022. "Modelling and analysis on effects of penetration of microporous layer into gas diffusion layer in PEM fuel cells: Focusing on mass transport," Energy, Elsevier, vol. 254(PA).
    2. Chen, Huicui & Zhang, Ruirui & Xia, Zhifeng & Weng, Qianyao & Zhang, Tong & Pei, Pucheng, 2023. "Experimental investigation on PEM fuel cell flooding mitigation under heavy loading condition," Applied Energy, Elsevier, vol. 349(C).
    3. Chen, Chaogang & Gao, Yuan, 2024. "Using multi-threshold non-local means joint distribution method to analysis the spatial distribution patterns of binder and fibers in gas diffusion layers of fuel cells," Applied Energy, Elsevier, vol. 358(C).
    4. Liao, Shuxin & Qiu, Diankai & Yi, Peiyun & Peng, Linfa & Lai, Xinmin, 2022. "Modeling of a novel cathode flow field design with optimized sub-channels to improve drainage for proton exchange membrane fuel cells," Energy, Elsevier, vol. 261(PB).
    5. Liu, Huize & Hu, Zunyan & Li, Jianqiu & Xu, Liangfei & Shao, Yangbin & Ouyang, Minggao, 2023. "Investigation on the optimal GDL thickness design for PEMFCs considering channel/rib geometry matching and operating conditions," Energy, Elsevier, vol. 282(C).
    6. Zhao, Jian & Ozden, Adnan & Shahgaldi, Samaneh & Alaefour, Ibrahim E. & Li, Xianguo & Hamdullahpur, Feridun, 2018. "Effect of Pt loading and catalyst type on the pore structure of porous electrodes in polymer electrolyte membrane (PEM) fuel cells," Energy, Elsevier, vol. 150(C), pages 69-76.
    7. Yan, Xiaohui & Lin, Chen & Zheng, Zhifeng & Chen, Junren & Wei, Guanghua & Zhang, Junliang, 2020. "Effect of clamping pressure on liquid-cooled PEMFC stack performance considering inhomogeneous gas diffusion layer compression," Applied Energy, Elsevier, vol. 258(C).
    8. Abdul Ghani Olabi & Tabbi Wilberforce & Abdulrahman Alanazi & Parag Vichare & Enas Taha Sayed & Hussein M. Maghrabie & Khaled Elsaid & Mohammad Ali Abdelkareem, 2022. "Novel Trends in Proton Exchange Membrane Fuel Cells," Energies, MDPI, vol. 15(14), pages 1-35, July.
    9. Zhang, Jingjing & Wang, Biao & Jin, Junhong & Yang, Shenglin & Li, Guang, 2022. "A review of the microporous layer in proton exchange membrane fuel cells: Materials and structural designs based on water transport mechanism," Renewable and Sustainable Energy Reviews, Elsevier, vol. 156(C).
    10. Lin, Rui & Diao, Xiaoyu & Ma, Tiancai & Tang, Shenghao & Chen, Liang & Liu, Dengcheng, 2019. "Optimized microporous layer for improving polymer exchange membrane fuel cell performance using orthogonal test design," Applied Energy, Elsevier, vol. 254(C).
    11. Wang, Qing-Hui & Yang, Song & Zhou, Wei & Li, Jing-Rong & Xu, Zhi-Jia & Ke, Yu-Zhi & Yu, Wei & Hu, Guang-Hua, 2018. "Optimizing the porosity configuration of porous copper fiber sintered felt for methanol steam reforming micro-reactor based on flow distribution," Applied Energy, Elsevier, vol. 216(C), pages 243-261.
    12. Deng, Hao & Wang, Dawei & Wang, Renfang & Xie, Xu & Yin, Yan & Du, Qing & Jiao, Kui, 2016. "Effect of electrode design and operating condition on performance of hydrogen alkaline membrane fuel cell," Applied Energy, Elsevier, vol. 183(C), pages 1272-1278.
    13. Zhang, Yong & He, Shirong & Jiang, Xiaohui & Wang, Zhuo & Wang, Yonggang & Gu, Meng & Yang, Xi & Zhang, Shuanyang & Cao, Jing & Fang, Haoyan & Li, Qiming, 2024. "Performance and configuration optimization of proton exchange membrane fuel cell considering dual symmetric Tesla valve flow field," Energy, Elsevier, vol. 288(C).
    14. Hosseini, Mirollah & Afrouzi, Hamid Hassanzadeh & Arasteh, Hossein & Toghraie, Davood, 2019. "Energy analysis of a proton exchange membrane fuel cell (PEMFC) with an open-ended anode using agglomerate model: A CFD study," Energy, Elsevier, vol. 188(C).
    15. Huang, Haozhong & Li, Xuan & Li, Songwei & Guo, Xiaoyu & Liu, Mingxin & Wang, Tongying & Lei, Han, 2023. "Evaluating the effect of refined flow channels in a developed biomimetic flow field on PEMFC performance," Energy, Elsevier, vol. 266(C).
    16. Kermani, M.J. & Moein-Jahromi, M. & Hasheminasab, M.R. & Ebrahimi, F. & Wei, L. & Guo, J. & Jiang, F.M., 2022. "Application of a foam-based functionally graded porous material flow-distributor to PEM fuel cells," Energy, Elsevier, vol. 254(PB).
    17. Kim, Kyunghyun & Kim, Jaeyeon & Choi, Heesoo & Kwon, Obeen & Jang, Yujae & Ryu, Sangbong & Lee, Heeyun & Shim, Kyuhwan & Park, Taehyun & Cha, Suk Won, 2023. "Pre-diagnosis of flooding and drying in proton exchange membrane fuel cells by bagging ensemble deep learning models using long short-term memory and convolutional neural networks," Energy, Elsevier, vol. 266(C).
    18. Lin, Rui & Lan, Shunbo & Wu, Xiaoyan & Hao, Zhixian, 2024. "Effect of perforated cracks on liquid water in microporous layers by lattice Boltzmann method," Renewable Energy, Elsevier, vol. 222(C).
    19. Zhang, Yong & He, Shirong & Jiang, Xiaohui & Xiong, Mu & Ye, Yuntao & Yang, Xi, 2023. "Three-dimensional multi-phase simulation of proton exchange membrane fuel cell performance considering constriction straight channel," Energy, Elsevier, vol. 267(C).
    20. Cha, Dowon & Yang, Wonseok & Kim, Yongchan, 2019. "Performance improvement of self-humidifying PEM fuel cells using water injection at various start-up conditions," Energy, Elsevier, vol. 183(C), pages 514-524.

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:gam:jeners:v:16:y:2023:i:16:p:6010-:d:1218709. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: MDPI Indexing Manager (email available below). General contact details of provider: https://www.mdpi.com .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.