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Diagnosis of water failures in proton exchange membrane fuel cell with zero-phase ohmic resistance and fixed-low-frequency impedance

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  • Ren, Peng
  • Pei, Pucheng
  • Li, Yuehua
  • Wu, Ziyao
  • Chen, Dongfang
  • Huang, Shangwei
  • Jia, Xiaoning

Abstract

Water failures, which can be diagnosed with alternating-current impedance, is harmful to output properties and durability of the proton exchange membrane fuel cell. In this paper, an impedance-based measuring method of the zero-phase ohmic resistance is presented, which adjusts the measuring frequency to confine the impedance point within the ±3° sampling limitation area so as to guarantee the accuracy of 0.01 mΩ. The zero-phase ohmic resistance is sensitive to the membrane dehydration, and it decreases in the flooding process due to the gradual liquid water accumulation in the catalyst layer. The fluctuation of the zero-phase ohmic resistance increases in the flooding process, owing to the water state variation resulting from increasingly frequent water removal. A semi-empirical equivalent circuit model is used to analyze the change of mass transfer in the flooding process, and it is found that the diffusion resistance and the dissolution resistance of the reactant increase sharply. The fixed-low-frequency resistance is applicable in the flooding diagnosis, whose sensitivity changes with the chosen frequency. The highest sensitivity is corresponding to the peak value of the impedance magnitude. This paper provides adequate information about the water fault diagnosis, making sense to the fault-avoidance and the durability-promotion of the fuel cell.

Suggested Citation

  • Ren, Peng & Pei, Pucheng & Li, Yuehua & Wu, Ziyao & Chen, Dongfang & Huang, Shangwei & Jia, Xiaoning, 2019. "Diagnosis of water failures in proton exchange membrane fuel cell with zero-phase ohmic resistance and fixed-low-frequency impedance," Applied Energy, Elsevier, vol. 239(C), pages 785-792.
    • Handle: RePEc:eee:appene:v:239:y:2019:i:c:p:785-792
    DOI: 10.1016/j.apenergy.2019.01.235
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    2. Li, Yuehua & Pei, Pucheng & Wu, Ziyao & Ren, Peng & Jia, Xiaoning & Chen, Dongfang & Huang, Shangwei, 2018. "Approaches to avoid flooding in association with pressure drop in proton exchange membrane fuel cells," Applied Energy, Elsevier, vol. 224(C), pages 42-51.
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    Cited by:

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    2. Xiao, Fei & Chen, Tao & Gan, Zhongyu & Zhang, Ruixuan, 2023. "The influence of external operating conditions on membrane drying faults of proton-exchange membrane fuel cells," Energy, Elsevier, vol. 285(C).
    3. Chen, Guohua & Li, Geliang & Xie, Mulin & Xu, Qiming & Zhang, Geng, 2024. "A probabilistic analysis method based on Noisy-OR gate Bayesian network for hydrogen leakage of proton exchange membrane fuel cell," Reliability Engineering and System Safety, Elsevier, vol. 243(C).
    4. Kim, Kyunghyun & Kim, Jaeyeon & Choi, Heesoo & Kwon, Obeen & Jang, Yujae & Ryu, Sangbong & Lee, Heeyun & Shim, Kyuhwan & Park, Taehyun & Cha, Suk Won, 2023. "Pre-diagnosis of flooding and drying in proton exchange membrane fuel cells by bagging ensemble deep learning models using long short-term memory and convolutional neural networks," Energy, Elsevier, vol. 266(C).
    5. Bahrami, Milad & Martin, Jean-Philippe & Maranzana, Gaël & Pierfederici, Serge & Weber, Mathieu & Didierjean, Sophie, 2022. "Fuel cell management system: An approach to increase its durability," Applied Energy, Elsevier, vol. 306(PB).
    6. Li, Yuehua & Pei, Pucheng & Ma, Ze & Ren, Peng & Wu, Ziyao & Chen, Dongfang & Huang, Hao, 2019. "Characteristic analysis in lowering current density based on pressure drop for avoiding flooding in proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 248(C), pages 321-329.
    7. Li, Yuehua & Pei, Pucheng & Ma, Ze & Ren, Peng & Huang, Hao, 2020. "Analysis of air compression, progress of compressor and control for optimal energy efficiency in proton exchange membrane fuel cell," Renewable and Sustainable Energy Reviews, Elsevier, vol. 133(C).
    8. Zhang, Xiaojie & Zhang, Tong & Chen, Huicui & Cao, Yinliang, 2021. "A review of online electrochemical diagnostic methods of on-board proton exchange membrane fuel cells," Applied Energy, Elsevier, vol. 286(C).
    9. Ren, Peng & Pei, Pucheng & Chen, Dongfang & Li, Yuehua & Wu, Ziyao & Zhang, Lu & Li, Zizhao & Wang, Mingkai & Wang, He & Wang, Bozheng & Wang, Xizhong, 2022. "Novel analytic method of membrane electrode assembly parameters for fuel cell consistency evaluation by micro-current excitation," Applied Energy, Elsevier, vol. 306(PB).
    10. Lin, Chen & Yan, Xiaohui & Wei, Guanghua & Ke, Changchun & Shen, Shuiyun & Zhang, Junliang, 2019. "Optimization of configurations and cathode operating parameters on liquid-cooled proton exchange membrane fuel cell stacks by orthogonal method," Applied Energy, Elsevier, vol. 253(C), pages 1-1.
    11. Zhao, Lei & Yuan, Hao & Xie, Jiaping & Jiang, Shangfeng & Wei, Xuezhe & Tang, Wei & Ming, Pingwen & Dai, Haifeng, 2023. "Inconsistency evaluation of vehicle-oriented fuel cell stacks based on electrochemical impedance under dynamic operating conditions," Energy, Elsevier, vol. 265(C).
    12. Zhao, Lei & Hong, Jichao & Xie, Jiaping & Jiang, Shangfeng & Wei, Xuezhe & Ming, Pingwen & Dai, Haifeng, 2023. "Investigation of local sensitivity for vehicle-oriented fuel cell stacks based on electrochemical impedance spectroscopy," Energy, Elsevier, vol. 262(PA).
    13. Fan Yang & Xiaoming Xu & Yuehua Li & Dongfang Chen & Song Hu & Ziwen He & Yi Du, 2023. "A Review on Mass Transfer in Multiscale Porous Media in Proton Exchange Membrane Fuel Cells: Mechanism, Modeling, and Parameter Identification," Energies, MDPI, vol. 16(8), pages 1-24, April.
    14. Lu Zhang & Yongfeng Liu & Guijun Bi & Xintong Liu & Long Wang & Yuan Wan & Hua Sun, 2022. "Modeling and Experimental Investigation of the Anode Inlet Relative Humidity Effect on a PEM Fuel Cell," Energies, MDPI, vol. 15(13), pages 1-20, June.
    15. Bizon, Nicu & Pierfederici, Serge & Bahrami, Milad & Thounthong, Phatiphat, 2022. "Power equalizer for a series fuel cell architecture based on load tracking control," Renewable and Sustainable Energy Reviews, Elsevier, vol. 166(C).
    16. Cheng, Ming & Luo, Liuxuan & Feng, Yong & Feng, Qilong & Yan, Xiaohui & Shen, Shuiyun & Guo, Yangge & Zhang, Junliang, 2024. "Numerical studies on porous water transport plates applied in PEMFCs under pure oxygen condition," Applied Energy, Elsevier, vol. 362(C).
    17. Jiaping Xie & Hao Yuan & Yufeng Wu & Chao Wang & Xuezhe Wei & Haifeng Dai, 2023. "Impedance Acquisition of Proton Exchange Membrane Fuel Cell Using Deeper Learning Network," Energies, MDPI, vol. 16(14), pages 1-18, July.
    18. Ren, Peng & Meng, Yining & Pei, Pucheng & Fu, Xi & Chen, Dongfang & Li, Yuehua & Zhu, Zijing & Zhang, Lu & Wang, Mingkai, 2023. "Rapid synchronous state-of-health diagnosis of membrane electrode assemblies in fuel cell stacks," Applied Energy, Elsevier, vol. 330(PA).
    19. Lee, Jiseung & Salihi, Hassan & Lee, Jaeseung & Ju, Hyunchul, 2022. "Impedance modeling for polymer electrolyte membrane fuel cells by combining the transient two-phase fuel cell and equivalent electric circuit models," Energy, Elsevier, vol. 239(PC).
    20. Kwon, Obeen & Kim, Jaeyeon & Choi, Heesoo & Cha, Hyeonjin & Shin, Myunggyu & Jeong, Youngjin & Park, Taehyun, 2022. "CNT sheet as a cathodic functional interlayer in polymer electrolyte membrane fuel cells," Energy, Elsevier, vol. 245(C).
    21. Kim, Jaeyeon & Kim, Hyeok & Song, Hyeonjun & Kim, Dasol & Kim, Geon Hwi & Im, Dasom & Jeong, Youngjin & Park, Taehyun, 2021. "Carbon nanotube sheet as a microporous layer for proton exchange membrane fuel cells," Energy, Elsevier, vol. 227(C).
    22. Behzad Najafi & Paolo Bonomi & Andrea Casalegno & Fabio Rinaldi & Andrea Baricci, 2020. "Rapid Fault Diagnosis of PEM Fuel Cells through Optimal Electrochemical Impedance Spectroscopy Tests," Energies, MDPI, vol. 13(14), pages 1-19, July.

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