IDEAS home Printed from https://ideas.repec.org/a/eee/appene/v352y2023ics0306261923013260.html
   My bibliography  Save this article

Investigation of output performance and temperature distribution uniformity of PEMFC based on Pt loading gradient design

Author

Listed:
  • Wei, Pengnan
  • Chang, Guofeng
  • Fan, Ruijia
  • Xu, Yiming
  • Chen, Siqi

Abstract

Temperature distribution uniformity within the cathode catalyst layer (CCL) and power density are two crucial parameters to characterize the durability and output performance of proton exchange membrane fuel cells (PEMFCs), which are affected by the Pt distribution within the CCL. Therefore, the temperature distribution uniformity within the CCL and the output performance at different operating voltages for a PEMFC with various Pt loading gradient distributions along the in-plane (IP) direction are investigated in this paper. Moreover, a two-dimensional, two-phase, non-isothermal model is developed, and the concepts of high power density range (HPDR) and temperature uniformity index (TUI) are defined in this study. The results indicate that gradient Pt distribution has the opposite effect on output performance and temperature distribution uniformity at low and medium operating voltages; the improvement of one indicator means the deterioration of another. Besides, the optimal output performance is obtained with the uniform Pt distribution at high operating voltages, while the ideal temperature distribution uniformity is achieved by loading more Pt under the channel. Consequently, the output performance and temperature distribution uniformity must be traded off to obtain optimal comprehensive performance of PEMFC at different operating voltages when designing the Pt loading gradient distribution.

Suggested Citation

  • Wei, Pengnan & Chang, Guofeng & Fan, Ruijia & Xu, Yiming & Chen, Siqi, 2023. "Investigation of output performance and temperature distribution uniformity of PEMFC based on Pt loading gradient design," Applied Energy, Elsevier, vol. 352(C).
    • Handle: RePEc:eee:appene:v:352:y:2023:i:c:s0306261923013260
    DOI: 10.1016/j.apenergy.2023.121962
    as

    Download full text from publisher

    File URL: http://www.sciencedirect.com/science/article/pii/S0306261923013260
    Download Restriction: Full text for ScienceDirect subscribers only
    File URL: https://libkey.io/10.1016/j.apenergy.2023.121962?utm_source=ideas
    LibKey link: if access is restricted and if your library uses this service, LibKey will redirect you to where you can use your library subscription to access this item
    ---><---

    As the access to this document is restricted, you may want to search for a different version of it.

    References listed on IDEAS

    as
    1. Wang, Qianqian & Tang, Fumin & Li, Bing & Dai, Haifeng & Zheng, Jim P. & Zhang, Cunman & Ming, Pingwen, 2022. "Investigation of the thermal responses under gas channel and land inside proton exchange membrane fuel cell with assembly pressure," Applied Energy, Elsevier, vol. 308(C).
    2. Song, Zhen & Pan, Yue & Chen, Huicui & Zhang, Tong, 2021. "Effects of temperature on the performance of fuel cell hybrid electric vehicles: A review," Applied Energy, Elsevier, vol. 302(C).
    3. Roshandel, Ramin & Ahmadi, Farzad, 2013. "Effects of catalyst loading gradient in catalyst layers on performance of polymer electrolyte membrane fuel cells," Renewable Energy, Elsevier, vol. 50(C), pages 921-931.
    4. Ebrahimi, Sasan & Ghorbani, Babak & Vijayaraghavan, Krishna, 2017. "Optimization of catalyst distribution along PEMFC channel through a numerical two-phase model and genetic algorithm," Renewable Energy, Elsevier, vol. 113(C), pages 846-854.
    5. He, Pu & Mu, Yu-Tong & Park, Jae Wan & Tao, Wen-Quan, 2020. "Modeling of the effects of cathode catalyst layer design parameters on performance of polymer electrolyte membrane fuel cell," Applied Energy, Elsevier, vol. 277(C).
    6. Fan, Ruijia & Chang, Guofeng & Xu, Yiming & Xu, Jiamin, 2023. "Multi-objective optimization of graded catalyst layer to improve performance and current density uniformity of a PEMFC," Energy, Elsevier, vol. 262(PB).
    7. Chen, Ben & Liu, Qi & Zhang, Cheng & Liu, Yang & Shen, Jun & Tu, Zhengkai, 2022. "Numerical study on water transfer characteristics under joint effect of placement orientation and flow channel size for PEMFC with dead-ended anode," Energy, Elsevier, vol. 254(PB).
    8. Li, Yubai & Zhou, Zhifu & Liu, Xianglei & Wu, Wei-Tao, 2019. "Modeling of PEM fuel cell with thin MEA under low humidity operating condition," Applied Energy, Elsevier, vol. 242(C), pages 1513-1527.
    9. Xing, Lei & Das, Prodip K. & Song, Xueguan & Mamlouk, Mohamed & Scott, Keith, 2015. "Numerical analysis of the optimum membrane/ionomer water content of PEMFCs: The interaction of Nafion® ionomer content and cathode relative humidity," Applied Energy, Elsevier, vol. 138(C), pages 242-257.
    10. Zeng, Tao & Zhang, Caizhi & Hao, Dong & Cao, Dongpu & Chen, Jiawei & Chen, Jinrui & Li, Jin, 2020. "Data-driven approach for short-term power demand prediction of fuel cell hybrid vehicles," Energy, Elsevier, vol. 208(C).
    Full references (including those not matched with items on IDEAS)

    Citations

    Citations are extracted by the CitEc Project, subscribe to its RSS feed for this item.
    as


    Cited by:

    1. Ma, Haoran & Liu, Junheng & Liang, Wenwen & Li, Jiyu & Zhao, Wenyao & Sun, Ping & Ji, Qian, 2024. "Effects of PEMFC cooling channel insulation coating on heat transfer and electrical discharge characteristics of nanofluid coolants," Applied Energy, Elsevier, vol. 357(C).
    2. Mehrazi, Shirin & Homayouni, Taymaz & Kakati, Nitul & Sarker, Mrittunjoy & Rolfe, Philip & Chuang, Po-Ya Abel, 2024. "A Rheo-Impedance investigation on the interparticle interactions in the catalyst ink and its impact on electrode network formation in a proton exchange membrane fuel cell," Applied Energy, Elsevier, vol. 359(C).

    Most related items

    These are the items that most often cite the same works as this one and are cited by the same works as this one.
    1. Fan, Ruijia & Chang, Guofeng & Xu, Yiming & Zhang, Yuanzhi, 2024. "Investigating the transient electrical behaviors in PEM fuel cells under various platinum distributions within cathode catalyst layers," Applied Energy, Elsevier, vol. 359(C).
    2. Fan, Ruijia & Chang, Guofeng & Xu, Yiming & Xu, Jiamin, 2024. "Investigating and quantifying the effects of catalyst layer gradients, operating conditions, and their interactions on PEMFC performance through global sensitivity analysis," Energy, Elsevier, vol. 290(C).
    3. Fan, Ruijia & Chang, Guofeng & Xu, Yiming & Xu, Jiamin, 2023. "Multi-objective optimization of graded catalyst layer to improve performance and current density uniformity of a PEMFC," Energy, Elsevier, vol. 262(PB).
    4. Chen, Ke & Luo, Zongkai & Zou, Guofu & He, Dandi & Xiong, Zhongzhuang & Zhou, Yu & Chen, Ben, 2024. "Multi-objective optimization of gradient gas diffusion layer structures for enhancing proton exchange membrane fuel cell performance based on response surface methodology and non-dominated sorting gen," Energy, Elsevier, vol. 288(C).
    5. Yao, Jing & Wu, Zhen & Wang, Huan & Yang, Fusheng & Xuan, Jin & Xing, Lei & Ren, Jianwei & Zhang, Zaoxiao, 2022. "Design and multi-objective optimization of low-temperature proton exchange membrane fuel cells with efficient water recovery and high electrochemical performance," Applied Energy, Elsevier, vol. 324(C).
    6. Saeidfar, Asal & Yesilyurt, Serhat, 2023. "Numerical investigation of the effects of catalyst layer composition and channel to rib width ratios for low platinum loaded PEMFCs," Applied Energy, Elsevier, vol. 339(C).
    7. Abdollahipour, Armin & Sayyaadi, Hoseyn, 2022. "A novel electrochemical refrigeration system based on the combined proton exchange membrane fuel cell-electrolyzer," Applied Energy, Elsevier, vol. 316(C).
    8. Wu, Horng-Wen, 2016. "A review of recent development: Transport and performance modeling of PEM fuel cells," Applied Energy, Elsevier, vol. 165(C), pages 81-106.
    9. Yuan, Hao & Dai, Haifeng & Ming, Pingwen & Li, Sida & Wei, Xuezhe, 2022. "A new insight into the effects of agglomerate parameters on internal dynamics of proton exchange membrane fuel cell by an advanced impedance dimension model," Energy, Elsevier, vol. 253(C).
    10. Chen, Ben & Deng, Qihao & Yang, Guanghua & Zhou, Yu & Chen, Wenshang & Cai, Yonghua & Tu, Zhengkai, 2023. "Numerical study on heat transfer characteristics and performance evaluation of PEMFC based on multiphase electrochemical model coupled with cooling channel," Energy, Elsevier, vol. 285(C).
    11. Abdollahzadeh, M. & Ribeirinha, P. & Boaventura, M. & Mendes, A., 2018. "Three-dimensional modeling of PEMFC with contaminated anode fuel," Energy, Elsevier, vol. 152(C), pages 939-959.
    12. Ahmed Mohmed Dafalla & Lin Wei & Bereket Tsegai Habte & Jian Guo & Fangming Jiang, 2022. "Membrane Electrode Assembly Degradation Modeling of Proton Exchange Membrane Fuel Cells: A Review," Energies, MDPI, vol. 15(23), pages 1-26, December.
    13. Teng Teng & Xin Zhang & Qicheng Xue & Baodi Zhang, 2024. "Research of Proton Exchange Membrane Fuel Cell Modeling on Concentration Polarization under Variable-Temperature Operating Conditions," Energies, MDPI, vol. 17(3), pages 1-17, February.
    14. Su, Chao & Chen, Zhidong & Wu, Zexuan & Zhang, Jing & Li, Kaiyang & Hao, Junhong & Kong, Yanqiang & Zhang, Naiqiang, 2024. "Experimental and numerical study of thermal coupling on catalyst-coated membrane for proton exchange membrane water electrolyzer," Applied Energy, Elsevier, vol. 357(C).
    15. Tzelepis, Stefanos & Kavadias, Kosmas A. & Marnellos, George E. & Xydis, George, 2021. "A review study on proton exchange membrane fuel cell electrochemical performance focusing on anode and cathode catalyst layer modelling at macroscopic level," Renewable and Sustainable Energy Reviews, Elsevier, vol. 151(C).
    16. Wang, Qianqian & Tang, Fumin & Li, Bing & Dai, Haifeng & Zheng, Jim P. & Zhang, Cunman & Ming, Pingwen, 2022. "Investigation of the thermal responses under gas channel and land inside proton exchange membrane fuel cell with assembly pressure," Applied Energy, Elsevier, vol. 308(C).
    17. Li, Xiang & Tang, Fumin & Wang, Qianqian & Li, Bing & Dai, Haifeng & Chang, Guofeng & Zhang, Cunman & Ming, Pingwen, 2023. "Effect of cathode catalyst layer on proton exchange membrane fuel cell performance: Considering the spatially variable distribution," Renewable Energy, Elsevier, vol. 212(C), pages 644-654.
    18. Zhang, Ruiyuan & Min, Ting & Chen, Li & Li, Hailong & Yan, Jinyue & Tao, Wen-Quan, 2022. "Pore-scale study of effects of relative humidity on reactive transport processes in catalyst layers in PEMFC," Applied Energy, Elsevier, vol. 323(C).
    19. Ebrahimi, Sasan & Ghorbani, Babak & Vijayaraghavan, Krishna, 2017. "Optimization of catalyst distribution along PEMFC channel through a numerical two-phase model and genetic algorithm," Renewable Energy, Elsevier, vol. 113(C), pages 846-854.
    20. Pan, Mingzhang & Pan, Chengjie & Li, Chao & Zhao, Jian, 2021. "A review of membranes in proton exchange membrane fuel cells: Transport phenomena, performance and durability," Renewable and Sustainable Energy Reviews, Elsevier, vol. 141(C).

    Corrections

    All material on this site has been provided by the respective publishers and authors. You can help correct errors and omissions. When requesting a correction, please mention this item's handle: RePEc:eee:appene:v:352:y:2023:i:c:s0306261923013260. See general information about how to correct material in RePEc.

    If you have authored this item and are not yet registered with RePEc, we encourage you to do it here. This allows to link your profile to this item. It also allows you to accept potential citations to this item that we are uncertain about.

    If CitEc recognized a bibliographic reference but did not link an item in RePEc to it, you can help with this form .

    If you know of missing items citing this one, you can help us creating those links by adding the relevant references in the same way as above, for each refering item. If you are a registered author of this item, you may also want to check the "citations" tab in your RePEc Author Service profile, as there may be some citations waiting for confirmation.

    For technical questions regarding this item, or to correct its authors, title, abstract, bibliographic or download information, contact: Catherine Liu (email available below). General contact details of provider: http://www.elsevier.com/wps/find/journaldescription.cws_home/405891/description#description .

    Please note that corrections may take a couple of weeks to filter through the various RePEc services.

    IDEAS is a RePEc service. RePEc uses bibliographic data supplied by the respective publishers.