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Hydrogen production from steam gasification of polyethylene using a two-stage gasifier and active carbon

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  • Jeong, Yong-Seong
  • Park, Ki-Bum
  • Kim, Joo-Sik

Abstract

Steam gasification of polyethylene was conducted using a two-stage gasifier consisting of a fluidized bed gasifier and a tar-cracking reactor filled with active carbon. The main aim of the work was to produce H2-rich syngas and simultaneously reduce tar. The main reaction variable was the steam-to-fuel ratio. The possibility of gasification without using an electrostatic precipitator was also examined in the study. In addition, the effect of the type of distributor (hook-type and mesh-type distributor) located between the fluidized bed gasifier and tar-cracking reactor on coke formation was investigated. Finally, the possibility of in situ regeneration of active carbon with steam was explored. As a result, the syngas from the two-stage gasifier contained a maximum 66 vol% hydrogen and a minimum 0 mg/Nm3 tar. The syngas produced without using an electrostatic precipitator had similar quality to that obtained with an electrostatic precipitator, providing a positive indication for the implementation of the two-stage gasifier in commercial applications. Additionally, the mesh-type distributor was found to be excellent against coke formation. The in situ regeneration of active carbon with steam significantly recovered the textural properties of the original active carbon, yielding a surface area recovery rate of approximately 63%. A long-term gasification for 4 h with repetitive in situ regeneration of active carbon with steam produced a syngas having 55 vol% H2 on average and toluene as a tar component.

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  • Jeong, Yong-Seong & Park, Ki-Bum & Kim, Joo-Sik, 2020. "Hydrogen production from steam gasification of polyethylene using a two-stage gasifier and active carbon," Applied Energy, Elsevier, vol. 262(C).
    • Handle: RePEc:eee:appene:v:262:y:2020:i:c:s0306261920300076
    DOI: 10.1016/j.apenergy.2020.114495
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    5. Ehsan Doniavi & Reza Babazadeh & Rezgar Hasanzadeh, 2023. "Optimization of Renewable Energy Supply Chain for Sustainable Hydrogen Energy Production from Plastic Waste," Sustainability, MDPI, vol. 15(24), pages 1-26, December.
    6. Zou, Jiecheng & Zhao, Lanxun & Hu, Qiang & Yao, Dingding & Yang, Haiping, 2024. "Pyrolysis and catalytic reforming of disposable plastic waste for syngas production with adjustable H2/CO ratio," Applied Energy, Elsevier, vol. 362(C).
    7. Kim, Jae-Kyung & Jeong, Yong-Seong & Kim, Jong-Woo & Kim, Joo-Sik, 2023. "Two-stage thermochemical conversion of polyethylene terephthalate using steam to produce a clean and H2- and CO-rich syngas," Energy, Elsevier, vol. 276(C).
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