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Analysis of the reduction of energy cost by using MEA-MDEA-PZ solvent for post-combustion carbon dioxide capture (PCC)

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  • Zhang, Rui
  • Zhang, Xiaowen
  • Yang, Qi
  • Yu, Hai
  • Liang, Zhiwu
  • Luo, Xiao

Abstract

The blends of monoethanolamine (MEA), N-methyl-diethanolamine (MDEA) and piperazine (PZ) as a solvent for CO2 capture were investigated in terms of CO2 absorption-desorption performance. The total concentration of the blends was 6M mixed with different amine molar ratios, 3M MEA-2.5M MDEA-0.5M PZ (Blend-1), 3M MEA-2M MDEA-1M PZ (Blend-2) and 3M MEA-1.5M MDEA-1.5M PZ (Blend-3). The CO2 equilibrium solubility, absorption capacity, initial absorption rate, speciation, relative energy consumption and heat of absorption for each blend were investigated in this work. The results showed that Blend-3 had the best CO2 absorption performance in terms of the CO2 equilibrium solubility, initial CO2 absorption rate and CO2 absorption capacity compared to Blend-1 and Blend-2 and 5M MEA. 13C NMR spectroscopy was used to quantify species formed in the CO2-loaded MEA-MDEA-PZ solution and the results shows that Blend-1 system produced more bicarbonate and less carbamate compared to Blend-2 and Blend-3 systems. The heat of CO2 absorption was calculated using Gibbs-Helmholtz equation and the results showed that MEA-MDEA-PZ systems had lower absorption heat than that of MEA, DEA, AMP, PZ and trio-amine blends of MEA-AMP-PZ. For the CO2 desorption performance, three blends studied in this work had lower relative energy consumption for the solvent regeneration compared to 5M MEA and Blend-1 showed the best desorption performance. Among these blends, an increase in molar ratio of MDEA/PZ in the blends led to a decrease in energy consumption and an increase in cyclic capacity and the CO2 desorption rate. In addition, the blend of MEA-MDEA-PZ reduced the energy consumption by 15.22–49.92% compared to 5M MEA.

Suggested Citation

  • Zhang, Rui & Zhang, Xiaowen & Yang, Qi & Yu, Hai & Liang, Zhiwu & Luo, Xiao, 2017. "Analysis of the reduction of energy cost by using MEA-MDEA-PZ solvent for post-combustion carbon dioxide capture (PCC)," Applied Energy, Elsevier, vol. 205(C), pages 1002-1011.
    • Handle: RePEc:eee:appene:v:205:y:2017:i:c:p:1002-1011
    DOI: 10.1016/j.apenergy.2017.08.130
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    15. Hosseini-Ardali, Seyed Mohsen & Hazrati-Kalbibaki, Majid & Fattahi, Moslem & Lezsovits, Ferenc, 2020. "Multi-objective optimization of post combustion CO2 capture using methyldiethanolamine (MDEA) and piperazine (PZ) bi-solvent," Energy, Elsevier, vol. 211(C).
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    17. Xiao, Min & Zheng, Wenchao & Liu, Helei & Luo, Xiao & Gao, Hongxia & Liang, Zhiwu, 2021. "Thermodynamic analysis of carbamate formation and carbon dioxide absorption in N-methylaminoethanol solution," Applied Energy, Elsevier, vol. 281(C).
    18. Meng, Fanzhi & Meng, Yuan & Ju, Tongyao & Han, Siyu & Lin, Li & Jiang, Jianguo, 2022. "Research progress of aqueous amine solution for CO2 capture: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 168(C).
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    20. Otitoju, Olajide & Oko, Eni & Wang, Meihong, 2021. "Technical and economic performance assessment of post-combustion carbon capture using piperazine for large scale natural gas combined cycle power plants through process simulation," Applied Energy, Elsevier, vol. 292(C).
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    Keywords

    Caron dioxide; Amine; MEA; MDEA; PZ; Energy;
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