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Formation of aromatic ring structures during the thermal treatment of mallee wood cylinders at low temperature

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  • Jiang, Shengjuan
  • Hu, Xun
  • Xia, Daohong
  • Li, Chun-Zhu

Abstract

Aromatics are important components in the tars from biomass gasification or in bio-oil from pyrolysis. This study investigated the formation of polycyclic aromatics during the thermal treatment of mallee wood at low temperature. The formation of tar was negligible below 200°C but became significant above 230°C. At the same time, the abundance of aromatics also became significant above 230°C. In addition, it was found that some aromatics were formed even at temperatures as low as 150°C. These aromatics were trapped in the resultant chars but could be extracted with solvents (i.e. methanol/chloroform). The abundance of trapped aromatics was different between the outer surface and the centre of the char (cylinder shape). FT-IR and UV-fluorescence analysis revealed that the aromatics contained polar functionalities (e.g. carbonyl groups) on the benzene rings. Some unsaturated hydroxyl aldehyde/ketone intermediates were formed in parallel with the aromatics.

Suggested Citation

  • Jiang, Shengjuan & Hu, Xun & Xia, Daohong & Li, Chun-Zhu, 2016. "Formation of aromatic ring structures during the thermal treatment of mallee wood cylinders at low temperature," Applied Energy, Elsevier, vol. 183(C), pages 542-551.
    • Handle: RePEc:eee:appene:v:183:y:2016:i:c:p:542-551
    DOI: 10.1016/j.apenergy.2016.09.015
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