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Numerical analysis of mass and heat transport in proton-conducting SOFCs with direct internal reforming

Author

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  • Menon, Vikram
  • Banerjee, Aayan
  • Dailly, Julian
  • Deutschmann, Olaf

Abstract

A computational model to investigate proton-conducting Solid-Oxide Fuel Cells (SOFCs) with direct internal reforming is developed. The numerical framework employs a 42-step elementary heterogeneous mechanism for Ni catalysts, using mean-field approximation. Mass transport through the porous media is described by the dusty gas model (DGM). Electrochemical parameters are deduced by reproducing two sets of experimental data, via the non-linear Butler–Volmer equation. A simple 1-D energy balance model is used to predict temperature profiles. The performance of the cell is analyzed by assuming the co-flow planar cell to be adiabatic. Simulations are carried out to understand the influence of various operating conditions on temperature distribution, species transport, and electrochemistry in the cell. The effect of dividing the anode into four zones, with different specific catalytic areas, on macroscopic performance parameters is investigated.

Suggested Citation

  • Menon, Vikram & Banerjee, Aayan & Dailly, Julian & Deutschmann, Olaf, 2015. "Numerical analysis of mass and heat transport in proton-conducting SOFCs with direct internal reforming," Applied Energy, Elsevier, vol. 149(C), pages 161-175.
    • Handle: RePEc:eee:appene:v:149:y:2015:i:c:p:161-175
    DOI: 10.1016/j.apenergy.2015.03.037
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    References listed on IDEAS

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    1. Hajimolana, S. Ahmad & Hussain, M. Azlan & Daud, W.M. Ashri Wan & Soroush, M. & Shamiri, A., 2011. "Mathematical modeling of solid oxide fuel cells: A review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 15(4), pages 1893-1917, May.
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    5. Kupecki, Jakub & Motylinski, Konrad & Milewski, Jaroslaw, 2018. "Dynamic analysis of direct internal reforming in a SOFC stack with electrolyte-supported cells using a quasi-1D model," Applied Energy, Elsevier, vol. 227(C), pages 198-205.
    6. Ouyang, Tiancheng & Zhang, Mingliang & Qin, Peijia & Liu, Wenjun & Shi, Xiaomin, 2022. "Converting waste into electric energy and carbon fixation through biosyngas-fueled SOFC hybrid system: A simulation study," Renewable Energy, Elsevier, vol. 193(C), pages 725-743.
    7. Kishimoto, Masashi & Kishida, Shohei & Seo, Haewon & Iwai, Hiroshi & Yoshida, Hideo, 2021. "Prediction of electrochemical characteristics of practical-size solid oxide fuel cells based on database of unit cell performance," Applied Energy, Elsevier, vol. 283(C).
    8. Han, Yuan & Gao, Wenzhi & Qin, Yanzhou, 2024. "Conceptual design and multi-objective optimization of a hybrid system based on direct ammonia protonic ceramic fuel cell and alkali metal thermal electric converter," Energy, Elsevier, vol. 297(C).
    9. Li, Ang & Song, Ce & Lin, Zijing, 2017. "A multiphysics fully coupled modeling tool for the design and operation analysis of planar solid oxide fuel cell stacks," Applied Energy, Elsevier, vol. 190(C), pages 1234-1244.
    10. Dai, Huidong & Besser, R.S., 2022. "Understanding hydrogen sulfide impact on a portable, commercial, propane-powered solid-oxide fuel cell," Applied Energy, Elsevier, vol. 307(C).
    11. Chien-Chang Wu & Tsung-Lin Chen, 2020. "Dynamic Modeling of a Parallel-Connected Solid Oxide Fuel Cell Stack System," Energies, MDPI, vol. 13(2), pages 1-20, January.
    12. Khojaste Effatpanah, Saeed & Rahbari, Hamid Reza & Ahmadi, Mohammad H. & Farzaneh, Ali, 2023. "Green hydrogen production and utilization in a novel SOFC/GT-based zero-carbon cogeneration system: A thermodynamic evaluation," Renewable Energy, Elsevier, vol. 219(P2).
    13. Silva-Mosqueda, Dulce María & Elizalde-Blancas, Francisco & Pumiglia, Davide & Santoni, Francesca & Boigues-Muñoz, Carlos & McPhail, Stephen J., 2019. "Intermediate temperature solid oxide fuel cell under internal reforming: Critical operating conditions, associated problems and their impact on the performance," Applied Energy, Elsevier, vol. 235(C), pages 625-640.
    14. Rashid, Kashif & Dong, Sang Keun & Mehran, Muhammad Taqi & Lee, Dong Won, 2017. "Design and analysis of compact hotbox for solid oxide fuel cell based 1kW-class power generation system," Applied Energy, Elsevier, vol. 208(C), pages 620-636.
    15. Shao, Qian & Gao, Enlai & Mara, Thierry & Hu, Heng & Liu, Tong & Makradi, Ahmed, 2020. "Global sensitivity analysis of solid oxide fuel cells with Bayesian sparse polynomial chaos expansions," Applied Energy, Elsevier, vol. 260(C).
    16. Emilio Audasso & Fiammetta Rita Bianchi & Barbara Bosio, 2020. "2D Simulation for CH 4 Internal Reforming-SOFCs: An Approach to Study Performance Degradation and Optimization," Energies, MDPI, vol. 13(16), pages 1-19, August.
    17. Emadi, Mohammad Ali & Chitgar, Nazanin & Oyewunmi, Oyeniyi A. & Markides, Christos N., 2020. "Working-fluid selection and thermoeconomic optimisation of a combined cycle cogeneration dual-loop organic Rankine cycle (ORC) system for solid oxide fuel cell (SOFC) waste-heat recovery," Applied Energy, Elsevier, vol. 261(C).
    18. Wang, Baoxuan & Zhu, Jiang & Lin, Zijing, 2016. "A theoretical framework for multiphysics modeling of methane fueled solid oxide fuel cell and analysis of low steam methane reforming kinetics," Applied Energy, Elsevier, vol. 176(C), pages 1-11.
    19. Ström, Henrik, 2017. "Computational optimization of catalyst distributions at the nano-scale," Applied Energy, Elsevier, vol. 185(P2), pages 2224-2231.
    20. Barelli, L. & Bidini, G. & Cinti, G. & Gallorini, F. & Pöniz, M., 2017. "SOFC stack coupled with dry reforming," Applied Energy, Elsevier, vol. 192(C), pages 498-507.

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