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Porous materials with optimal adsorption thermodynamics and kinetics for CO2 separation

Author

Listed:
  • Patrick Nugent

    (University of South Florida, 4202 East Fowler Avenue, Tampa, Florida 33620, USA)

  • Youssef Belmabkhout

    (Advanced Membranes and Porous Materials Center, 4700 King Abdullah University of Science and Technology (KAUST))

  • Stephen D. Burd

    (University of South Florida, 4202 East Fowler Avenue, Tampa, Florida 33620, USA)

  • Amy J. Cairns

    (Advanced Membranes and Porous Materials Center, 4700 King Abdullah University of Science and Technology (KAUST))

  • Ryan Luebke

    (Advanced Membranes and Porous Materials Center, 4700 King Abdullah University of Science and Technology (KAUST))

  • Katherine Forrest

    (University of South Florida, 4202 East Fowler Avenue, Tampa, Florida 33620, USA)

  • Tony Pham

    (University of South Florida, 4202 East Fowler Avenue, Tampa, Florida 33620, USA)

  • Shengqian Ma

    (University of South Florida, 4202 East Fowler Avenue, Tampa, Florida 33620, USA)

  • Brian Space

    (University of South Florida, 4202 East Fowler Avenue, Tampa, Florida 33620, USA)

  • Lukasz Wojtas

    (University of South Florida, 4202 East Fowler Avenue, Tampa, Florida 33620, USA)

  • Mohamed Eddaoudi

    (University of South Florida, 4202 East Fowler Avenue, Tampa, Florida 33620, USA
    Advanced Membranes and Porous Materials Center, 4700 King Abdullah University of Science and Technology (KAUST))

  • Michael J. Zaworotko

    (University of South Florida, 4202 East Fowler Avenue, Tampa, Florida 33620, USA)

Abstract

A series of porous crystalline materials known as metal–organic materials are prepared, and a full sorption study shows that controlled pore size (rather than large surface area) coupled with appropriate chemistry lead to materials exhibiting fast and highly selective CO2 sorption.

Suggested Citation

  • Patrick Nugent & Youssef Belmabkhout & Stephen D. Burd & Amy J. Cairns & Ryan Luebke & Katherine Forrest & Tony Pham & Shengqian Ma & Brian Space & Lukasz Wojtas & Mohamed Eddaoudi & Michael J. Zaworo, 2013. "Porous materials with optimal adsorption thermodynamics and kinetics for CO2 separation," Nature, Nature, vol. 495(7439), pages 80-84, March.
    • Handle: RePEc:nat:nature:v:495:y:2013:i:7439:d:10.1038_nature11893
    DOI: 10.1038/nature11893
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    Cited by:

    1. Jian Yu & Wenting He & Bin Liu, 2020. "Adsorption of Acid Orange Ⅱ with Two Step Modified Sepiolite: Optimization, Adsorption Performance, Kinetics, Thermodynamics and Regeneration," IJERPH, MDPI, vol. 17(5), pages 1-14, March.
    2. Wei Xia & Zhijie Zhou & Liangzheng Sheng & Lihang Chen & Fuxing Shen & Fang Zheng & Zhiguo Zhang & Qiwei Yang & Qilong Ren & Zongbi Bao, 2024. "Bioinspired recognition in metal-organic frameworks enabling precise sieving separation of fluorinated propylene and propane mixtures," Nature Communications, Nature, vol. 15(1), pages 1-9, December.
    3. Hengcong Huang & Luyao Wang & Xiaoyu Zhang & Hongshuo Zhao & Yifan Gu, 2022. "CO 2 -Selective Capture from Light Hydrocarbon Mixtures by Metal-Organic Frameworks: A Review," Clean Technol., MDPI, vol. 5(1), pages 1-24, December.
    4. Hong-Hua Qiu & Lu-Ge Liu, 2018. "A Study on the Evolution of Carbon Capture and Storage Technology Based on Knowledge Mapping," Energies, MDPI, vol. 11(5), pages 1-25, May.
    5. Bacsik, Zoltán & Cheung, Ocean & Vasiliev, Petr & Hedin, Niklas, 2016. "Selective separation of CO2 and CH4 for biogas upgrading on zeolite NaKA and SAPO-56," Applied Energy, Elsevier, vol. 162(C), pages 613-621.
    6. Qingju Wang & Lifeng Yang & Tian Ke & Jianbo Hu & Xian Suo & Xili Cui & Huabin Xing, 2024. "Selective sorting of hexane isomers by anion-functionalized metal-organic frameworks with optimal energy regulation," Nature Communications, Nature, vol. 15(1), pages 1-8, December.
    7. Jiyu Cui & Fang Wu & Wen Zhang & Lifeng Yang & Jianbo Hu & Yin Fang & Peng Ye & Qiang Zhang & Xian Suo & Yiming Mo & Xili Cui & Huajun Chen & Huabin Xing, 2023. "Direct prediction of gas adsorption via spatial atom interaction learning," Nature Communications, Nature, vol. 14(1), pages 1-9, December.
    8. Xinming Xia & Feng Zhou & Jing Xu & Zhongteng Wang & Jian Lan & Yan Fan & Zhikun Wang & Wei Liu & Junlang Chen & Shangshen Feng & Yusong Tu & Yizhou Yang & Liang Chen & Haiping Fang, 2022. "Unexpectedly efficient ion desorption of graphene-based materials," Nature Communications, Nature, vol. 13(1), pages 1-7, December.
    9. Dissanayake, Pavani Dulanja & You, Siming & Igalavithana, Avanthi Deshani & Xia, Yinfeng & Bhatnagar, Amit & Gupta, Souradeep & Kua, Harn Wei & Kim, Sumin & Kwon, Jung-Hwan & Tsang, Daniel C.W. & Ok, , 2020. "Biochar-based adsorbents for carbon dioxide capture: A critical review," Renewable and Sustainable Energy Reviews, Elsevier, vol. 119(C).
    10. Qingju Wang & Jianbo Hu & Lifeng Yang & Zhaoqiang Zhang & Tian Ke & Xili Cui & Huabin Xing, 2022. "One-step removal of alkynes and propadiene from cracking gases using a multi-functional molecular separator," Nature Communications, Nature, vol. 13(1), pages 1-8, December.
    11. Al-Qahtani, Amjad & Parkinson, Brett & Hellgardt, Klaus & Shah, Nilay & Guillen-Gosalbez, Gonzalo, 2021. "Uncovering the true cost of hydrogen production routes using life cycle monetisation," Applied Energy, Elsevier, vol. 281(C).
    12. Budzianowski, Wojciech M., 2016. "A review of potential innovations for production, conditioning and utilization of biogas with multiple-criteria assessment," Renewable and Sustainable Energy Reviews, Elsevier, vol. 54(C), pages 1148-1171.
    13. Xiuling Chen & Yanfang Fan & Lei Wu & Linzhou Zhang & Dong Guan & Canghai Ma & Nanwen Li, 2021. "Ultra-selective molecular-sieving gas separation membranes enabled by multi-covalent-crosslinking of microporous polymer blends," Nature Communications, Nature, vol. 12(1), pages 1-11, December.
    14. Yaumi, A.L. & Bakar, M.Z. Abu & Hameed, B.H., 2017. "Recent advances in functionalized composite solid materials for carbon dioxide capture," Energy, Elsevier, vol. 124(C), pages 461-480.
    15. Jingqi Wang & Jiapeng Liu & Hongshuai Wang & Musen Zhou & Guolin Ke & Linfeng Zhang & Jianzhong Wu & Zhifeng Gao & Diannan Lu, 2024. "A comprehensive transformer-based approach for high-accuracy gas adsorption predictions in metal-organic frameworks," Nature Communications, Nature, vol. 15(1), pages 1-14, December.
    16. Wang, Pengfei & Teng, Ying & Zhu, Jinlong & Bao, Wancheng & Han, Songbai & Li, Yun & Zhao, Yusheng & Xie, Heping, 2022. "Review on the synergistic effect between metal–organic frameworks and gas hydrates for CH4 storage and CO2 separation applications," Renewable and Sustainable Energy Reviews, Elsevier, vol. 167(C).

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