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Impact-resistant supercapacitor by hydrogel-infused lattice

Author

Listed:
  • Shixiang Zhou

    (National University of Singapore)

  • Yijing Zhao

    (National University of Singapore)

  • Kaixi Zhang

    (National University of Singapore)

  • Yanran Xun

    (National University of Singapore)

  • Xueyu Tao

    (China University of Mining and Technology)

  • Wentao Yan

    (National University of Singapore)

  • Wei Zhai

    (National University of Singapore)

  • Jun Ding

    (National University of Singapore)

Abstract

The safety of energy storage devices is increasingly crucial due to the growing requirements for application under harsh conditions. Effective methods for enhancing robustness without compromising functionality are necessary. Here we present an impact-resistant, ready-to-use supercapacitor constructed from self-healable hydrogel electrolyte-infused lattice electrodes. Three-dimensional-printed carbon-coated silicon oxycarbide current collectors provide mechanical protection, with compressive stress, Young’s modulus, and energy absorption up to 70.61 MPa, 2.75 GPa, and 92.15 kJ/m3, respectively. Commercially viable polyaniline and self-healable polyvinyl alcohol hydrogel are used as active coatings and electrolytes. I-wrapped package structured supercapacitor electrode exhibits a static specific capacitance of 585.51 mF/cm3 at 3 mA/cm3, with an energy density of 97.63 μWh/cm3 at a power density of 0.5 mW/cm3. It maintains operational integrity under extreme conditions, including post-impact with energy of 0.3 J/cm3, dynamic loading ranging from 0 to 18.83 MPa, and self-healing after electrolyte damage, demonstrating its promise for applications in extreme environments.

Suggested Citation

  • Shixiang Zhou & Yijing Zhao & Kaixi Zhang & Yanran Xun & Xueyu Tao & Wentao Yan & Wei Zhai & Jun Ding, 2024. "Impact-resistant supercapacitor by hydrogel-infused lattice," Nature Communications, Nature, vol. 15(1), pages 1-13, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-50707-0
    DOI: 10.1038/s41467-024-50707-0
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    References listed on IDEAS

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    1. Mohamed, Ahmed A.S. & Shaier, Ahmed A. & Metwally, Hamid & Selem, Sameh I., 2020. "A comprehensive overview of inductive pad in electric vehicles stationary charging," Applied Energy, Elsevier, vol. 262(C).
    2. Quyang Liu & Xinyu Dong & Haobo Qi & Haoqi Zhang & Tian Li & Yijing Zhao & Guanjin Li & Wei Zhai, 2024. "3D printable strong and tough composite organo-hydrogels inspired by natural hierarchical composite design principles," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    3. Jianxiang Cheng & Rong Wang & Zechu Sun & Qingjiang Liu & Xiangnan He & Honggeng Li & Haitao Ye & Xingxin Yang & Xinfeng Wei & Zhenqing Li & Bingcong Jian & Weiwei Deng & Qi Ge, 2022. "Centrifugal multimaterial 3D printing of multifunctional heterogeneous objects," Nature Communications, Nature, vol. 13(1), pages 1-10, December.
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