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Triboiontronics with temporal control of electrical double layer formation

Author

Listed:
  • Xiang Li

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Roujuan Li

    (Chinese Academy of Sciences
    University of Chinese Academy of Sciences)

  • Shaoxin Li

    (Chinese Academy of Sciences)

  • Zhong Lin Wang

    (Chinese Academy of Sciences
    Chinese Academy of Sciences
    Huangpu District
    Georgia Institute of Technology)

  • Di Wei

    (Chinese Academy of Sciences
    9 JJ Thomson Avenue)

Abstract

The nanoscale electrical double layer plays a crucial role in macroscopic ion adsorption and reaction kinetics. In this study, we achieve controllable ion migration by dynamically regulating asymmetric electrical double layer formation. This tailors the ionic-electronic coupling interface, leading to the development of triboiontronics. Controlling the charge-collecting layer coverage on dielectric substrates allows for charge collection and adjustment of the substrate-liquid contact electrification property. By dynamically managing the asymmetric electrical double layer formation between the dielectric substrate and liquids, we develop a direct-current triboiontronic nanogenerator. This nanogenerator produces a transferred charge density of 412.54 mC/m2, significantly exceeding that of current hydrovoltaic technology and conventional triboelectric nanogenerators. Additionally, incorporating redox reactions to the process enhances the peak power and transferred charge density to 38.64 W/m2 and 540.70 mC/m2, respectively.

Suggested Citation

  • Xiang Li & Roujuan Li & Shaoxin Li & Zhong Lin Wang & Di Wei, 2024. "Triboiontronics with temporal control of electrical double layer formation," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
  • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-50518-3
    DOI: 10.1038/s41467-024-50518-3
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