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Flash healing of laser-induced graphene

Author

Listed:
  • Le Cheng

    (City University of Hong Kong
    Shenzhen)

  • Chi Shun Yeung

    (City University of Hong Kong
    Shenzhen)

  • Libei Huang

    (City University of Hong Kong
    The Hong Kong Polytechnic University)

  • Ge Ye

    (City University of Hong Kong)

  • Jie Yan

    (City University of Hong Kong)

  • Wanpeng Li

    (City University of Hong Kong)

  • Chunki Yiu

    (City University of Hong Kong)

  • Fu-Rong Chen

    (City University of Hong Kong)

  • Hanchen Shen

    (Shenzhen (CUHK-Shenzhen))

  • Ben Zhong Tang

    (Shenzhen (CUHK-Shenzhen)
    The Hong Kong University of Science and Technology)

  • Yang Ren

    (City University of Hong Kong
    Kowloon)

  • Xinge Yu

    (City University of Hong Kong)

  • Ruquan Ye

    (City University of Hong Kong
    Shenzhen)

Abstract

The advancement of laser-induced graphene (LIG) technology has streamlined the fabrications of flexible graphene devices. However, the ultrafast kinetics triggered by laser irradiation generates intrinsic amorphous characteristics, leading to high resistivity and compromised performance in electronic devices. Healing graphene defects in specific patterns is technologically challenging by conventional methods. Herein, we report the rapid rectification of LIG’s topological defects by flash Joule heating in milliseconds (referred to as F-LIG), whilst preserving its overall structure and porosity. The F-LIG exhibits a decreased ID/IG ratio from 0.84 – 0.33 and increased crystalline domain from Raman analysis, coupled with a 5-fold surge in conductivity. Pair distribution function and atomic-resolution imaging delineate a broader-range order of F-LIG with a shorter C-C bond of 1.425 Å. The improved crystallinity and conductivity of F-LIG with excellent flexibility enables its utilization in high-performance soft electronics and low-voltage disinfections. Notably, our F-LIG/polydimethylsiloxane strain sensor exhibits a gauge factor of 129.3 within 10% strain, which outperforms pristine LIG by 800%, showcasing significant potential for human-machine interfaces.

Suggested Citation

  • Le Cheng & Chi Shun Yeung & Libei Huang & Ge Ye & Jie Yan & Wanpeng Li & Chunki Yiu & Fu-Rong Chen & Hanchen Shen & Ben Zhong Tang & Yang Ren & Xinge Yu & Ruquan Ye, 2024. "Flash healing of laser-induced graphene," Nature Communications, Nature, vol. 15(1), pages 1-11, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-024-47341-1
    DOI: 10.1038/s41467-024-47341-1
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    References listed on IDEAS

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    1. K. S. Novoselov & V. I. Fal′ko & L. Colombo & P. R. Gellert & M. G. Schwab & K. Kim, 2012. "A roadmap for graphene," Nature, Nature, vol. 490(7419), pages 192-200, October.
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