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Theory predicts 2D chiral polaritons based on achiral Fabry–Pérot cavities using apparent circular dichroism

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  • Andrew H. Salij

    (Northwestern University)

  • Randall H. Goldsmith

    (University of Wisconsin-Madison)

  • Roel Tempelaar

    (Northwestern University)

Abstract

Realizing polariton states with high levels of chirality offers exciting prospects for quantum information, sensing, and lasing applications. Such chirality must emanate from either the involved optical resonators or the quantum emitters. Here, we theoretically demonstrate a rare opportunity for realizing polaritons with so-called 2D chirality by strong coupling of the optical modes of (high finesse) achiral Fabry–Pérot cavities with samples exhibiting “apparent circular dichroism” (ACD). ACD is a phenomenon resulting from an interference between linear birefringence and dichroic interactions. By introducing a quantum electrodynamical theory of ACD, we identify the design rules based on which 2D chiral polaritons can be produced, and their chirality can be optimized.

Suggested Citation

  • Andrew H. Salij & Randall H. Goldsmith & Roel Tempelaar, 2024. "Theory predicts 2D chiral polaritons based on achiral Fabry–Pérot cavities using apparent circular dichroism," Nature Communications, Nature, vol. 15(1), pages 1-12, December.
    • Handle: RePEc:nat:natcom:v:15:y:2024:i:1:d:10.1038_s41467-023-44523-1
    DOI: 10.1038/s41467-023-44523-1
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    References listed on IDEAS

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    1. Peter Lodahl & Sahand Mahmoodian & Søren Stobbe & Arno Rauschenbeutel & Philipp Schneeweiss & Jürgen Volz & Hannes Pichler & Peter Zoller, 2017. "Chiral quantum optics," Nature, Nature, vol. 541(7638), pages 473-480, January.
    2. Charles R. Harris & K. Jarrod Millman & Stéfan J. Walt & Ralf Gommers & Pauli Virtanen & David Cournapeau & Eric Wieser & Julian Taylor & Sebastian Berg & Nathaniel J. Smith & Robert Kern & Matti Picu, 2020. "Array programming with NumPy," Nature, Nature, vol. 585(7825), pages 357-362, September.
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    Cited by:

    1. Tzu-Ling Chen & Andrew Salij & Katherine A. Parrish & Julia K. Rasch & Francesco Zinna & Paige J. Brown & Gennaro Pescitelli & Francesco Urraci & Laura A. Aronica & Abitha Dhavamani & Michael S. Arnol, 2024. "A 2D chiral microcavity based on apparent circular dichroism," Nature Communications, Nature, vol. 15(1), pages 1-11, December.

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